Exploring Novel Methods: Acid Treatment, Metal Nanoparticle Doping, and Graphene Insertion for Enhanced Electrical Conductivity of nm Thin PEDOT:PSS Films DOI Creative Commons
Amrita Chakraborty,

Aaron DiFilippo,

Sheena Deivasigamani

et al.

Synthetic Metals, Journal Year: 2024, Volume and Issue: 307, P. 117694 - 117694

Published: July 20, 2024

This study builds upon our previous research aimed at enhancing the electrical conductivity of Poly(3,4-ethylenedioxythiophene) Polystyrene Sulfonate (PEDOT:PSS). We investigate a range techniques, including acid treatments, doping with metal nanoparticles (Cu and Ag), deposition multiple PEDOT:PSS layers, incorporation mono/multiatomic layer graphene. Our investigations reveal that optimizing multilayers treating them nitric yields superior results compared to alternative methods employing optimized process not only enhances but also offers advantages in terms reduced errors, increased stability, cost-effectiveness when use graphene layers nanoparticles. Optimization parameters such as spinning speed, etchant concentration, etching time are crucial factors achieving these outcomes. Compared single-layer films same thickness, nine-layer treated demonstrates significant enhancement from 0.18 S/cm 15,699 S/cm. Furthermore, we address film aging mitigate reliability issues induced by ambient conditions.

Language: Английский

Two-Dimensional Materials for Highly Efficient and Stable Perovskite Solar Cells DOI Creative Commons
Xiangqian Shen, Xuesong Lin, Yong Peng

et al.

Nano-Micro Letters, Journal Year: 2024, Volume and Issue: 16(1)

Published: May 23, 2024

Perovskite solar cells (PSCs) offer low costs and high power conversion efficiency. However, the lack of long-term stability, primarily stemming from interfacial defects susceptible metal electrodes, hinders their practical application. In past few years, two-dimensional (2D) materials (e.g., graphene its derivatives, transitional dichalcogenides, MXenes, black phosphorus) have been identified as a promising solution to solving these problems because dangling bond-free surfaces, layer-dependent electronic band structures, tunable functional groups, inherent compactness. Here, recent progress 2D material toward efficient stable PSCs is summarized, including role both interface electrodes. We discuss beneficial effects on perovskite growth, energy level alignment, defect passivation, well blocking external stimulus. particular, unique properties form van der Waals heterojunction at bottom are emphasized. Finally, perspectives further development using provided, such designing high-quality heterojunction, enhancing uniformity coverage nanosheets, developing new materials-based

Language: Английский

Citations

28

Exploring the impact of cyano substitutions in non-fullerene acceptors for enhanced organic solar cell performance: A DFT and TD-DFT investigation DOI
Walid Taouali, Amel Azazi, Rym Hassani

et al.

Computational and Theoretical Chemistry, Journal Year: 2025, Volume and Issue: 1246, P. 115102 - 115102

Published: Feb. 3, 2025

Language: Английский

Citations

4

Advancements in tailoring PEDOT: PSS properties for bioelectronic applications: A comprehensive review DOI
Miriam Seiti, Antonella Giuri, Carola Esposito Corcione

et al.

Biomaterials Advances, Journal Year: 2023, Volume and Issue: 154, P. 213655 - 213655

Published: Oct. 10, 2023

Language: Английский

Citations

38

Recent advances in the construction and application of stretchable PEDOT smart electronic membranes DOI
Jia−Hua Chen,

Chunfa Ye,

Tianyu Cang

et al.

Journal of Materials Chemistry C, Journal Year: 2023, Volume and Issue: 11(43), P. 14930 - 14967

Published: Jan. 1, 2023

A comprehensive overview of stretchable PEDOT membranes for smart electronics, including structures, preparation strategies and recent applications.

Language: Английский

Citations

23

Solvent-doped PEDOT:PSS: Structural transformations towards enhanced electrical conductivity and transferable electromagnetic shields DOI Creative Commons

Hatef Yousefian,

Amin Babaei‐Ghazvini,

Ali Akbar Isari

et al.

Surfaces and Interfaces, Journal Year: 2024, Volume and Issue: 51, P. 104481 - 104481

Published: May 15, 2024

The enhanced electrical conductivity of solvent-doped poly(3,4-ethylenedioxythiophene): poly(styrene sulfonate) (PEDOT:PSS) is attributed to the screening effect between PSS and PEDOT chains. Yet, precise manner in which this influences crystalline structure conformation PEDOT:PSS remains unclear. In study, we utilize Raman spectroscopy, X-ray photoelectron spectroscopy (XPS), Grazing-incidence wide-angle scattering (GIWAXS) examine conformational changes two-dimensional (2D) when doped with a variety solvents, including dimethyl sulfoxide (DMSO), ethylene glycol (EG), dimethylformamide (DMF), methanol (MeOH), ethanol (EtOH), tetrahydrofuran (THF), acetone. Our observations unveil that solvent doping improves by modifying its structure. This alteration leads reduced inter-lamellar (d200) π-π stacking distance (d010), facilitating formation densely packed well-ordered crystallites both face-on edge-on orientations. Moreover, process enhances transferability mechanical properties drop-casted films, resulting flexible transferable electromagnetic interference (EMI) shield exceptional total shielding effectiveness (SET) 35.70 dB specific (SSE/t) 7105.34 cm2.g−1.

Language: Английский

Citations

14

The mechanism of enhancing the conductivity of PEDOT: PSS films through molecular weight optimization of PSS DOI
Qiao Fan, Kai Zhang, Shigui Peng

et al.

Progress in Organic Coatings, Journal Year: 2024, Volume and Issue: 189, P. 108308 - 108308

Published: Feb. 7, 2024

Language: Английский

Citations

11

Organic Metasurfaces with Contrasting Conducting Polymers DOI

Xiangyu Huang,

Robin Kaissner,

Benjamin Renz

et al.

Nano Letters, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 6, 2025

Conducting polymers have emerged as promising active materials for metasurfaces due to their electrically tunable states and large refractive index modulation. However, existing approaches are often limited infrared operation or single-polymer systems, restricting versatility. In this Letter, we present organic featuring dual conducting polymers, polyaniline (PANI) poly(3,4-ethylenedioxythiophene) (PEDOT), achieve contrasting dynamic optical responses at visible frequencies. Sequential electrochemical polymerizations locally conjugate subwavelength-thin layers of PANI PEDOT onto preselected gold nanorods, creating electro-plasmonic antennas with distinct optoelectronic properties. This dual-polymer approach enables metasurface pixel control without individual electrode routing, thereby simplifying designs. The exhibit dual-channel functions, including anomalous transmission holography, through the redox-state switching both polymers. Our work underscores potential applications, offering a pathway advanced reconfigurable devices

Language: Английский

Citations

1

Applied research and recent advances in the development of flexible sensing hydrogels from cellulose: A review DOI
Jinru Liu, Shenghua Lv, Yanlu Mu

et al.

International Journal of Biological Macromolecules, Journal Year: 2024, Volume and Issue: 281, P. 136100 - 136100

Published: Oct. 24, 2024

Language: Английский

Citations

7

Modulation of Charge Transport Layer for Perovskite Light‐Emitting Diodes DOI
Yuqing Li,

Xiang Guan,

Yaping Zhao

et al.

Advanced Materials, Journal Year: 2024, Volume and Issue: unknown

Published: Oct. 23, 2024

Abstract Perovskite light‐emitting diodes (Pero‐LEDs) have garnered significant attention due to their exceptional emission characteristics, including narrow full width at half maximum, high color purity, and tunable colors. Recent efficiency operational stability advancements positioned Pero‐LEDs as a promising next‐generation display technology. Extensive research review articles on the compositional engineering defect passivation of perovskite layers substantially contributed development multi‐color high‐efficiency Pero‐LEDs. However, crucial aspect charge transport layer (CTL) modulation in remains relatively underexplored. CTL not only impacts carrier injection balance but also plays critical role passivating surface, blocking ion migration, enhancing crystallinity, improving light extraction efficiency. Therefore, optimizing CTLs is pivotal for further Pero‐LED performance. Herein, this discusses roles categorizes both reported potential materials. Then, various optimization strategies are presented, alongside an analysis selection criteria high‐performance Finally, summary outlook advance performances provided.

Language: Английский

Citations

5

Advances in electrically functional nanocomposites: classification and future prospects DOI

Ziyuan Han,

Shifeng Cao, Suli Huang

et al.

Advanced Composites and Hybrid Materials, Journal Year: 2024, Volume and Issue: 7(6)

Published: Nov. 25, 2024

Language: Английский

Citations

5