Journal of Colloid and Interface Science, Journal Year: 2024, Volume and Issue: 683, P. 1087 - 1095
Published: Dec. 19, 2024
Language: Английский
Journal of Colloid and Interface Science, Journal Year: 2024, Volume and Issue: 683, P. 1087 - 1095
Published: Dec. 19, 2024
Language: Английский
Advanced Materials, Journal Year: 2025, Volume and Issue: unknown
Published: Feb. 24, 2025
Developing high-performance single-atom catalysts (SACs) with maximum metal utilization efficiency is of significance, which presents enormous potentials to be extensively applied. It desired yet challenging elaborately tailor the coordination structures active sites in SACs and simultaneously enable sufficient accessibility these reactants. Here, a facile general strategy prepare conjugated polymer aerogels (CCPA) porous architectures that can markedly increase their elaborately-tailored sites, as new electrocatalyst paradigm fully present both structural advantages aerogel materials, reported. Taking nickel (Ni) an example, Ni-based CCPA (Ni-CCPA) its counterpart Ni-CCP non-aerogel feature are studied proof-of-concept case. Electrochemical measurements show that, relative Ni-CCP, Ni-CCPA exhibits appreciably higher performance toward alkaline oxygen evolution reaction (OER). Both experimental results theoretical simulations unravel improved OER arises from accelerated OH- diffusion within architecture enhanced concentration near highly exposed at high-curvature surfaces localized electric fields. Importantly, evidenced by Cu-CCPA Zn-CCPA examples, such promisingly applied targeted various catalytic reactions beyond.
Language: Английский
Citations
1Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: unknown, P. 158120 - 158120
Published: Nov. 1, 2024
Language: Английский
Citations
5Chinese Chemical Letters, Journal Year: 2025, Volume and Issue: unknown, P. 110830 - 110830
Published: Jan. 1, 2025
Language: Английский
Citations
0Journal of Colloid and Interface Science, Journal Year: 2024, Volume and Issue: 683, P. 1087 - 1095
Published: Dec. 19, 2024
Language: Английский
Citations
3