ACS Nano,
Journal Year:
2023,
Volume and Issue:
17(12), P. 11679 - 11691
Published: June 5, 2023
The
discovery
of
room-temperature
single-photon
emitters
(SPEs)
hosted
by
two-dimensional
hexagonal
boron
nitride
(2D
hBN)
has
sparked
intense
research
interest.
Although
in
the
vicinity
2
eV
have
been
studied
extensively,
their
microscopic
identity
remained
elusive.
discussion
this
class
SPEs
centered
on
point
defects
hBN
crystal
lattice,
but
none
candidate
defect
structures
able
to
capture
great
heterogeneity
emitter
properties
that
is
observed
experimentally.
Employing
a
widely
used
sample
preparation
protocol
disentangling
several
confounding
factors,
we
demonstrate
conclusively
heterogeneous
emission
~2
associated
with
originates
from
organic
molecules,
presumably
aromatic
fluorophores.
appearance
those
depends
critically
presence
processing
residues
during
preparation,
and
formed
heat
treatment
are
not
located
within
as
previously
thought,
at
hBN/substrate
interface.
We
further
same
can
be
different
2D
insulator,
fluorophlogopite
mica.
ACS Photonics,
Journal Year:
2022,
Volume and Issue:
9(5), P. 1434 - 1457
Published: April 18, 2022
In
the
last
two
decades,
bulk,
homoepitaxial,
and
heteroepitaxial
growth
of
silicon
carbide
(SiC)
has
witnessed
many
advances,
giving
rise
to
electronic
devices
widely
used
in
high-power
high-frequency
applications.
Recent
research
revealed
that
SiC
also
exhibits
unique
optical
properties
can
be
utilized
for
novel
photonic
devices.
is
a
transparent
material
from
UV
infrared,
possess
nonlinear
visible
mid-infrared
it
meta-material
range.
fluorescence
due
color
centers
associated
with
single
photon
emitters
as
spin
qubits
quantum
computation
communication
networks
sensing.
This
combination
excellent
electronic,
spintronic
prompted
develop
sensors
technology
domain.
this
perspective,
we
highlight
progress,
current
trends
prospects
science
underpinning
development
classical
Specifically,
lay
out
main
steps
recently
undertaken
achieve
high
quality
components,
outline
some
challenges
faces
establish
its
relevance
viable
technology.
We
will
focus
on
potential
bridge
gap
between
photonics,
technologically
advance
sensing
finally
provide
an
outlook
possible
alternative
applications
where
electronics,
spintronics
could
merge.
Advances in Physics X,
Journal Year:
2023,
Volume and Issue:
8(1)
Published: April 29, 2023
Color
centers
in
hexagonal
boron
nitride
(hBN)
have
recently
emerged
as
promising
candidates
for
a
new
wave
of
quantum
applications.
Thanks
to
hBN's
high
stability
and
two-dimensional
(2D)
layered
structure,
color
hBN
can
be
readily
integrated
into
nanophotonic
plasmonic
structures
on
chip.
More
importantly,
the
discovered
optically
addressable
spin
defects
provide
interface
between
photons
electron
spins
sensing
The
most
well-studied
defects,
negatively
charged
vacancy
(VB−)
been
used
static
magnetic
fields,
noise,
temperature,
strain,
nuclear
spins,
paramagnetic
liquids,
RF
signals,
beyond.
In
particular,
nanosheets
with
form
van
der
Waals
(vdW)
heterostructures
other
2D
materials
situ
imaging.
This
review
summarizes
rapidly
evolving
field
hBN.
We
introduce
basic
properties
protocols,
recent
experimental
demonstrations
imaging
defects.
also
discuss
methods
enhance
their
sensitivity.
Finally,
we
envision
some
potential
developments
applications
Physical Review Letters,
Journal Year:
2021,
Volume and Issue:
126(8)
Published: Feb. 22, 2021
We
report
the
detection
of
individual
emitters
in
silicon
belonging
to
seven
different
families
optically-active
point
defects.
These
fluorescent
centers
are
created
by
carbon
implantation
a
commercial
silicon-on-insulator
wafer
usually
employed
for
integrated
photonics.
Single
photon
emission
is
demonstrated
over
[1.1,1.55]-$\mu$m
range,
spanning
O-
and
C-telecom
bands.
analyse
their
photoluminescence
spectrum,
dipolar
optical
relaxation
dynamics
at
10K.
For
specific
family,
we
show
constant
intensity
saturation
from
10K
temperatures
well
above
77K-liquid
nitrogen
temperature.
Given
advanced
control
nanofabrication
integration
silicon,
these
novel
artificial
atoms
promising
candidates
Si-based
quantum
technologies.
Advanced Materials,
Journal Year:
2022,
Volume and Issue:
35(27)
Published: Feb. 9, 2022
Quantum
information
science
and
engineering
(QISE)
which
entails
use
of
quantum
mechanical
states
for
processing,
communications,
sensing
the
area
nanoscience
nanotechnology
have
dominated
condensed
matter
physics
materials
research
in
21st
century.
Solid
state
devices
QISE
have,
to
this
point,
predominantly
been
designed
with
bulk
as
their
constituents.
In
review,
we
consider
how
nanomaterials
(i.e.
intrinsic
confinement)
may
offer
inherent
advantages
over
conventional
QISE.
We
identify
challenges
specific
types
qubits,
emerging
overcome
these
challenges.
Challenges
progress
towards
based
are
identified.
aim
help
close
gap
between
communities
inspire
that
will
lead
next
generation
scalable
practical
applications.
ACS Photonics,
Journal Year:
2022,
Volume and Issue:
9(7), P. 2337 - 2345
Published: July 5, 2022
Controlling
the
quantum
properties
of
individual
fluorescent
defects
in
silicon
is
a
key
challenge
towards
advanced
photonic
devices
prone
to
scalability.
Research
efforts
have
so
far
focused
on
extrinsic
based
impurities
incorporated
inside
lattice.
Here
we
demonstrate
detection
single
intrinsic
silicon,
which
are
linked
tri-interstitial
complex
called
W-center,
with
zero-phonon
line
at
1.218${\mu}$m.
Investigating
their
single-photon
emission
reveals
new
information
about
this
common
radiation
damage
center,
such
as
its
dipolar
orientation
and
photophysics.
We
also
identify
microscopic
structure
show
that
although
defect
does
not
feature
electronic
states
bandgap,
Coulomb
interactions
lead
excitonic
radiative
recombination
below
bandgap.
These
results
could
set
stage
for
numerous
perspectives
luminescent
integrated
photonics,
communications
sensing.
Nature Communications,
Journal Year:
2022,
Volume and Issue:
13(1)
Published: July 27, 2022
Spin
defects
in
hexagonal
boron
nitride
(hBN)
are
promising
quantum
systems
for
the
design
of
flexible
two-dimensional
sensing
platforms.
Here
we
rely
on
hBN
crystals
isotopically
enriched
with
either
Materials for Quantum Technology,
Journal Year:
2022,
Volume and Issue:
2(3), P. 032002 - 032002
Published: July 5, 2022
Abstract
Quantum
technology
grown
out
of
quantum
information
theory,
including
communication,
computation
and
sensing,
not
only
provides
powerful
research
tools
for
numerous
fields,
but
also
is
expected
to
go
civilian
use
in
the
future.
Solid-state
spin-active
defects
are
one
promising
platforms
technology,
host
materials
include
three-dimensional
diamond
silicon
carbide,
emerging
two-dimensional
hexagonal
boron
nitride
(hBN)
transition-metal
dichalcogenides.
In
this
review,
we
will
focus
on
spin
hBN,
summarize
theoretical
experimental
progresses
made
understanding
properties
these
defects.
particular,
combination
prediction
verification
highlighted.
We
discuss
future
advantages
challenges
solid-state
spins
hBN
path
towards
applications.
Advanced Quantum Technologies,
Journal Year:
2023,
Volume and Issue:
6(9)
Published: July 3, 2023
Abstract
Achieving
fast,
sensitive,
and
parallel
measurement
of
a
large
number
quantum
particles
is
an
essential
task
in
building
large‐scale
platforms
for
different
information
processing
applications
such
as
sensing,
computation,
simulation,
communication.
Current
experimental
atomic
optical
physics
based
on
CMOS
sensors
charged
coupled
device
cameras
are
limited
by
either
low
sensitivity
or
slow
operational
speed.
Here
array
single‐photon
avalanche
diodes
integrated
with
solid‐state
spin
defects
diamond
to
build
fast
wide‐field
sensor,
achieving
frame
rate
up
100
kHz.
The
design
the
setup
perform
spatially
resolved
imaging
systems
presented.
A
few
exemplary
applications,
including
sensing
DC
AC
magnetic
fields,
temperature,
strain,
local
density,
charge
dynamics,
experimentally
demonstrated
using
nitrogen‐vacancy
ensemble
sample.
developed
photon
detection
broadly
applicable
other
atom
arrays
trapped
tweezers,
lattices,
donors
silicon,
rare
earth
ions
solids.
Nanophotonics,
Journal Year:
2023,
Volume and Issue:
12(3), P. 359 - 397
Published: Jan. 31, 2023
Solid-state
defects
acting
as
single
photon
sources
and
quantum
bits
are
leading
contenders
in
technologies.
Despite
great
efforts,
not
all
the
properties
behaviours
of
presently
known
solid-state
defect
understood.
Furthermore,
various
technologies
require
novel
solutions,
thus
new
should
be
explored
to
this
end.
These
issues
call
develop