Sequential Dosing Strategies for Controlling Selectivity and Plasma-Phase Contributions in Plasma Catalysis DOI Creative Commons
Hope O. Otor, Jason C. Hicks

Energy & Fuels, Journal Year: 2025, Volume and Issue: unknown

Published: March 21, 2025

Plasma-assisted catalysis has advanced in recent years, particularly for transforming stable reactants at atmospheric pressure and ambient temperature. However, achieving a deeper understanding of the many plasma catalytic contributions remains significant goal, as improving product yield selectivity depends on proper catalyst selection, which is often challenging due to complex interplay between plasma-phase plasma-surface reactions. A sequential methodology emerged means decouple activity from In this approach, nonthermal used one step activate and/or convert gas phase or surface bound reactant, while second step, directs formation under steady-state temperature-programmed conditions. This review examines studies using technique reactions involving N2, CO2, SO2, offering insights into reaction mechanisms behavior/selection these transformations. These systematic provide framework that can be applied other plasma-assisted We also highlight remaining questions, propose directions future studies, discuss potential applying systems.

Language: Английский

Sequential Dosing Strategies for Controlling Selectivity and Plasma-Phase Contributions in Plasma Catalysis DOI Creative Commons
Hope O. Otor, Jason C. Hicks

Energy & Fuels, Journal Year: 2025, Volume and Issue: unknown

Published: March 21, 2025

Plasma-assisted catalysis has advanced in recent years, particularly for transforming stable reactants at atmospheric pressure and ambient temperature. However, achieving a deeper understanding of the many plasma catalytic contributions remains significant goal, as improving product yield selectivity depends on proper catalyst selection, which is often challenging due to complex interplay between plasma-phase plasma-surface reactions. A sequential methodology emerged means decouple activity from In this approach, nonthermal used one step activate and/or convert gas phase or surface bound reactant, while second step, directs formation under steady-state temperature-programmed conditions. This review examines studies using technique reactions involving N2, CO2, SO2, offering insights into reaction mechanisms behavior/selection these transformations. These systematic provide framework that can be applied other plasma-assisted We also highlight remaining questions, propose directions future studies, discuss potential applying systems.

Language: Английский

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