Environmentally Friendly and Earth-Abundant Self-Healing Electrocatalyst Systems for Durable and Efficient Acidic Water Splitting DOI
Xuan Minh Chau Ta, Thành Trần‐Phú, Thi Kim Anh Nguyen

et al.

ACS Applied Materials & Interfaces, Journal Year: 2025, Volume and Issue: unknown

Published: April 21, 2025

Electrochemical water splitting under acidic conditions is an efficient route for green hydrogen production from renewable electricity. Its implementation on a globally relevant scale hindered by the lack of abundant and low-cost electrocatalysts oxygen evolution reaction that can operate stably efficiently highly anodic conditions. Here, we report design stable OER consisting self-healing bismuth (Bi)-based matrix hosting transition metal active sites. Comprehensive structural performance investigation Co- Ni-BiOx electrodes provides insights into role electrolyte composition pH in mechanism Our best-performing [Co-Bi]Ox [Ni-Bi]Ox anodes achieve over 200 h continuous electrolysis at catalytic current 10 mA cm-2 with overpotential 590 670 mV 1 0.1 M H2SO4 electrolyte. Notably, while [Bi]Ox did not contribute to activity, it was essential stabilize Co Ni sites during OER. findings provide promising strategy engineering earth-abundant materials splitting, as alternative use poorly scalable expensive noble catalysts.

Language: Английский

Recent Progress on the Stability of Electrocatalysts under High Current Densities toward Industrial Water Splitting DOI

Shumin Gong,

Yao Meng,

Zeying Jin

et al.

ACS Catalysis, Journal Year: 2024, Volume and Issue: unknown, P. 14399 - 14435

Published: Sept. 14, 2024

Language: Английский

Citations

11
Stable Dual Metal Oxide Matrix for Tuning Selectivity in Acidic Electrochemical Carbon Dioxide Reduction DOI Creative Commons

Ziling Zhang,

Thành Trần‐Phú, Jodie A. Yuwono

et al.

Applied Catalysis B Environment and Energy, Journal Year: 2025, Volume and Issue: unknown, P. 125203 - 125203

Published: Feb. 1, 2025

Language: Английский

Citations

0
Environmentally Friendly and Earth-Abundant Self-Healing Electrocatalyst Systems for Durable and Efficient Acidic Water Splitting DOI
Xuan Minh Chau Ta, Thành Trần‐Phú, Thi Kim Anh Nguyen

et al.

ACS Applied Materials & Interfaces, Journal Year: 2025, Volume and Issue: unknown

Published: April 21, 2025

Electrochemical water splitting under acidic conditions is an efficient route for green hydrogen production from renewable electricity. Its implementation on a globally relevant scale hindered by the lack of abundant and low-cost electrocatalysts oxygen evolution reaction that can operate stably efficiently highly anodic conditions. Here, we report design stable OER consisting self-healing bismuth (Bi)-based matrix hosting transition metal active sites. Comprehensive structural performance investigation Co- Ni-BiOx electrodes provides insights into role electrolyte composition pH in mechanism Our best-performing [Co-Bi]Ox [Ni-Bi]Ox anodes achieve over 200 h continuous electrolysis at catalytic current 10 mA cm-2 with overpotential 590 670 mV 1 0.1 M H2SO4 electrolyte. Notably, while [Bi]Ox did not contribute to activity, it was essential stabilize Co Ni sites during OER. findings provide promising strategy engineering earth-abundant materials splitting, as alternative use poorly scalable expensive noble catalysts.

Language: Английский

Citations

0