Unanticipated optical properties of π-conjugated cyclometalated Pt(II) complexes for advanced information storage and anti-counterfeiting materials DOI
Yinghao Zhang,

Ke Shao,

Yihang Zhu

et al.

Chinese Chemical Letters, Journal Year: 2024, Volume and Issue: unknown, P. 110735 - 110735

Published: Dec. 1, 2024

Language: Английский

Multi-step FRET systems based on discrete supramolecular assemblies DOI Creative Commons

Dengli Chen,

Tangxin Xiao, Éric Monflier

et al.

Communications Chemistry, Journal Year: 2024, Volume and Issue: 7(1)

Published: April 18, 2024

Fluorescence resonance energy transfer (FRET) from the excited state of donor to ground acceptor is one most important fluorescence mechanisms and has wide applications in light-harvesting systems, light-mediated therapy, bioimaging, optoelectronic devices, information security fields. The phenomenon sequential natural photosynthetic systems provides great inspiration for scientists make full use light energy. In recent years, discrete supramolecular assemblies (DSAs) have been successively constructed incorporate multiple acceptors, achieve multi-step FRET between them. This perspective describes advances fabrication application DSAs with FRET. These are categorized based on non-covalent scaffolds, such as amphiphilic nanoparticles, host-guest assemblies, metal-coordination biomolecular scaffolds. will also outline opportunities future challenges this research area.

Language: Английский

Citations

17
A sequential light-harvesting system with thermosensitive colorimetric emission in both aqueous solution and hydrogel DOI
Lu Tang,

Zhiying Wu,

Qiaona Zhang

et al.

Chemical Communications, Journal Year: 2024, Volume and Issue: 60(35), P. 4719 - 4722

Published: Jan. 1, 2024

An artificial thermoresponsive light-harvesting system with sequential energy transfer has been successfully constructed, which shows thermosensitive colorimetric fluorescence in both aqueous solution and hydrogel.

Language: Английский

Citations

12
Supramolecular Sequential Light‐Harvesting Systems for Constructing White LED Device and Latent Fingerprint Imaging DOI

Qiaona Zhang,

Fengyao Cui,

Xiaoman Dang

et al.

Chemistry - A European Journal, Journal Year: 2024, Volume and Issue: 30(41)

Published: May 17, 2024

Abstract The fabrication of supramolecular light‐harvesting systems (LHS) with sequential energy transfer is significance in utilizing light energy. In this study, we report the non‐covalent self‐assembly a LHS by pillar[5]arene‐based host‐guest interaction water and its applications white light‐emitting diode (LED) device latent fingerprint imaging. complex WP5 G self‐assembles into nanoparticles shows enhanced aggregation‐induced emission (AIE) effect. can be further used to construct fluorescent dyes 4,7‐di(2‐thienyl)‐benzo[2,1,3]thiadiazole ( DBT ) sulforhodamine 101 SR101 ). Impressively, system white‐light when molar ratio / 1100/2/16. material coated on LED bulb achieve emission. addition, exhibit multicolor fluorescence including red emission, which have been successfully applied high‐resolution imaging fingerprints. Therefore, demonstrated general strategy for construction based macrocyclic explored multi‐functional fingerprints, will promote future development application LHSs.

Language: Английский

Citations

10
Supramolecular light-harvesting systems utilizing tetraphenylethylene chromophores as antennas DOI

Qiaona Zhang,

Xiaoman Dang,

Fengyao Cui

et al.

Chemical Communications, Journal Year: 2024, Volume and Issue: 60(74), P. 10064 - 10079

Published: Jan. 1, 2024

This comprehensive Feature Article summarizes the recent progress of supramolecular light-harvesting systems utilizing tetraphenylethylene (TPE) chromophores as antennas.

Language: Английский

Citations

10
Construction of a supramolecular light-harvesting system based on pillar[5]arene-mediated nanoparticles in water DOI Creative Commons
Xiuxiu Li,

Qiaona Zhang,

Xiaoman Dang

et al.

Energy Advances, Journal Year: 2024, Volume and Issue: 3(7), P. 1672 - 1677

Published: Jan. 1, 2024

An artificial light-harvesting system has been fabricated through the host–guest complexation of WP5 and CPy in water. The resultant materials show adjustable fluorescence have employed as a fluorescent ink for information encryption.

Language: Английский

Citations

4
Supramolecular light-harvesting systems based on cyanostilbene derivatives DOI Creative Commons

Fengyao Cui,

Qiaona Zhang,

Xiaoman Dang

et al.

Tetrahedron Chem, Journal Year: 2025, Volume and Issue: unknown, P. 100120 - 100120

Published: Jan. 1, 2025

Language: Английский

Citations

0
Multipath cascade light harvesting for multicolor luminescence based on macrocyclic sulfonatocalix[4]arene DOI
Wenwen Xu,

Yue‐Xiu Qin,

Xiao-Yong Yu

et al.

Chinese Chemical Letters, Journal Year: 2025, Volume and Issue: unknown, P. 111068 - 111068

Published: March 1, 2025

Language: Английский

Citations

0
Enhanced Emission in Polyelectrolyte Assemblies for the Development of Artificial Light‐Harvesting Systems and Color‐Tunable LED Device DOI
Qunpeng Duan, Xiuxiu Li,

Zhiying Wu

et al.

Macromolecular Rapid Communications, Journal Year: 2024, Volume and Issue: unknown

Published: Nov. 9, 2024

Artificial light-harvesting systems (LHSs) are of growing interest for their potential in energy capture and conversion, but achieving efficient fluorescence aqueous environments remains challenging. In this study, a novel tetraphenylethylene (TPE) derivative, TPEN, is synthesized co-assembled with poly(sodium 4-styrenesulfonate) (PSS) to enhance its via electrostatic interactions. The resulting PSS⊃TPEN network significantly increased blue emission, which further harnessed by an energy-matched dye, 4,7-di(2-thienyl)benzo[2,1,3]thiadiazole (DBT), produce LHS yellow emission. Moreover, system successfully applied develop color-tunable light-emitting diode (LED) devices. findings demonstrate cost-effective environmentally friendly approach designing tunable luminescent materials, promising future advancements energy-efficient lighting technologies.

Language: Английский

Citations

2
Luminescent terphen[3]arene sulfate-activated FRET assemblies for cell imaging DOI
Zhixue Liu, Haiqi Chen, Lijuan Guo

et al.

Chinese Chemical Letters, Journal Year: 2024, Volume and Issue: 35(9), P. 109666 - 109666

Published: Feb. 22, 2024

Language: Английский

Citations

1
Scaffold-Free Efficient Light-Harvesting Nanoparticles Based on One-Pot Self-Assembly of Donor–Acceptor Aggregation-Induced Emission Luminogens DOI
Chuanqi Li, Jiaxiang Yan, Bohan Yin

et al.

ACS Applied Nano Materials, Journal Year: 2024, Volume and Issue: 7(21), P. 24469 - 24476

Published: Oct. 17, 2024

Constructing highly efficient artificial light-harvesting (LH) systems via a scaffold-free approach for capturing and utilizing light energy to emulate photosynthesis-inspired transfer processes is great challenge. Herein, we report an nanoparticle (LHN) based on two derivatives of tetraphenylethylene as donor/acceptor (D/A) pair in skeleton compact effective stacking prepared by simple ultrasound-assisted self-assembly within ∼1 h water aggregation-induced emission (AIE) effect intermolecular transfer. By simply adjusting the D/A mixture ratio, LHN shows tunable multicolor (from cyan near-infrared) with remarkable efficiency 96.5% at ratio 50:1 attains high antenna 79.2 4000:1. Importantly, exhibits nearly pure white color coordinates (0.32, 0.35) 300:1 quantum yield 51%. Moreover, our biocompatibility brightness cellular imaging MCF-7 cells over 3 days. Compared direct excitation acceptors uptaken LHN, it approximately 14-fold enhancement cell brightness. This fabrication strategy opens up possibilities large-scale AIEgen-based luminescent materials potential applications fields real-time imaging.

Language: Английский

Citations

1