Impact of terahertz short pulses on the oxygen defect state in TiO2x DOI Creative Commons
Paola Di Pietro, Johannes Schmidt, Nidhi Adhlakha

et al.

Physical Review Research, Journal Year: 2025, Volume and Issue: 7(2)

Published: April 3, 2025

Oxygen-deficient titanium dioxide (TiO2x) is a very attractive material for several applications ranging from photocatalysis to resistive switching. Oxygen vacancies turn insulating anatase into polaronic conductor, while creating defect-state band below the ultraviolet semiconducting gap. Here we employ combination of broadband infrared (IR) reflectivity and THz-pump/IR-probe measurements investigate relationship between localized defect states delocalized conducting states. We show that THz pump allows convert deeply electrons metastable polarons with lifetime in ns range. These long-lived may find application novel optoelectronic exploiting interplay dc resistivity, terahertz signals. Published by American Physical Society 2025

Language: Английский

Hybrid Ferroelectric Tunnel Junctions: State of the Art, Challenges, and Opportunities DOI

King-Fa Luo,

Zhijun Ma, Daniel Sando

et al.

ACS Nano, Journal Year: 2025, Volume and Issue: unknown

Published: Feb. 12, 2025

Ferroelectric tunnel junctions (FTJs) harness the combination of ferroelectricity and quantum tunneling thus herald opportunities in next-generation nonvolatile memory technologies. Recent advancements fabrication ultrathin heterostructures have enabled integration ferroelectrics with various functional materials, forming hybrid tunneling-diode junctions. These benefit from modulation layer/ferroelectric interface through ferroelectric polarization, enabling further modalities capabilities addition to electroresistance. This Perspective aims provide in-depth insight into physical phenomena several typical junctions, ranging ferroelectric/dielectric, ferroelectric/multiferroic, ferroelectric/superconducting ferroelectric/2D finally their expansion realm resonant diodes (FeRTDs). latter aspect, i.e., tunneling, offers an approach exploiting behavior heterostructures. We discuss examples that successfully shown room-temperature control parameters such as peak, current ratio at negative differential resistance. conclude by summarizing challenges highlighting for future development FTJs, a special emphasis on possible type FeRTD device. The prospects enhanced performance expanded functionality ignite tremendous excitement FTJs FeRTDs nanoelectronics.

Language: Английский

Citations

0

P3OT-Based Organic Polymer Memristors for Artificial Synaptic Behavior and Neuromorphic Computing Applications DOI
Hongguang Zhang,

Linkai Li,

Aiqian Guo

et al.

ACS Applied Electronic Materials, Journal Year: 2025, Volume and Issue: unknown

Published: Feb. 26, 2025

Language: Английский

Citations

0

Uncontrolled Learning: Codesign of Neuromorphic Hardware Topology for Neuromorphic Algorithms DOI Creative Commons
Frank Barrows,

Jonathan Lin,

Francesco Caravelli

et al.

Advanced Intelligent Systems, Journal Year: 2025, Volume and Issue: unknown

Published: March 14, 2025

Neuromorphic computing has the potential to revolutionize future technologies and our understanding of intelligence, yet it remains challenging realize in practice. The learning‐from‐mistakes algorithm, inspired by brain's simple learning rules inhibition pruning, is one few brain‐like training methods. This algorithm implemented neuromorphic memristive hardware through a codesign process that evaluates essential trade‐offs. While effectively trains small networks as binary classifiers perceptrons, performance declines significantly with increasing network size unless tailored algorithm. work investigates trade‐offs between depth, controllability, capacity—the number learnable patterns—in hardware. highlights importance topology governing equations, providing theoretical tools evaluate device's computational capacity based on its measurements circuit structure. findings show breaking neural symmetry enhances both controllability capacity. Additionally, pruning circuit, algorithms all‐memristive circuits can utilize stochastic resources create local contrasts weights. Through combined experimental simulation efforts, parameters are identified enable exhibit emergent intelligence from rules, advancing computing.

Language: Английский

Citations

0

Artificial oxyanion reservoir accelerates oriented ionic migration in MXene-based synaptic memristor for neuromorphic computing DOI

Zhongrong Zheng,

Xu Yang,

Lin Lv

et al.

Surfaces and Interfaces, Journal Year: 2025, Volume and Issue: unknown, P. 106315 - 106315

Published: March 1, 2025

Language: Английский

Citations

0

Impact of terahertz short pulses on the oxygen defect state in TiO2x DOI Creative Commons
Paola Di Pietro, Johannes Schmidt, Nidhi Adhlakha

et al.

Physical Review Research, Journal Year: 2025, Volume and Issue: 7(2)

Published: April 3, 2025

Oxygen-deficient titanium dioxide (TiO2x) is a very attractive material for several applications ranging from photocatalysis to resistive switching. Oxygen vacancies turn insulating anatase into polaronic conductor, while creating defect-state band below the ultraviolet semiconducting gap. Here we employ combination of broadband infrared (IR) reflectivity and THz-pump/IR-probe measurements investigate relationship between localized defect states delocalized conducting states. We show that THz pump allows convert deeply electrons metastable polarons with lifetime in ns range. These long-lived may find application novel optoelectronic exploiting interplay dc resistivity, terahertz signals. Published by American Physical Society 2025

Language: Английский

Citations

0