Organic Molecules as Origin of Visible-Range Single Photon Emission from Hexagonal Boron Nitride and Mica DOI
Michael Neumann,

Xu Wei,

Luis Morales‐Inostroza

et al.

ACS Nano, Journal Year: 2023, Volume and Issue: 17(12), P. 11679 - 11691

Published: June 5, 2023

The discovery of room-temperature single-photon emitters (SPEs) hosted by two-dimensional hexagonal boron nitride (2D hBN) has sparked intense research interest. Although in the vicinity 2 eV have been studied extensively, their microscopic identity remained elusive. discussion this class SPEs centered on point defects hBN crystal lattice, but none candidate defect structures able to capture great heterogeneity emitter properties that is observed experimentally. Employing a widely used sample preparation protocol disentangling several confounding factors, we demonstrate conclusively heterogeneous emission ~2 associated with originates from organic molecules, presumably aromatic fluorophores. appearance those depends critically presence processing residues during preparation, and formed heat treatment are not located within as previously thought, at hBN/substrate interface. We further same can be different 2D insulator, fluorophlogopite mica.

Language: Английский

Optical observation of single spins in silicon DOI
Daniel Higginbottom,

A. T. K. Kurkjian,

Camille Chartrand

et al.

Nature, Journal Year: 2022, Volume and Issue: 607(7918), P. 266 - 270

Published: July 13, 2022

Language: Английский

Citations

109

Silicon Carbide Photonics Bridging Quantum Technology DOI
Stefania Castelletto, Alberto Peruzzo, Cristian Bonato

et al.

ACS Photonics, Journal Year: 2022, Volume and Issue: 9(5), P. 1434 - 1457

Published: April 18, 2022

In the last two decades, bulk, homoepitaxial, and heteroepitaxial growth of silicon carbide (SiC) has witnessed many advances, giving rise to electronic devices widely used in high-power high-frequency applications. Recent research revealed that SiC also exhibits unique optical properties can be utilized for novel photonic devices. is a transparent material from UV infrared, possess nonlinear visible mid-infrared it meta-material range. fluorescence due color centers associated with single photon emitters as spin qubits quantum computation communication networks sensing. This combination excellent electronic, spintronic prompted develop sensors technology domain. this perspective, we highlight progress, current trends prospects science underpinning development classical Specifically, lay out main steps recently undertaken achieve high quality components, outline some challenges faces establish its relevance viable technology. We will focus on potential bridge gap between photonics, technologically advance sensing finally provide an outlook possible alternative applications where electronics, spintronics could merge.

Language: Английский

Citations

76

Quantum sensing and imaging with spin defects in hexagonal boron nitride DOI Creative Commons
Sumukh Vaidya, Xingyu Gao,

Saakshi Dikshit

et al.

Advances in Physics X, Journal Year: 2023, Volume and Issue: 8(1)

Published: April 29, 2023

Color centers in hexagonal boron nitride (hBN) have recently emerged as promising candidates for a new wave of quantum applications. Thanks to hBN's high stability and two-dimensional (2D) layered structure, color hBN can be readily integrated into nanophotonic plasmonic structures on chip. More importantly, the discovered optically addressable spin defects provide interface between photons electron spins sensing The most well-studied defects, negatively charged vacancy (VB−) been used static magnetic fields, noise, temperature, strain, nuclear spins, paramagnetic liquids, RF signals, beyond. In particular, nanosheets with form van der Waals (vdW) heterostructures other 2D materials situ imaging. This review summarizes rapidly evolving field hBN. We introduce basic properties protocols, recent experimental demonstrations imaging defects. also discuss methods enhance their sensitivity. Finally, we envision some potential developments applications

Language: Английский

Citations

43

Broad Diversity of Near-Infrared Single-Photon Emitters in Silicon DOI
Alrik Durand, Yoann Baron, Walid Redjem

et al.

Physical Review Letters, Journal Year: 2021, Volume and Issue: 126(8)

Published: Feb. 22, 2021

We report the detection of individual emitters in silicon belonging to seven different families optically-active point defects. These fluorescent centers are created by carbon implantation a commercial silicon-on-insulator wafer usually employed for integrated photonics. Single photon emission is demonstrated over [1.1,1.55]-$\mu$m range, spanning O- and C-telecom bands. analyse their photoluminescence spectrum, dipolar optical relaxation dynamics at 10K. For specific family, we show constant intensity saturation from 10K temperatures well above 77K-liquid nitrogen temperature. Given advanced control nanofabrication integration silicon, these novel artificial atoms promising candidates Si-based quantum technologies.

Language: Английский

Citations

91

Nanomaterials for Quantum Information Science and Engineering DOI
Adam Alfieri, Surendra B. Anantharaman, Huiqin Zhang

et al.

Advanced Materials, Journal Year: 2022, Volume and Issue: 35(27)

Published: Feb. 9, 2022

Quantum information science and engineering (QISE) which entails use of quantum mechanical states for processing, communications, sensing the area nanoscience nanotechnology have dominated condensed matter physics materials research in 21st century. Solid state devices QISE have, to this point, predominantly been designed with bulk as their constituents. In review, we consider how nanomaterials (i.e. intrinsic confinement) may offer inherent advantages over conventional QISE. We identify challenges specific types qubits, emerging overcome these challenges. Challenges progress towards based are identified. aim help close gap between communities inspire that will lead next generation scalable practical applications.

Language: Английский

Citations

66

Detection of Single W-Centers in Silicon DOI
Yoann Baron, Alrik Durand, Péter Udvarhelyi

et al.

ACS Photonics, Journal Year: 2022, Volume and Issue: 9(7), P. 2337 - 2345

Published: July 5, 2022

Controlling the quantum properties of individual fluorescent defects in silicon is a key challenge towards advanced photonic devices prone to scalability. Research efforts have so far focused on extrinsic based impurities incorporated inside lattice. Here we demonstrate detection single intrinsic silicon, which are linked tri-interstitial complex called W-center, with zero-phonon line at 1.218${\mu}$m. Investigating their single-photon emission reveals new information about this common radiation damage center, such as its dipolar orientation and photophysics. We also identify microscopic structure show that although defect does not feature electronic states bandgap, Coulomb interactions lead excitonic radiative recombination below bandgap. These results could set stage for numerous perspectives luminescent integrated photonics, communications sensing.

Language: Английский

Citations

61

Decoherence of V$${}_{{{{{{{{\rm{B}}}}}}}}}^{-}$$ spin defects in monoisotopic hexagonal boron nitride DOI Creative Commons
Angela Haykal,

Rana Tanos,

Noel Minotto

et al.

Nature Communications, Journal Year: 2022, Volume and Issue: 13(1)

Published: July 27, 2022

Spin defects in hexagonal boron nitride (hBN) are promising quantum systems for the design of flexible two-dimensional sensing platforms. Here we rely on hBN crystals isotopically enriched with either

Language: Английский

Citations

55

Spin-active defects in hexagonal boron nitride DOI Creative Commons
Wei Liu,

Nai‐Jie Guo,

Shang Yu

et al.

Materials for Quantum Technology, Journal Year: 2022, Volume and Issue: 2(3), P. 032002 - 032002

Published: July 5, 2022

Abstract Quantum technology grown out of quantum information theory, including communication, computation and sensing, not only provides powerful research tools for numerous fields, but also is expected to go civilian use in the future. Solid-state spin-active defects are one promising platforms technology, host materials include three-dimensional diamond silicon carbide, emerging two-dimensional hexagonal boron nitride (hBN) transition-metal dichalcogenides. In this review, we will focus on spin hBN, summarize theoretical experimental progresses made understanding properties these defects. particular, combination prediction verification highlighted. We discuss future advantages challenges solid-state spins hBN path towards applications.

Language: Английский

Citations

42

Fast Wide‐Field Quantum Sensor Based on Solid‐State Spins Integrated with a SPAD Array DOI Creative Commons
Guoqing Wang, Francesca Madonini, Boning Li

et al.

Advanced Quantum Technologies, Journal Year: 2023, Volume and Issue: 6(9)

Published: July 3, 2023

Abstract Achieving fast, sensitive, and parallel measurement of a large number quantum particles is an essential task in building large‐scale platforms for different information processing applications such as sensing, computation, simulation, communication. Current experimental atomic optical physics based on CMOS sensors charged coupled device cameras are limited by either low sensitivity or slow operational speed. Here array single‐photon avalanche diodes integrated with solid‐state spin defects diamond to build fast wide‐field sensor, achieving frame rate up 100 kHz. The design the setup perform spatially resolved imaging systems presented. A few exemplary applications, including sensing DC AC magnetic fields, temperature, strain, local density, charge dynamics, experimentally demonstrated using nitrogen‐vacancy ensemble sample. developed photon detection broadly applicable other atom arrays trapped tweezers, lattices, donors silicon, rare earth ions solids.

Language: Английский

Citations

35

Recent advances in theab initiotheory of solid-state defect qubits DOI Creative Commons
Ádám Gali

Nanophotonics, Journal Year: 2023, Volume and Issue: 12(3), P. 359 - 397

Published: Jan. 31, 2023

Solid-state defects acting as single photon sources and quantum bits are leading contenders in technologies. Despite great efforts, not all the properties behaviours of presently known solid-state defect understood. Furthermore, various technologies require novel solutions, thus new should be explored to this end. These issues call develop

Language: Английский

Citations

29