The Role of Reticular Chemistry in Photoenzymatic Reaction DOI
Ying Shu, Jimin Lee, Weibin Liang

et al.

Green Chemistry, Journal Year: 2024, Volume and Issue: 26(23), P. 11468 - 11489

Published: Jan. 1, 2024

Photoenzymatic catalysis faces challenges like low stability and recyclability. Reticular framework materials offer solutions by enabling enzyme protection reuse. This review highlights recent advances, design strategies, future directions.

Language: Английский

Solar-Driven Degradation of Malachite Green by Photoenzyme: Mechanisms and Sustainable Water Treatment DOI
Yang Zheng, Gan Luo, Guosheng Chen

et al.

Journal of Cleaner Production, Journal Year: 2025, Volume and Issue: unknown, P. 145335 - 145335

Published: March 1, 2025

Language: Английский

Citations

1
Efficient Photocatalytic Water Purification Through Novel Janus‐Nanomicelles with Long‐Lived Charge Separation Properties DOI Open Access
Jin Gao,

Liujun Yang,

Guan Wang

et al.

Small, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 17, 2025

Although the design of photocatalysts incorporating donor-acceptor units has garnered significant attention for its potential to enhance efficiency photocatalysis process, primary bottleneck lies in challenge generating long-lived charge separation states during exciton separation. Therefore, a novel Janus-nanomicelles photocatalyst is developed using carbazole (Cz) as donor unit, perylene-3,4,9,10-tetracarboxydiimide (PDI) with long-excited state acceptor unit and polyethylene glycol (PEG) hydrophilic segment through ROMP polymerization. After optimizing ratio, Cz19-PDI18-PEG10 rapidly adsorbs bisphenol A (BPA) within 10 s π-π interaction, hydrogen-bonding hydrophobic interaction between BPA blocks when exposed aqueous humor efficiently photodegrades (50 ppm) 120 min water purification purposes due achieving highest reported so far. Mechanistic studies have shown that this excellent performance can be attributed synergistic interactions highly efficient adsorption capacity photocatalysis. This strategy holds promise an effective candidate purification.

Language: Английский

Citations

0
Design, Synthesis, and Application of Immobilized Enzymes on Artificial Porous Materials DOI Creative Commons
Ran Lu, Yuan Lu, Chen Li

et al.

Advanced Science, Journal Year: 2025, Volume and Issue: unknown

Published: April 30, 2025

Enzymes have been recognized as highly efficient biocatalysts, whereas characteristics such poor stability and single reaction type greatly significantly limit their wide application. Hence, the exploitation of suitable carriers for immobilized enzymes enables provision a protective layer enzyme, with capability chemical biological cascade catalysis. Among various immobilization carriers, metal-organic frameworks (MOFs), covalent organic (COFs) hydrogen-bonded (HOFs) emerging promising strategy to surpass inherent instability other limitations free enzymes. Specifically, integration artificial porous materials improves reusability enzymes, while simultaneously affording platform multifunctional applications. Herein, this review systematically discusses preparation strategies advantages materials, elucidating effects different methods on enzyme activity. Furthermore, innovative applications in field fields photocatalysts, catalysts sensing are also comprehensively summarized here, thus demonstrating addressing complex biotransformation challenges.

Language: Английский

Citations

0
Sp-Hybridized Carbon- Facilitated Peroxymonosulfate Activation for Superior Phenolic Pollutant Removal DOI
Pan Yang,

Jinlan Tang,

Zhenhua Ding

et al.

Journal of Hazardous Materials, Journal Year: 2025, Volume and Issue: 490, P. 137843 - 137843

Published: March 4, 2025

Language: Английский

Citations

0
Recent progress of hydrogen-bonded organic framework-based photocatalysis DOI

Heng Yuan,

Jian Xiao, An‐An Zhang

et al.

EnergyChem, Journal Year: 2025, Volume and Issue: unknown, P. 100151 - 100151

Published: March 1, 2025

Language: Английский

Citations

0
Achieving efficient photo-enzyme coupling via a novel diketone derivative to expand the scope of enzyme action DOI Creative Commons
Wentao Zhang,

Shuyu Zhou,

Hao Dong

et al.

Chemical Engineering Journal Advances, Journal Year: 2025, Volume and Issue: unknown, P. 100732 - 100732

Published: March 1, 2025

Language: Английский

Citations

0
Site-specific surface amination strategy facilitates biomimetic encapsulation of enzymes within hydrogen-bonded organic framework DOI

Haoquan Huang,

Haiting Chen, Xinran Dong

et al.

Chinese Chemical Letters, Journal Year: 2025, Volume and Issue: unknown, P. 111223 - 111223

Published: April 1, 2025

Language: Английский

Citations

0
The Role of Reticular Chemistry in Photoenzymatic Reaction DOI
Ying Shu, Jimin Lee, Weibin Liang

et al.

Green Chemistry, Journal Year: 2024, Volume and Issue: 26(23), P. 11468 - 11489

Published: Jan. 1, 2024

Photoenzymatic catalysis faces challenges like low stability and recyclability. Reticular framework materials offer solutions by enabling enzyme protection reuse. This review highlights recent advances, design strategies, future directions.

Language: Английский

Citations

2