Perspective on Crystal Structures, Synthetic Methods, and New Directions in Thermoelectric Materials DOI Creative Commons
Marta María González-Barrios, Marina Tabuyo‐Martínez, David Ávila‐Brande

et al.

Small Structures, Journal Year: 2024, Volume and Issue: unknown

Published: June 10, 2024

This review explores the state‐of‐the‐art of thermoelectric materials, covering different crystalline structures and material families (e.g., chalcogenides, Zintl phases, skutterudites, clathrates, oxides, half‐Heusler, organic–inorganic composites, metal–organic frameworks, silicides). It examines their corresponding properties while considering synthesis methods employed, paying significant attention to those that particularly follow sustainable routes. Additionally, work addresses current challenges in field, such as enhancing stability at high temperatures reducing manufacturing costs. The understanding gained this field opens avenues for designing more efficient devices convert waste heat into electrical energy, thereby advancing cleaner technologies.

Language: Английский

Lattice dynamics and thermoelectric properties of diamondoid materials DOI Creative Commons
Hongyao Xie, Li‐Dong Zhao, Mercouri G. Kanatzidis

et al.

Interdisciplinary materials, Journal Year: 2024, Volume and Issue: 3(1), P. 5 - 28

Published: Jan. 1, 2024

Abstract The diamondoid compounds are a large family of important semiconductors, which possess various unique transport properties and had been widely investigated in the fields photoelectricity nonlinear optics. For significantly long period time, materials were not given much attention field thermoelectricity. However, this changed when series showed thermoelectric figure merit ( ZT ) greater than 1.0. This discovery sparked considerable interest further exploring materials. review aims to provide comprehensive view our current understanding thermal electronic stimulate their development applications. We present collection recent discoveries concerning lattice dynamics structure underlying physics responsible for electrical phonon behaviors. Moreover, we insights into advancements made thermoelectricity corresponding strategies employed optimize performance. Lastly, emphasize challenges that lie ahead outline potential avenues future research domain

Language: Английский

Citations

38

Advancing flexible thermoelectrics for integrated electronics DOI
Xiao‐Lei Shi, Lijun Wang, Wanyu Lyu

et al.

Chemical Society Reviews, Journal Year: 2024, Volume and Issue: 53(18), P. 9254 - 9305

Published: Jan. 1, 2024

With the increasing demand for energy and climate challenges caused by consumption of traditional fuels, there is an urgent need to accelerate adoption green sustainable conversion storage technologies. The integration flexible thermoelectrics with other various technologies plays a crucial role, enabling multiple forms such as temperature differentials, solar energy, mechanical force, humidity into electricity. development these lays foundation power solutions promotes research progress in conversion. Given complexity rapid this field, review provides detailed overview multifunctional integrated based on thermoelectric focus improving material performance, optimizing design device structures, achieving flexibility expand their application scenarios, particularly multi-functionalization wearable Additionally, we discuss current bottlenecks future directions facilitate continuous advancement field.

Language: Английский

Citations

29

Photovoltaics for indoor energy harvesting DOI Creative Commons
Abhisek Chakraborty, Giulia Lucarelli, Jie Xu

et al.

Nano Energy, Journal Year: 2024, Volume and Issue: 128, P. 109932 - 109932

Published: June 29, 2024

The Internet of Things revolution requires a low-cost, stable, and highly efficient power source to allow autonomous operation smart objects wireless sensors even at very low light levels. Indoor photovoltaics (PV) has the potential fulfil these requirements, providing independence from main grid, portability, improved sustainability for low-consumption devices. Whereas polycrystalline silicon dominates outdoor solar cell market, amorphous is commercially more suited products used inside buildings, delivering higher efficiencies under indoor illumination (with its extremely lower intensities narrower spectra compared sunlight). In recent years, there been remarkable rise in research development new generation photovoltaic cells, i.e., those based on organic, dye-sensitized perovskite absorbers, focused applications with rising well above possible sun reaching surpassing 30 % conversion efficiency threshold. This review provides systematic overview PV devices, highlighting progress achieved strategies design cells as issues be resolved this field continue prosper. We also analyse differences device meant outdoors vs indoors. Markets tapped by harvesting are huge, ranging building-integrated elements consumer products, biomedical communication technologies.

Language: Английский

Citations

28

Roadmap on printable electronic materials for next-generation sensors DOI Creative Commons
Vincenzo Pecunia, Luisa Petti, Joseph Andrews

et al.

Nano Futures, Journal Year: 2024, Volume and Issue: 8(3), P. 032001 - 032001

Published: March 22, 2024

Abstract The dissemination of sensors is key to realizing a sustainable, ‘intelligent’ world, where everyday objects and environments are equipped with sensing capabilities advance the sustainability quality our lives—e.g. via smart homes, cities, healthcare, logistics, Industry 4.0, precision agriculture. realization full potential these applications critically depends on availability easy-to-make, low-cost sensor technologies. Sensors based printable electronic materials offer ideal platform: they can be fabricated through simple methods (e.g. printing coating) compatible high-throughput roll-to-roll processing. Moreover, often allow fabrication flexible/stretchable/biodegradable substrates, thereby enabling deployment in unconventional settings. Fulfilling promise for will require device innovations enhance their ability transduce external stimuli—light, ionizing radiation, pressure, strain, force, temperature, gas, vapours, humidity, other chemical biological analytes. This Roadmap brings together viewpoints experts various materials—and devices thereof—to provide insights into status outlook field. Alongside recent innovations, roadmap discusses outstanding challenges pertaining each technology. Finally, points promising directions overcome thus enable ubiquitous world.

Language: Английский

Citations

17

Harvesting Ocean Wave Energy via Magnetoelastic Generators for Self-Powered Hydrogen Production DOI

Il Woo Ock,

Yihao Zhou, Xun Zhao

et al.

ACS Energy Letters, Journal Year: 2024, Volume and Issue: 9(4), P. 1701 - 1709

Published: March 25, 2024

Extracting energy from ocean waves for electrolysis, while highly desirable, poses significant challenges, especially in achieving high current generation sustainable water splitting. This work introduces an innovative high-current wave harvesting system, employing a self-floating magnetoelastic generator (MEG) ball network designed autonomous seawater electrolysis and on-site hydrogen (H2) production. Leveraging the effect, MEG is naturally waterproof can generate density of 0.24 mA cm–2, paired with low internal resistance 9 Ω at frequency 2 Hz. Its spherical design ensures exceptional mechanical durability, maintaining consistent electrical output even under extremely humid harsh conditions. In practical applications, this system continuously produce H2 rate 0.76 × 10–3 mL min–1. These results underscore its potential as viable technology large-scale

Language: Английский

Citations

16

Efficient Integration of Ultra-low Power Techniques and Energy Harvesting in Self-Sufficient Devices: A Comprehensive Overview of Current Progress and Future Directions DOI Creative Commons
Rocco Citroni, Fabio Mangini, Fabrizio Frezza

et al.

Sensors, Journal Year: 2024, Volume and Issue: 24(14), P. 4471 - 4471

Published: July 10, 2024

Compact, energy-efficient, and autonomous wireless sensor nodes offer incredible versatility for various applications across different environments. Although these devices transmit receive real-time data, efficient energy storage (ES) is crucial their operation, especially in remote or hard-to-reach locations. Rechargeable batteries are commonly used, although they often have limited capacity. To address this, ultra-low-power design techniques (ULPDT) can be implemented to reduce consumption prolong battery life. The Energy Harvesting Technique (EHT) enables perpetual operation an eco-friendly manner, but may not fully replace due its intermittent nature power generation. ensure uninterrupted supply, such as ES management unit (PMU) needed. This review focuses on the importance of minimizing maximizing efficiency improve autonomy longevity nodes. It examines current advancements, challenges, future direction ULPDT, ES, PMU, communication protocols, EHT develop implement robust technology solutions practical long-lasting use real-world scenarios.

Language: Английский

Citations

16

Thermoelectric Performance Predictions Combining Experiments with Multi‐Band Modelling DOI Open Access
Bharti Agrawal, Titas Dasgupta

Advanced Theory and Simulations, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 17, 2025

Abstract The search for high‐performance thermoelectric (TE) materials requires accurate property predictions and the development of analytical models to mimic temperature dependent charge heat transport in semiconductors. This is a non‐trivial task as most have complex electronic band structures with multiple bands contributing transport. In this work, it shown that using combination experiments recently developed multi‐band modelling technique, possible accurately predict doping properties TE materials. steps involved are experimental data collection, model parameter generation, interpolation. methodology elaborated example Mg 2 Si 0.3 Sn 0.7 which high‐performance, low‐cost material. 3‐D maps power factor figure merit () generated function concentration. Model validation carried out randomly prepared composition yields maximum deviations ±10% plots. results highlight potential tool rapid screening compositions.

Language: Английский

Citations

2

Weavable thermoelectrics: advances, controversies, and future developments DOI Creative Commons
Xiao‐Lei Shi,

Shuai Sun,

Ting Wu

et al.

Materials Futures, Journal Year: 2023, Volume and Issue: 3(1), P. 012103 - 012103

Published: Nov. 14, 2023

Abstract Owing to the capability of conversion between thermal energy and electrical their advantages light weight, compactness, noise-free operation, precision reliability, wearable thermoelectrics show great potential for diverse applications. Among them, weavable thermoelectrics, a subclass with inherent flexibility, wearability, operability, find utility in harnessing waste heat from irregular sources. Given rapid advancements this field, timely review is essential consolidate progress challenge. Here, we provide an overview state thermoelectric materials devices smart textiles, encompassing mechanisms, materials, fabrications, device structures, applications recent advancements, challenges, prospects. This can serve as valuable reference researchers field flexible

Language: Английский

Citations

31

Highly Efficient Flexible Perovskite Solar Cells on Polyethylene Terephthalate Films via Dual Halide and Low‐Dimensional Interface Engineering for Indoor Photovoltaics DOI
Zeynab Skafi, Jie Xu, Vahid Mottaghitalab

et al.

Solar RRL, Journal Year: 2023, Volume and Issue: 7(20)

Published: Aug. 1, 2023

Flexible perovskite solar cells are lightweight, bendable, and applicable to curved surfaces. Polyethylene terephthalate (PET) has become the substrate of choice compared other plastic substrates like polyethylene naphthalate. PET is not only stable but also much cheaper manufacture, an important factor for photovoltaics (PV). Herein, highly efficient devices on demonstrated using a dual low‐temperature (≤100 °C) approach, first by anion mixing (replacing I with Br) lead‐containing composition, increasing bandgap (42% improvement), then interfacial engineering tetrabutylammonium bromide (TBAB) (a further 26% reaching efficiencies 28.9% at 200 lx record 32.5% 1000 lx. The TBA + cation intercalates into structure, substituting formamidinium cations perovskite/TBAB interface, inducing formation large‐sized, lower dimensional structures over 3D matrix. resulting PV cell 1.4 times higher carrier lifetime, one order magnitude leakage currents, 3 defect densities, suppressing recombination. Importantly, stability (ISOS‐D1 protocol) improves more than double treatment. Highly films enable seamless integration wearable, portable, smart building, Internet Things electronic devices, expanding reach indoor applications.

Language: Английский

Citations

26

Advances in MXene-based triboelectric nanogenerators DOI
Sadegh Ghorbanzadeh, Wei Zhang

Nano Energy, Journal Year: 2024, Volume and Issue: 125, P. 109558 - 109558

Published: March 30, 2024

Language: Английский

Citations

15