Ocean alkalinity enhancement – avoiding runaway CaCO3 precipitation during quick and hydrated lime dissolution DOI Creative Commons
Charly A. Moras, Lennart T. Bach, Tyler Cyronak

et al.

Biogeosciences, Journal Year: 2022, Volume and Issue: 19(15), P. 3537 - 3557

Published: Aug. 1, 2022

Abstract. Ocean alkalinity enhancement (OAE) is a method that can remove carbon dioxide (CO2) from the atmosphere and counteract ocean acidification through dissolution of alkaline minerals. Currently, critical knowledge gaps exist regarding different minerals suitable for OAE in natural seawater. Of particular importance to understand how much mineral be dissolved before secondary precipitation calcium carbonate (CaCO3) occurs, since CaCO3 reduces atmospheric CO2 uptake potential OAE. Using two types proposed OAE, quick lime (CaO) hydrated (Ca(OH)2), we show both (<63 µm diameter) seawater within few hours. No occurred at saturation state (ΩA) ∼5, but form aragonite above an ΩA value 7. This limit lower than expected typical pseudo-homogeneous precipitation, i.e. presence colloids organic matter. Secondary low (∼ 7) was result heterogeneous onto surfaces, most likely added CaO Ca(OH)2 particles. Most importantly, runaway observed, condition where significantly more total (TA) removed initially added. Such could reduce efficiency ∼ 0.8 mol per mole TA down 0.1 TA. Runaway appears avoidable by dilution below threshold 5, ideally hours additions minimise initial precipitation. Finally, simulations suggest same threshold, amount would 3 times higher 5 ∘C 30 ∘C. The maximum addition also increased equilibrating levels (i.e. pCO2 416 µatm) during addition. allow without inducing using its removal potential.

Language: Английский

Endemism increases species' climate change risk in areas of global biodiversity importance DOI
Stella Manes, Mark J. Costello, Heath Beckett

et al.

Biological Conservation, Journal Year: 2021, Volume and Issue: 257, P. 109070 - 109070

Published: April 9, 2021

Language: Английский

Citations

240

Overcoming the coupled climate and biodiversity crises and their societal impacts DOI
Hans‐Otto Pörtner, Robert J. Scholes, Almut Arneth

et al.

Science, Journal Year: 2023, Volume and Issue: 380(6642)

Published: April 20, 2023

Earth's biodiversity and human societies face pollution, overconsumption of natural resources, urbanization, demographic shifts, social economic inequalities, habitat loss, many which are exacerbated by climate change. Here, we review links among climate, biodiversity, society develop a roadmap toward sustainability. These include limiting warming to 1.5°C effectively conserving restoring functional ecosystems on 30 50% land, freshwater, ocean "scapes." We envision mosaic interconnected protected shared spaces, including intensively used strengthen self-sustaining the capacity people nature adapt mitigate change, nature's contributions people. Fostering interlinked human, ecosystem, planetary health for livable future urgently requires bold implementation transformative policy interventions through institutions, governance, systems from local global levels.

Language: Английский

Citations

234

Climate Change and Small Island Developing States DOI Open Access
Adelle Thomas, April Karen Baptiste, Rosanne Martyr-Koller

et al.

Annual Review of Environment and Resources, Journal Year: 2020, Volume and Issue: 45(1), P. 1 - 27

Published: May 14, 2020

Despite their heterogeneity, small island developing states (SIDS) are recognized as being particularly at risk to climate change, and, they share numerous common traits, the United Nations recognizes them a special group. SIDS have been quite vocal in calling attention challenges face from change and advocating for greater international ambition limit global warming. Here, we unpack factors that helpful understanding relationship between through review of studies span disciplines methodologies. We assess patterns hazards, exposure, vulnerability; impacts risks; awareness knowledge; adaptation planning implementation; mitigation; loss damage; justice provide an overarching literature on SIDS.

Language: Английский

Citations

197

Atomic Tuning of Single-Atom Fe–N–C Catalysts with Phosphorus for Robust Electrochemical CO2 Reduction DOI
Ke Li, Shengbo Zhang, Xiuli Zhang

et al.

Nano Letters, Journal Year: 2022, Volume and Issue: 22(4), P. 1557 - 1565

Published: Feb. 1, 2022

The electrochemical reduction of CO2 to produce carbon-based fuels and chemicals possesses huge potentials alleviate current environmental problems. However, it is confronted by great challenges in the design active electrocatalysts with low overpotentials high product selectivity. Here we report atomic tuning a single-Fe-atom catalyst phosphorus (Fe-N/P-C) on commercial carbon black as robust electrocatalyst for reduction. Fe-N/P-C exhibits impressive performance CO, Faradaic efficiency 98% mass-normalized turnover frequency 508.8 h-1 at overpotential 0.34 V. On basis ex-situ X-ray absorption spectroscopy measurements DFT calculations, reveal that P catalysts reduces oxidation state Fe center decreases free-energy barrier *CO intermediate formation, consequently maintaining electrocatalytic activity stability catalysts.

Language: Английский

Citations

182

Solar utilization beyond photosynthesis DOI
Jiangquan Lv, Jiafang Xie, Aya Gomaa Abdelkader Mohamed

et al.

Nature Reviews Chemistry, Journal Year: 2022, Volume and Issue: 7(2), P. 91 - 105

Published: Dec. 19, 2022

Language: Английский

Citations

163

Equity, technological innovation and sustainable behaviour in a low-carbon future DOI
Benjamin K. Sovacool, Peter Newell, Sanya Carley

et al.

Nature Human Behaviour, Journal Year: 2022, Volume and Issue: 6(3), P. 326 - 337

Published: Jan. 31, 2022

Language: Английский

Citations

161

The importance of food systems and the environment for nutrition DOI Creative Commons
Jessica Fanzo, Alexandra L. Bellows, Marie L. Spiker

et al.

American Journal of Clinical Nutrition, Journal Year: 2020, Volume and Issue: 113(1), P. 7 - 16

Published: Oct. 7, 2020

Global and local food system transformation is necessary in order to ensure the delivery of healthy, safe, nutritious foods both sustainable equitable ways. Food systems are complex entities that affect diets, human health, a range other outcomes including economic growth, natural resource environmental resiliency, sociocultural factors. However, contribute vulnerable ongoing climate changes threaten their sustainability. Although there has been increased focus on this topic recent years, many gaps our knowledge persist relation between factors, systems, nutritional outcomes. In article, we summarize emerging field describe what innovative nutrition research needed bring about policy era disruption degradation.

Language: Английский

Citations

150

Changing Lengths of the Four Seasons by Global Warming DOI
Jiamin Wang, Yuping Guan, Lixin Wu

et al.

Geophysical Research Letters, Journal Year: 2021, Volume and Issue: 48(6)

Published: Feb. 19, 2021

Abstract How long will the four seasons be by 2100? Increasing evidence suggests that length of a single season or in regional scales has changed under global warming, but hemispherical‐scale response past and future remains unknown. We find summer Northern Hemisphere midlatitudes lengthened, whereas winter shortened, owing to shifts their onsets withdrawals, accompanied shorter spring autumn. Such changes lengths can mainly attributed greenhouse‐warming. Even if current warming rate does not accelerate, still exacerbated future. Under business‐as‐usual scenario, is projected last nearly half year, less than 2 months 2100. The changing seasonal clock signifies disturbed agriculture rhythm species activities, more frequent heat waves, storms wildfires, amounting increased risks humanity.

Language: Английский

Citations

147

Compound droughts and hot extremes: Characteristics, drivers, changes, and impacts DOI Creative Commons
Zengchao Hao, Fanghua Hao,

Youlong Xia

et al.

Earth-Science Reviews, Journal Year: 2022, Volume and Issue: 235, P. 104241 - 104241

Published: Nov. 8, 2022

Language: Английский

Citations

135

A review on cathode processes and materials for electro-reduction of carbon dioxide in solid oxide electrolysis cells DOI

Yunan Jiang,

Fanglin Chen, Changrong Xia

et al.

Journal of Power Sources, Journal Year: 2021, Volume and Issue: 493, P. 229713 - 229713

Published: March 6, 2021

Language: Английский

Citations

130