ac Stark Spectroscopy of Interactions between Moiré Excitons and Polarons
Physical Review X,
Journal Year:
2025,
Volume and Issue:
15(2)
Published: April 1, 2025
We
use
nonlinear
pump-probe
spectroscopy
to
study
optical
excitations
in
a
charge-tunable
MoSe2/WS2
moiré
heterostructure.
An
intense
red-detuned
laser
pulse
creates
photonic
dressing
of
the
material
by
introducing
large
population
excitons
or
exciton
polarons
deep
potential.
By
measuring
resulting
ac
Stark
effect
with
weak
resonant
pulse,
we
gain
access
nature
and
mutual
interactions
elementary
excitations.
At
charge
neutrality,
our
measurements
reveal
that
different
resonances,
associated
confinement
their
center-of-mass
motion
potential,
have
significant
spatial
overlap.
The
short-range
manifest
themselves
as
density-dependent
blueshift
for
same-valley
bound
biexciton
states
opposite-valley
excitons.
attractive
polaron
resonance
appears
upon
injection
electrons
into
heterostructure
shows
contrasting
behavior:
Here,
observe
an
electron-density-independent
light
shift
clear
pump-power-dependent
saturation.
These
features
are
equivalent
ensemble
independent
two-level
emitters
indicate
breakdown
Fermi-polaron
picture
subject
strong
Our
work
establishes
experimental
approach
elucidate
semiconductor
heterostructures,
providing
solid
ground
correlated
electronic
excitonic
such
materials.
Published
American
Physical
Society
2025
Language: Английский
Moiré Potential Independent of Moiré Size Down to a Few Nanometers in Sliding Ferroelectrics
Nano Letters,
Journal Year:
2025,
Volume and Issue:
unknown
Published: April 14, 2025
Sliding
ferroelectricity
represents
a
way
to
realize
atomically
thin
ferroelectric
materials.
Due
the
moiré
pattern
formed
during
stacking
process,
alternating
domain
network
provides
an
attractive
superlattice
of
electrostatic
potential
modulate
electronic
structures
another
material
sitting
on
it.
The
relationship
between
magnitude
and
size,
however,
has
been
controversial
in
literature.
In
addition,
how
strong
remains
for
sizes
down
10
nm
range
is
unclear.
this
study,
we
use
contact-mode
scanning
tunneling
microscopy
with
high
spatial
energy
resolution
show
that
independent
size
ranging
from
hundreds
several
nanometers.
We
also
determined
solely
by
specific
materials
used
fabricate
stack.
This
study
important
information
sliding
ferroelectrics
can
foster
their
application
modulating
other
Language: Английский