Abstract.
Our
global
understanding
of
clouds
and
aerosols
relies
on
the
remote
sensing
their
optical,
microphysical,
macrophysical
properties
using,
in
part,
scattered
solar
radiation.
Current
retrievals
assume
form
plane-parallel,
homogeneous
layers
utilize
1D
radiative
transfer
(RT)
models.
These
assumptions
limit
detail
that
can
be
retrieved
about
3D
variability
cloud
aerosol
fields
induce
biases
for
highly
heterogeneous
structures
such
as
cumulus
smoke
plumes.
In
Part
1
this
two-part
study,
we
validated
a
tomographic
method
utilizes
multi-angle
passive
imagery
to
retrieve
distributions
species
using
RT
overcome
these
issues.
That
validation
characterized
uncertainty
approximate
Jacobian
used
retrieval
over
wide
range
atmospheric
surface
conditions
several
horizontal
boundary
conditions.
Here
2,
test
algorithm’s
effectiveness
synthetic
data
whether
accuracy
is
limited
by
use
Jacobian.
We
volume
extinction
coefficient
(σ3D)
at
40
m
resolution
from
multi-angle,
mono-spectral
35
derived
stochastically-generated
‘cumuliform’
(1
km)3
domains.
The
are
idealized
neglect
forward
modelling
instrumental
errors
with
exception
radiometric
noise;
thus
reported
lower
bounds.
σ3D
with,
average,
Relative
Root
Mean
Square
Error
(RRMSE)
<
20
%
bias
0.1
Maximum
Optical
Depth
(MOD)
17,
RRMSE
radiances
0.5
%,
indicating
very
high
shallow
As
MOD
increases
80,
worsen
60
−35
respectively,
reaches
16
incomplete
convergence.
This
expected
increasing
ill-conditioning
inverse
problem
decreasing
mean-free-path
predicted
theory
discussed
1.
tested
model
better
conditioned
but
less
accurate
due
more
aggressive
delta-M
scaling.
reduces
radiance
9
σ3D
−8
~80,
no
improvement
σ3D.
illustrates
significant
sensitivity
numerical
configuration
which,
least
our
circumstances,
improves
accuracy.
All
ensemble-averaged
results
robust
inclusion
noise
during
retrieval.
However,
individual
realizations
have
large
deviations
up
18
mean
which
indicates
uncertainties
optically
thick
limit.
Using
tomography
also
accurately
infer
optical
depths
(OD)
spanning
majority
oceanic,
(MOD
80)
provides
OD
than
36
respectively.
RT,
between
−30
−23
29
80
here.
Prior
information
or
other
sources
will
required
improve
limit,
where
shown
strong
spatial
structure
varies
viewing
geometry.
Scientific Reports,
Journal Year:
2025,
Volume and Issue:
15(1)
Published: March 10, 2025
Abstract
The
prediction
of
climate
has
been
a
long-standing
problem
in
contemporary
science.
One
the
reasons
stems
from
gap
ability
to
obtain
3D
mapping
clouds,
especially
shallow
scattered
clouds.
These
clouds
are
strongly
affected
by
mixing
processes
with
their
surroundings,
rendering
internal
volumetric
structure
highly
heterogeneous.
heterogeneous
modulate
incoming
solar
energy
and
outgoing
long-wave
radiation,
thereby
having
crucial
role
system.
However,
is
major
challenge.
Here,
we
combine
machine
learning
space
engineering
enable,
for
first
time,
scatterers
We
employ
ten
nano-satellites
formation
simultaneously
view
same
per
scene
different
angles
recover
which
derive
statistics,
including
uncertainty.
demonstrate
this
on
real-world
data.
results
provide
key
features
predicting
precipitation
renewable
energy.
Journal of Geophysical Research Atmospheres,
Journal Year:
2025,
Volume and Issue:
130(5)
Published: March 8, 2025
Abstract
Cloud
adiabatic
fraction
(f
ad
)
is
an
important
metric
that
quantitatively
characterizes
the
impact
of
atmospheric
mixing
on
cloud
thermodynamic
properties.
Due
to
lack
vertical
profiling
water,
previous
studies
variability
f
within
clouds
have
been
confined
single
scales.
Our
prior
research
achieved
a
breakthrough
in
large‐scale
retrieval
fraction,
while
it
only
provided
two‐dimensional
information
leaving
variation
in‐cloud
unquantified.
In
this
study,
utilizing
global‐scale
data
derived
from
our
research,
we
developed
predictive
function
for
global
marine
low‐cloud
based
geometric
thickness
and
base
temperature
(CBT).
This
enabled
us
successfully
estimate
distributions
across
various
conditions
scale.
The
exhibits
quadratic
reduction
top,
which
more
pronounced
at
higher
temperatures.
Specifically,
as
CBT
rises
2
24°C,
diminishes
0.85
0.23.
decreasing
trend
with
increasing
temperatures
expected
reduce
albedo
coverage
potentially
constituting
positive
radiative
feedback
mechanism.
Geophysical Research Letters,
Journal Year:
2024,
Volume and Issue:
51(2)
Published: Jan. 19, 2024
Abstract
Understanding
the
nature
of
mixing
between
cloudy
air
and
its
surroundings
is
an
important
yet,
open
question.
In
this
research,
we
use
high‐resolution
(10
m)
bin‐microphysics
Large
Eddy
Simulation
a
cumulus
cloud,
together
with
Lagrangian
passive
tracer
tracking
method,
to
study
mixing.
We
analyze
tracers
as
function
their
trajectories
thermodynamic
conditions
they
undergo
inside
outside
cloud.
Three
main
regimes
(core,
periphery,
skin)
are
identified,
each
determining
subset
similar
trajectories.
These
can
be
observed
throughout
cloud's
lifetime
provide
evidence
for
presence
undiluted
core
in
shallow
clouds.
At
dissipation
stage,
fourth
regime
identified:
cloud‐top
entrainment
followed
by
downdrafts.
Journal of Geophysical Research Atmospheres,
Journal Year:
2024,
Volume and Issue:
129(14)
Published: July 10, 2024
Abstract
Shallow
convective
clouds
play
a
crucial
role
in
Earth's
energy
budget,
as
they
modulate
the
radiative
transfer
atmosphere
and
participate
vertical
transport
of
aerosols,
energy,
humidity.
The
parameterizations
representing
these
complex,
vital
players
weather
climate
models
are
mostly
based
on
description
steady‐state
plumes
source
major
uncertainty.
Recently,
several
studies
have
shown
that
buoyant
thermals
inherent
atmospheric
convection
contain
toroidal
(ring)
vortex.
This
work
those
vortices
growing
shallow
cumulus
(Cu)
using
high‐resolution
(10
m)
Large
Eddy
Simulations
resolve
much
detail.
Recent
analysis
such
data
showed
small‐scale
turbulent
diffusion
is
unable
to
explain
large
diluted
portion
cloud.
Here
we
advocate
for
important
Cu
vortex
(TV)
cloud
dilution
present
complex
dynamics
structure
TV.
Nevertheless,
since
dominates
cloud's
dilution,
simplicity
emerges
when
considering
lateral
mass
flux
profile.
mixing
quantified
direct
calculations
Eulerian
tracers.
In
addition,
Lagrangian
tracers
used
identify
origin
entrained
air
its
thermodynamic
properties.
It
shows
most
by
not
recycled
vortex,
yet
significantly
more
humid
than
environment.
We
suggest
development
new
describing
thermals,
together
with
their
vortices,
might
improve
models.
IEEE Transactions on Pattern Analysis and Machine Intelligence,
Journal Year:
2022,
Volume and Issue:
unknown, P. 1 - 12
Published: Aug. 2, 2022
Scattering-based
computed
tomography
(CT)
recovers
a
heterogeneous
volumetric
scattering
medium
using
images
taken
from
multiple
directions.
It
is
nonlinear
problem.
Prior
art
mainly
approached
it
by
explicit
physics-based
optimization
of
image-fitting,
being
slow
and
difficult
to
scale.
Scale
particularly
important
when
the
objects
constitute
large
cloud
fields,
where
recovery
for
climate
studies.
Besides
speed,
imaging
need
be
flexible,
efficiently
handle
variable
viewing
geometries
resolutions.
These
can
caused
perturbation
in
camera
poses
or
fusion
data
different
types
observational
sensors.
There
fast
projection
clouds
(VIP-CT).
We
develop
learning-based
solution,
deep-neural
network
(DNN)
which
trains
on
labeled
dataset.
The
DNN
parameters
are
oblivious
domain
scale,
hence
work
with
arbitrarily
domains.
VIP-CT
offers
much
better
quality
than
state
art.
inference
speed
flexibility
make
effectively
real-time
context
spaceborne
observations.
paper
first
demonstrate
CT
real
empirical
directly
DNN.
may
offer
model
solution
problems
other
scientific
Our
code
available
online.
Atmospheric measurement techniques,
Journal Year:
2023,
Volume and Issue:
16(7), P. 1803 - 1847
Published: April 5, 2023
Abstract.
Our
global
understanding
of
clouds
and
aerosols
relies
on
the
remote
sensing
their
optical,
microphysical,
macrophysical
properties
using,
in
part,
scattered
solar
radiation.
These
retrievals
assume
that
form
plane-parallel,
homogeneous
layers
utilize
1D
radiative
transfer
(RT)
models,
limiting
detail
can
be
retrieved
about
3D
variability
cloud
aerosol
fields
inducing
biases
for
highly
heterogeneous
structures
such
as
cumulus
smoke
plumes.
To
overcome
these
limitations,
we
introduce
validate
an
algorithm
retrieving
optical
or
microphysical
atmospheric
particles
using
multi-angle,
multi-pixel
radiances
a
RT
model.
The
retrieval
software,
which
have
made
publicly
available,
is
called
Atmospheric
Tomography
with
Radiative
Transfer
(AT3D).
It
uses
iterative,
local
optimization
technique
to
solve
generalized
least
squares
problem
thereby
find
best-fitting
state.
iterative
fast,
approximate
Jacobian
calculation,
extended
from
Levis
et
al.
(2020)
accommodate
open
periodic
horizontal
boundary
conditions
(BCs)
improved
treatment
non-black
surfaces.
We
validated
accuracy
calculation
derivatives
respect
both
volume
extinction
coefficient
parameters
controlling
across
media
range
depths
single-scattering
it
accurate
majority
over
oceanic
Relative
root
mean
square
errors
cloud-like
increase
2
%
12
maximum
(MODs)
medium
0.2
100.0
surfaces
Lambertian
albedos
<0.2.
Over
0.7,
20
%.
Errors
exceed
50
%,
unless
plane-parallel
providing
are
optically
very
thin
(∼0.1).
use
theory
linear
inverse
provide
insight
into
physical
processes
control
tomography
identify
its
supported
by
numerical
experiments.
show
matrix
becomes
increasing
ill-posed
size
increases
forward-scattering
peak
phase
function
decreases.
This
suggests
tomographic
will
become
increasingly
difficult
thicker.
Retrievals
asymptotically
thick
likely
require
other
sources
information
successful.
In
Loveridge
(2023a;
hereafter
Part
2),
examine
how
varies
target
synthetic
data.
do
this
explore
error
nature
inversion
limit
affect
retrieval.
also
assess
compare
them
transfer.
Journal of Geophysical Research Atmospheres,
Journal Year:
2023,
Volume and Issue:
128(2)
Published: Jan. 7, 2023
Abstract
Anthropogenic
activities
have
drastically
impacted
the
climate
system
since
Industrial
Revolution.
However,
to
what
extent
anthropogenic
emissions
influence
cloud
droplet
number
concentration
(
N
d
),
critical
parameter
for
understanding
aerosol‐cloud
interactions,
is
poorly
known
on
hemispheric
scale
due
considerable
retrieval
uncertainty.
We
employed
multiple
widely
used
sampling
methods
evaluate
long‐term
trend
in
contrast
(Δ
d(NH‐SH)
)
between
Northern
Hemisphere
(NH)
and
Southern
(SH).
Here
we
show
that
Δ
was
halved
from
2003
2020
using
different
channels,
even
though
range
of
magnitudes
large.
Such
dramatic
changes
are
dominated
by
significantly
decreased
over
NH
(∼20%)
emission
reductions
compared
relatively
stable
pristine
nature
SH.
Aerosol
optical
depth
(AOD)
aerosol
index
(AI)
correlate
with
based
trends,
they
replicate
trends.
This
poor
correlation
partly
contributed
stratospheric
smoke
wildfires
Australia
had
little
The
northwest
Atlantic
shows
largest
contribution,
∼38%,
trend,
whereas
Pacific
dominates
change
AOD
AI,
contributing
more
than
60%
∼50%
AI
NH.
Our
results
imply
reduced
provide
strong
observational
evidence
extensively
altered
liquid
clouds
last
two
decades.
Geophysical Research Letters,
Journal Year:
2023,
Volume and Issue:
50(13)
Published: June 29, 2023
Abstract
This
study
investigates
the
lifetime
and
temporal
evolution
of
physical
properties
trade‐wind
cumuli
based
on
tracking
individual
clouds
in
observations
with
Advanced
Baseline
Imager
aboard
geostationary
GOES‐16
satellite
during
“ElUcidating
RolE
Cloud–Circulation
Coupling
ClimAte”
(EUREC
4
A)
campaign
east
Barbados
winter
2020.
A
first
application
our
upgraded
cloud‐tracking
toolbox
to
measurements
high
spatio‐temporal
resolution
(2
×
2
km
1
min)
provides
probability
density
functions
area
that
develop
as
a
consequence
meso‐to‐synoptic
scale
motions.
By
separately
considering
exist
daytime
live
distinct
intervals,
we
find
shallow
marine
longer
when
they
cover
larger
surface
show
higher
cloud
optical
thickness
(COT).
Besides
effect
COT,
atmospheric
motions
which
interact
is
also
critical
their
lifetime.
Geophysical Research Letters,
Journal Year:
2023,
Volume and Issue:
50(22)
Published: Nov. 17, 2023
Abstract
The
fraction
of
cloud
water
compared
to
its
adiabatic
value
is
defined
as
the
fraction,
f
ad
.
accuracy
representation
in
climate
models
highly
sensitive
mixing
rate,
manifested
Here,
we
present
first
distribution
marine
boundary
layer
clouds
over
global
oceans,
retrieved
by
satellite
observations.
shown
decrease
exponentially
with
base
temperature
(CBT)
and
depth,
agreement
increasing
evaporation
capacity
entrained
warmer
air.
Cloud
cover
decreases
CBT,
but
a
much
lesser
extent
than
dependence
on
CBT
has
little
relative
humidity
or
precipitation.
relationship
between
highlights
importance
core
control
factor
evaporation.
simultaneous
content
can
lead
positive
feedback,
resulting
greater
future
warming.
Journal of the Atmospheric Sciences,
Journal Year:
2021,
Volume and Issue:
79(3), P. 793 - 813
Published: Dec. 22, 2021
Abstract
The
dynamic
structure
of
a
small
trade
wind
cumulus
(Cu)
is
analyzed
using
novel
approach.
Cu
developing
in
shear-free
environment
simulated
by
10-m-resolution
LES
model
with
spectral
bin
microphysics.
aim
to
clarify
the
dynamical
nature
cloud
updraft
zone
(CUZ)
including
entrainment
and
mixing
growing
Cu.
validity
concept
stating
that
at
state
can
be
represented
parcel
or
jet
tested.
To
investigate
CUZ
performed
motions
scales
larger
than
turbulence
scales,
modeled
fields
air
velocity
were
filtered
wavelet
filter
separated
convective
from
turbulent
ones.
Two
types
objects
investigated:
volume
ascending
maximal
(point
parcel)
CUZ.
It
was
found
point
representing
upper
part
core
adiabatic.
motion
this
base
determines
cloud-top
height.
top-hat
(i.e.,
averaged)
values
adiabatic
fraction
are
substantially
lower
those
parcel.
Evaluation
terms
equation
typically
used
1D
models
show
applied
for
calculation
vertical
velocities
stage
Cu,
least
up
heights
inversion
layer.
Dynamically,
resembles
starting
plume
tail
nonstationary
jet.
Both
buoyancy
acceleration
linearly
increase
height,
An
important
finding
lateral
(nonturbulent)
has
little
effect
on
cannot
explain
changes
conservative
variables
q
t
θ
l
.
In
contrast,
entrained
lifting
inside
decreases
liquid
water
content
its
fraction.
Possible
reasons
these
effects
discussed.
Significance
Statement
(i)
study
improves
understanding
mixing.
(ii)
shows
dominating
role
convective-scale
microphysics
dynamics.
(iii)
comparison
results
large-eddy
simulations
simple
allows
evaluating
current
schemes
parameterization.