Physical Review Research,
Journal Year:
2023,
Volume and Issue:
5(4)
Published: Dec. 20, 2023
We
show
that
the
coherent
interaction
between
free
electrons
and
photons
can
be
used
for
universal
control
of
continuous-variable
photonic
quantum
states
in
form
Gottesman-Kitaev-Preskill
(GKP)
qubits.
Specifically,
we
find
electron
energy
combs
enable
nondestructive
measurements
state
induce
arbitrary
gates.
Moreover,
a
single
interacting
with
multiple
modes
create
highly
entangled
such
as
Greenberger-Horne-Zeilinger
cluster
GKPs.
Applied Physics Reviews,
Journal Year:
2023,
Volume and Issue:
10(1)
Published: Jan. 18, 2023
When
impinging
on
optical
structures
or
passing
in
their
vicinity,
free
electrons
can
spontaneously
emit
electromagnetic
radiation,
a
phenomenon
generally
known
as
cathodoluminescence.
Free-electron
radiation
comes
many
guises:
Cherenkov,
transition,
and
Smith–Purcell
but
also
electron
scintillation,
commonly
referred
to
incoherent
While
those
effects
have
been
at
the
heart
of
fundamental
discoveries
technological
developments
high-energy
physics
past
century,
recent
demonstration
photonic
nanophotonic
systems
has
attracted
great
deal
attention.
Those
arose
from
predictions
that
exploit
nanophotonics
for
novel
regimes,
now
becoming
accessible
thanks
advances
nanofabrication.
In
general,
proper
design
enable
shaping,
control,
enhancement
free-electron
any
above-mentioned
effects.
opens
way
promising
applications,
such
widely
tunable
integrated
light
sources
x-ray
THz
frequencies,
miniaturized
particle
accelerators,
highly
sensitive
detectors.
Here,
we
review
emerging
field
nanophotonics.
We
first
present
unified
framework
describe
light–matter
interaction
arbitrary
systems.
then
show
how
this
sheds
physical
underpinnings
methods
used
control
enhance
radiation.
Namely,
points
central
role
played
by
eigenmodes
controlling
output
properties
(e.g.,
frequency,
directionality,
polarization).
experimental
techniques
characterize
scanning
transmission
microscopes,
which
emerged
platforms
realization
phenomena
described
review.
further
discuss
various
extract
spectral,
angular,
polarization-resolved
information
conclude
outlining
directions
field,
including
ultrafast
quantum
short-wavelength
emitters
ultraviolet
soft
topological
states
crystals.
Applied Physics Reviews,
Journal Year:
2023,
Volume and Issue:
10(2)
Published: June 1, 2023
In
the
past
20
years,
we
have
reached
a
broad
understanding
of
many
light-driven
phenomena
in
nanoscale
systems.
The
temporal
dynamics
excited
states
are
instead
quite
challenging
to
explore,
and,
at
same
time,
crucial
study
for
origin
fundamental
physical
and
chemical
processes.
this
review,
examine
current
state
prospects
ultrafast
driven
by
plasmons
both
from
applied
point
view.
This
research
area
is
referred
as
plasmonics
represents
an
outstanding
playground
tailor
control
fast
optical
electronic
processes
nanoscale,
such
switching,
single
photon
emission,
strong
coupling
interactions
photochemical
reactions.
Here,
provide
overview
field
describe
methodologies
monitor
with
timescales
terms
modeling
experimental
characterization.
Various
directions
showcased,
among
others
recent
advances
plasmon-driven
chemistry
multi-functional
plasmonics,
which
charge,
spin,
lattice
degrees
freedom
exploited
active
properties
materials.
As
focus
shifts
development
practical
devices,
all-optical
transistors,
also
emphasize
new
materials
applications
highlight
relativistic
realm.
latter
promising
potential
fusion
or
particle
light
sources
providing
attosecond
duration.
Proceedings of the National Academy of Sciences,
Journal Year:
2025,
Volume and Issue:
122(6)
Published: Feb. 5, 2025
Free-electron
radiation,
such
as
Cherenkov
radiation
and
transition
can
generate
light
at
arbitrary
frequencies
is
fundamental
to
diverse
applications,
ranging
from
electron
microscopy,
spectroscopy,
lasers,
particle
detectors.
Generally,
the
features
of
free-electron
are
stochastic
when
electrons
interact
with
random
media.
Counterintuitively,
here,
we
reveal
a
type
that
has
both
its
intensity
directionality
invariant
specific
sorts
long-range
structural
randomness.
Essentially,
this
invariance
enabled
by
Brewster
effect
judiciously
engineered
phase
coherence
condition
emitted
light,
namely
induced
electron’s
penetration
through
layered
aperiodic
nanostructure
interfere
constructively
angle.
As
such,
each
constituent
layer
thickness
fulfills
condition,
there
always
emergence
resonance
At
resonant
angle,
further
find
could
be
enhanced
orders
magnitude
readily
increasing
interface
number.
The
revealed
via
randomness
may
offer
feasible
route
explore
more
enticing
photonic
applications
driven
free
electrons,
sources
previously
unreachable
spectral
regimes,
optical
frequency
combs,
detectors,
lasers.
Physical review. A/Physical review, A,
Journal Year:
2025,
Volume and Issue:
111(1)
Published: Jan. 9, 2025
We
propose
a
tangible
experimental
scheme
for
demonstrating
quantum
entanglement
between
swift
electrons
and
light,
relying
on
coherent
cathodoluminescence
photon
generation
in
transmission
electron
microscope,
eraser
setup
formation
verification
of
entanglement.
The
free
with
light
is
key
to
developing
free-electron
optics
its
potential
applications
such
as
sensing,
novel
photonic
state
generation,
electrons.
Published
by
the
American
Physical
Society
2025
Science Advances,
Journal Year:
2022,
Volume and Issue:
8(40)
Published: Oct. 7, 2022
Following
the
lifespan
of
optical
excitations
from
their
creation
to
decay
into
photons
is
crucial
in
understanding
materials
properties.
Macroscopically,
techniques
such
as
photoluminescence
excitation
spectroscopy
provide
unique
information
on
photophysics
with
applications
diverse
quantum
optics
or
photovoltaics.
Materials
and
emission
pathways
are
affected
by
nanometer
scale
variations
directly
impacting
devices
performances.
However,
they
cannot
be
accessed,
despite
techniques,
spectroscopies
free
electrons,
having
relevant
spatial,
spectral
time
resolution.
Here,
we
explore
two
representative
devices:
plasmonic
nanoparticles
luminescent
2D
layers.
The
analysis
energy
lost
an
exciting
electron
that
coincident
a
visible-UV
photon
unveils
towards
light
emission.
This
demonstrated
for
phase-locked
interactions,
localized
surface
plasmons,
non-phase-locked
ones,
individual
point
defects.
newly
developed
cathodoluminescence
images
transfer
at
scale.
It
widens
toolset
available
nanoscale
materials.
Physical Review X,
Journal Year:
2023,
Volume and Issue:
13(1)
Published: Jan. 6, 2023
For
over
80
years
of
research,
the
conventional
description
free-electron
radiation
phenomena,
such
as
Cherenkov
radiation,
has
remained
unchanged:
classical
three-dimensional
electromagnetic
waves.
Interestingly,
in
reduced
dimensionality,
properties
are
predicted
to
fundamentally
change.
Here,
we
present
first
observation
surface
waves,
wherein
free
electrons
emit
narrow-bandwidth
photonic
quasiparticles
propagating
two-dimensions.
The
low
dimensionality
and
narrow
bandwidth
effect
enable
identify
quantized
emission
events
through
electron
energy
loss
spectroscopy.
Our
results
support
recent
theoretical
prediction
that
do
not
always
light
can
instead
become
entangled
with
photons
they
emit.
two-dimensional
interaction
achieves
quantum
coupling
strengths
two
orders
magnitude
larger
than
ever
reported,
reaching
single-electron-single-photon
regime
for
time
electrons.
findings
pave
way
previously
unexplored
phenomena
optics,
facilitating
bright,
free-electron-based
emitters
heralded
Fock
states.
Nature Physics,
Journal Year:
2023,
Volume and Issue:
19(10), P. 1410 - 1417
Published: June 22, 2023
Abstract
While
correlated
electrons
are
at
the
heart
of
many
phenomena
in
condensed
matter,
as
well
atomic
and
molecular
physics,
Coulomb
interactions
free-electron
beams
generally
considered
detrimental.
Here,
we
demonstrate
generation
Coulomb-correlated
pair,
triple
quadruple
states
free
by
femtosecond
photoemission
from
a
nanoscale
field
emitter
inside
transmission
electron
microscope.
Event-based
spectroscopy
allows
spatial
spectral
characterization
ensemble
emitted
each
laser
pulse.
We
identify
distinctive
energy
momentum
correlations
arising
acceleration-enhanced
interparticle
exchange,
revealing
strong
few-body
an
scale
2
eV.
State-sorted
beam
caustics
show
discrete
increase
virtual
source
size
longitudinal
shift
for
few-electron
states,
associated
with
transverse
correlations.
observe
field-controllable
antibunching,
attributed
primarily
to
deflection.
The
pronounced
characteristics
these
number
allow
filtering
schemes
that
control
statistical
distribution
pulse
charge.
In
this
way,
fraction
specific
can
be
actively
suppressed
or
enhanced,
facilitating
preparation
highly
non-Poissonian
microscopy
lithography,
including
future
heralding
multi-electron
probing.
Physical Review X,
Journal Year:
2023,
Volume and Issue:
13(3)
Published: July 6, 2023
A
new
approach
to
generating
quantum
states
of
light
most
suitable
for
robust
computing
draws
on
one
the
basic
interactions
in
physics---the
interaction
between
free
electrons
and
photons.