Bioenzyme Inspired Heterointerface Construction of NiFeSe/Ni3S2 for Improved Overall Water Splitting
Xiuling Xu,
No information about this author
Fumin Wang,
No information about this author
Liwen Wang
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et al.
Inorganic Chemistry,
Journal Year:
2025,
Volume and Issue:
unknown
Published: April 3, 2025
Electrocatalytic
water
splitting
for
hydrogen
production
represents
a
crucial
pathway
toward
establishing
sustainable
energy
infrastructure
and
addressing
environmental
concerns,
with
the
development
of
high-performance
nonprecious
metal
catalysts
being
central
focus.
While
Ni3S2
demonstrates
potential
as
an
electrocatalyst,
its
limited
functionality
suboptimal
performance
necessitate
further
enhancement.
In
this
study,
drawing
inspiration
from
natural
hydrogenases,
we
engineered
novel
NiFeSe/Ni3S2
composite
electrocatalyst
through
integration
NiFeSe
Ni3S2.
The
synthesized
catalyst
displayed
outstanding
overall
water-splitting
in
alkaline
media,
realizing
current
densities
100
10
mA
cm-2
at
remarkably
low
overpotentials
267.4
mV
(vs
RHE)
oxygen
evolution
reaction
(OER)
105.6
(HER),
respectively.
Remarkably,
two-electrode
electrolyzer
incorporating
achieved
density
20
substantially
reduced
cell
voltage
1.586
V.
Comprehensive
analysis
revealed
that
strategic
construction
biomimetic
active
centers
heterogeneous
interfaces
significantly
modulates
electronic
structure,
improved
charge
transfer,
redistribution
electron
catalytic
sites.
This
investigation
provides
valuable
insights
promising
framework
rational
design
bifunctional
electrocatalysts
applications.
Language: Английский
Flower-Sphere CoNiCuMnFe/C High-Entropy Alloy Catalysts for Enhanced Oxygen Evolution Reaction Kinetics
Z.H. Wang,
No information about this author
Kezhen Gao,
No information about this author
Xiao Yan
No information about this author
et al.
Journal of Alloys and Compounds,
Journal Year:
2025,
Volume and Issue:
unknown, P. 180421 - 180421
Published: April 1, 2025
Language: Английский
The Recent Progress of High-Entropy Layered Double Hydroxides and High-Entropy Amorphous Materials for Water Electrocatalysis
DeCarbon,
Journal Year:
2025,
Volume and Issue:
unknown, P. 100110 - 100110
Published: April 1, 2025
Language: Английский
Rational phosphorization of ferrocene-based metal organic framework for enhanced oxygen evolution and urea oxidation performance
Applied Surface Science,
Journal Year:
2024,
Volume and Issue:
680, P. 161392 - 161392
Published: Oct. 3, 2024
Language: Английский
Understanding the evolution of high-entropy oxide OER electrocatalyst with anion regulation
Dan Wang,
No information about this author
Yihang Yu,
No information about this author
Huan He
No information about this author
et al.
International Journal of Hydrogen Energy,
Journal Year:
2024,
Volume and Issue:
92, P. 639 - 647
Published: Oct. 29, 2024
Language: Английский
Ionic Liquid-Assisted Sustainable Preparation of Photo-catalytically Active Nanomaterials and their Composites with 2D Materials
Kanica Sharma,
No information about this author
Tejwant Singh Kang
No information about this author
Chemical Communications,
Journal Year:
2024,
Volume and Issue:
60(99), P. 14717 - 14732
Published: Jan. 1, 2024
This
feature
article
highlights
the
contribution
of
ionic
liquids,
as
better
alternatives
to
conventional
solvating
and
templating
media,
in
sustainable
synthesis
anisotropic
photo-catalytically
active
nanoparticles
their
composites.
Language: Английский