Proceedings of the National Academy of Sciences,
Journal Year:
2019,
Volume and Issue:
116(17), P. 8173 - 8177
Published: April 5, 2019
Significance
Laser-induced
electron
diffraction
is
a
molecular-scale
microscopy
that
captures
clean
snapshots
of
molecule’s
geometry
with
subatomic
picometer
and
attosecond
spatiotemporal
resolution.
We
induce
unambiguously
identify
the
stretching
bending
linear
triatomic
molecule
following
excitation
to
an
excited
electronic
state
bent
stretched
geometry.
show
we
can
directly
retrieve
structure
electronically
molecules
otherwise
possible
through
indirect
retrieval
methods
such
as
pump–probe
rotational
spectroscopy
measurements.
Advances in Optics and Photonics,
Journal Year:
2022,
Volume and Issue:
14(4), P. 652 - 652
Published: Aug. 31, 2022
The
advent
of
chirped-pulse
amplification
in
the
1980s
and
femtosecond
Ti:sapphire
lasers
1990s
enabled
transformative
advances
intense
laser–matter
interaction
physics.
Whereas
most
experiments
have
been
conducted
limited
near-infrared
range
0.8–1
μm,
theories
predict
that
many
physical
phenomena
such
as
high
harmonic
generation
gases
favor
long
laser
wavelengths
terms
extending
high-energy
cutoff.
Significant
progress
has
made
developing
few-cycle,
carrier-envelope
phase-stabilized,
high-peak-power
1.6–2
μm
laid
foundation
for
attosecond
X
ray
sources
water
window.
Even
longer
wavelength
are
becoming
available
suitable
to
study
light
filamentation,
generation,
laser–plasma
relativistic
regime.
Long-wavelength
sub-bandgap
strong-field
excitation
a
wide
solid
materials,
including
semiconductors.
In
limit,
bulk
crystals
also
produce
high-order
harmonics.
this
review,
we
first
introduce
several
important
scaling
laws
physics,
then
describe
recent
breakthroughs
short-
(1.4–3
μm),
mid-
(3–8
long-wave
(8–15
μm)
infrared
technology,
finally
provide
examples
applications
these
novel
lasers.
Some
broadband
ultrafast
will
profound
effects
on
medicine,
environmental
protection,
national
defense,
because
their
cover
absorption
band,
molecular
fingerprint
region,
well
atmospheric
transparent
APL Photonics,
Journal Year:
2018,
Volume and Issue:
3(11)
Published: Nov. 1, 2018
Mode-locked
fiber
laser
technology
to
date
has
been
limited
sub-3
μm
wavelengths
despite
significant
application-driven
demand
for
compact
picosecond
and
femtosecond
pulse
sources
at
longer
wavelengths.
Erbium-doped
holmium-doped
fluoride
lasers
incorporating
a
saturable
absorber
are
emerging
as
promising
2.7–2.9
μm,
yet
it
remains
major
challenge
extend
this
coverage.
Here,
we
propose
new
approach
using
dysprosium-doped
with
frequency
shifted
feedback
(FSF).
Using
simple
linear
cavity
an
acousto-optic
tunable
filter,
generate
∼33
ps
pulses
up
2.7
nJ
energy
330
nm
tunability
from
2.97
3.30
(∼3000–3400
cm−1)—the
first
mode-locked
cover
spectral
region
the
most
broadly
pulsed
date.
Numerical
simulations
show
excellent
agreement
experiments
also
offer
insights
into
underlying
dynamics
of
FSF
generation.
This
highlights
remarkable
potential
both
dysprosium
gain
material
versatile
generation,
opening
opportunities
mid-IR
development
practical
applications
outside
laboratory.
Optics Letters,
Journal Year:
2019,
Volume and Issue:
44(13), P. 3194 - 3194
Published: June 14, 2019
We
present
a
state-of-the-art
compact
high-energy
mid-infrared
(mid-IR)
laser
system
for
TW-level
eight-cycle
pulses
at
7
μm.
This
consists
of
an
Er:Tm:Ho:fiber
MOPA
which
serves
as
the
seeder
ZGP-based
optical
parametric
chirped
pulse
amplification
(OPCPA)
chain,
in
addition
to
Ho:YLF
amplifier
is
Tm:fiber
pumped.
Featuring
all-optical
synchronization,
delivers
260
mJ
pump
energy
2052
nm
and
16
ps
duration
100
Hz
with
stability
0.8%
rms
over
20
min.
show
that
chirp
inversion
OPCPA
chain
leads
excellent
extraction
aids
compression
μm
eight
cycles
(188
fs)
bulk
BaF2
93.5%
efficiency.
Using
21.7
available
energy,
we
generate
0.75
due
increased
efficiency
scheme.
The
quality
system's
output
shown
by
generating
high
harmonics
ZnSe
span
up
harmonic
order
13
contrast.
combination
passive
carrier-envelope
phase
stable
mid-IR
seed
picosecond
makes
this
key
enabling
tool
next
generation
studies
on
extreme
photonics,
strong
field
physics,
table-top
coherent
X-ray
science.
Optics Letters,
Journal Year:
2018,
Volume and Issue:
43(6), P. 1347 - 1347
Published: March 12, 2018
UV
guiding
fibers
are
highly
sought
after
in
laser
and
spectroscopy
applications.
Recent
advances
hollow-core
fiber
orient
a
practical
approach
for
proper
light
delivery
sustainable
to
high-power
long-term
irradiation.
In
this
Letter,
we
report
two
types
of
negative-curvature
(NCFs)
spectral
range.
Their
structures
consist
one
ring
six
small
(7.9
μm
diameter)
four
big
(20.8
tubes,
enclosing
hollow
core
similar
size
(∼15
diameter).
The
six-tube
NCF
shows
an
attenuation
level
0.13±0.01
dB/m
at
300
nm.
It
is
capable
delivering
20
ps,
160
μJ
pulses
355
nm
with
no
damage
the
facet.
novel
four-tube
exhibits
∼0.3±0.15
Its
fundamental
mode
guided
intentionally
designed
"cladding
mismatching"
region.
This
design
possesses
high
degree
down-scalability
deep-UV
guidance
has
potential
attaining
polarization-maintaining
performance.
Journal of Physics B Atomic Molecular and Optical Physics,
Journal Year:
2019,
Volume and Issue:
52(17), P. 171001 - 171001
Published: July 25, 2019
Abstract
We
publish
three
Roadmaps
on
photonic,
electronic
and
atomic
collision
physics
in
order
to
celebrate
the
60th
anniversary
of
ICPEAC
conference.
In
Roadmap
I,
we
focus
light–matter
interaction.
this
area,
studies
ultrafast
molecular
dynamics
have
been
rapidly
growing,
with
advent
new
light
sources
such
as
attosecond
lasers
x-ray
free
electron
lasers.
parallel,
experiments
established
synchrotron
radiation
femtosecond
using
cutting-edge
detection
schemes
are
revealing
scientific
insights
that
never
exploited.
Relevant
theories
also
being
developed.
Target
samples
for
photon-impact
expanding
from
atoms
small
molecules
complex
systems
biomolecules,
fullerene,
clusters
solids.
This
aims
look
back
along
road,
explaining
development
these
fields,
forward,
collecting
contributions
twenty
leading
groups
field.
Optics Express,
Journal Year:
2020,
Volume and Issue:
28(7), P. 9099 - 9099
Published: March 5, 2020
Over
the
past
years,
ultrafast
lasers
with
average
powers
in
100
W
range
have
become
a
mature
technology,
multitude
of
applications
science
and
technology.
Nonlinear
temporal
compression
these
to
few-
or
even
single-cycle
duration
is
often
essential,
yet
still
hard
achieve,
particular
at
high
repetition
rates.
Here
we
report
two-stage
system
for
compressing
pulses
from
1030
nm
ytterbium
fiber
laser
durations
5
µJ
output
pulse
energy
9.6
MHz
rate.
In
first
stage,
are
compressed
340
25
fs
by
spectral
broadening
krypton-filled
single-ring
photonic
crystal
(SR-PCF),
subsequent
phase
compensation
being
achieved
chirped
mirrors.
second
further
soliton-effect
self-compression
neon-filled
SR-PCF.
We
estimate
∼3.4
numerically
back-propagating
measured
pulses.
Finally,
directly
3.8
(1.25
optical
cycles)
after
compensating
(using
mirrors)
dispersion
introduced
elements
fiber,
more
than
50%
total
main
peak.
The
can
produce
peak
>0.6
GW
transmission
exceeding
66%.
Journal of Physics B Atomic Molecular and Optical Physics,
Journal Year:
2021,
Volume and Issue:
54(7), P. 070201 - 070201
Published: April 7, 2021
Since
2001
and
the
first
demonstrations
of
feasibility
generating
measuring
attosecond
light
pulses,
science
has
developed
into
a
very
active
quickly
evolving
research
field.
Its
ultimate
goal
is
real-time
tracking
electron
dynamics
in
all
forms
matter,
ranging
from
atoms
large
molecules
to
condensed
phase
plasmas.
The
accomplishment
this
required
still
calls
for
developments
ultrafast
laser
technology,
metrology,
extreme
ultra-violet
(XUV)
optics,
pump–probe
measurement
schemes
non-linear
laser-matter
interaction.
Moreover,
interpretation
experimental
results
experiments
stimulated
guided
major
theoretical
descriptions
electronic
processes
matter.
Motivated
by
these
two
decades
development,
several
large-scale
facilities,
including
infrastructure—attosecond
pulse
source
(ELI-ALPS)
free
facilities
(the
linac
coherent
(LCLS)
at
Stanford
European
XFEL
Hamburg)
are
now
pushing
development
new
generation
sources.
This
considerable
technological
effort
opens
important
perspectives
field
with
potential
applications
photochemistry,
photobiology
advanced
electronics.
In
context,
joint
focus
issue
on
Attosecond
technology(/ies)
J.
Phys.
Photon.
B:
At.
Mol.
Opt.
aims
provide
an
overview
state-of-the-art
science,
basic
involved
pulses
technologies
that
required.
Abstract
Bright,
coherent
soft
X-ray
radiation
is
essential
to
a
variety
of
applications
in
fundamental
research
and
life
sciences.
To
date,
high
photon
flux
this
spectral
region
can
only
be
delivered
by
synchrotrons,
free-electron
lasers
or
high-order
harmonic
generation
sources,
which
are
driven
kHz-class
repetition
rate
with
very
peak
powers.
Here,
we
establish
novel
route
toward
powerful
easy-to-use
SXR
sources
presenting
compact
experiment
nonlinear
pulse
self-compression
the
few-cycle
regime
combined
phase-matched
single,
helium-filled
antiresonant
hollow-core
fibre.
This
enables
first
100
rate,
table-top
source
that
delivers
an
application-relevant
2.8
×
10
6
s
−1
eV
around
300
eV.
The
fibre
integration
temporal
(leading
formation
necessary
strong-field
waveforms)
pressure-controlled
phase
matching
will
allow
compact,
high-repetition-rate
laser
technology,
including
commercially
available
systems,
drive
simple
cost-effective,
high-flux
sources.
Applied Physics Reviews,
Journal Year:
2021,
Volume and Issue:
8(1)
Published: March 1, 2021
Recent
developments
in
attosecond
technology
led
to
tabletop
X-ray
spectroscopy
the
soft
range,
thus
uniting
element-
and
state-specificity
of
core-level
x-ray
absorption
with
time
resolution
follow
electronic
dynamics
real
time.
We
describe
recent
work
investigations
into
materials
such
as
Si,
SiO2,
GaN,
Al2O3,
Ti,
TiO2,
enabled
by
convergence
these
two
capabilities.
showcase
state-of-the-art
on
isolated
pulses
for
near
edge
(XANES)
observe
3d-state
semi-metal
TiS2
at
Ti
L-edge
(460
eV).
how
transition
metal
quantum
material
allows
unambiguously
identify
where
optical
field
influences
charge
carriers.
This
precision
elucidates
that
Ti:3d
conduction
band
states
are
efficiently
photo-doped
a
density
1.9
x
10^21
cm^-3
light-field
induces
coherent
motion
intra-band
carriers
across
38%
first
Brillouin
zone.
Lastly,
we
prospects
unambiguous
real-time
observation
carrier
specific
bonding
or
anti-bonding
speculate
capability
will
bring
unprecedented
opportunities
towards
an
engineered
approach
designer
pre-defined
properties
efficiency.
Examples
composites
semiconductors
insulators
like
Ge,
BN,
graphene,
TMDCs,
high-Tc
superconductors
NbN
LaBaCuO.
Exiting
scrutinize
canonical
questions
multi-body
physics
whether
electrons
lattice
trigger
phase
transitions.
Abstract
Generating
intense
ultrashort
pulses
with
high-quality
spatial
modes
is
crucial
for
ultrafast
and
strong-field
science
can
be
achieved
by
nonlinear
supercontinuum
generation
(SCG)
pulse
compression.
In
this
work,
we
propose
that
the
of
quasi-stationary
solitons
in
periodic
layered
Kerr
media
greatly
enhance
light-matter
interaction
fundamentally
improve
performance
SCG
compression
condensed
media.
With
both
experimental
theoretical
studies,
successfully
identify
these
solitary
reveal
their
unified
condition
stability.
Space-time
coupling
shown
to
strongly
influence
stability
solitons,
leading
variations
spectral,
temporal
profiles
femtosecond
pulses.
Taking
advantage
unique
characteristics
modes,
first
demonstrate
single-stage
from
170
22
fs
an
efficiency
>85%.
The
high
spatiotemporal
quality
compressed
further
confirmed
high-harmonic
generation.
We
also
provide
evidence
efficient
mode
self-cleaning,
which
suggests
rich
self-organization
laser
beams
a
resonator.
This
work
offers
route
towards
highly
efficient,
simple,
stable
flexible
solutions
state-of-the-art
ytterbium
technology.