
Published: April 15, 2024
The use of homogeneous Bronsted acid cocatalysts (such as benzoic acid) in hydroacylation reactions via imine intermediates has been extensively studied, but the heterogeneous limited to montmorillonite K10. Thus, we can other solid acids increase efficiency reaction. Here, described effects sulfated zirconia, Al-MCM-41 or superacid modified on alkenes and alkynes with aldehydes presence Wilkinson complex. Furthermore, addressed dual role montmorillonite, a redox reagent TEMPO an solid, allowing direct benzyl alcohols substrates generate saturated a-b unsaturated ketones.
Language: Английский