Russian Investigations in the Field of Amtospheric Radiation in 2019–2022 DOI

Yu. M. Timofeyev,

Vladimir P. Budak, Ya. A. Virolainen

et al.

Известия Российской академии наук Физика атмосферы и океана, Journal Year: 2023, Volume and Issue: 59(7), P. 976 - 1007

Published: Dec. 1, 2023

The main results of scientific research and development in the field atmospheric radiation Russia for period 2019–2022 are considered attention is paid to radiative transfer theory, spectroscopy, climatology, aerosol forcing, remote sensing atmosphere surface, interpretation satellite measurements Lists major publications these areas this provided.

Language: Английский

Phase Behavior and Viscosity in Biomass Burning Organic Aerosol and Climatic Impacts DOI
Florence K. A. Gregson, Nealan G. A. Gerrebos, Meredith Schervish

et al.

Environmental Science & Technology, Journal Year: 2023, Volume and Issue: 57(39), P. 14548 - 14557

Published: Sept. 20, 2023

Smoke particles generated by burning biomass consist mainly of organic aerosol termed (BBOA). BBOA influences the climate scattering and absorbing solar radiation or acting as nuclei for cloud formation. The viscosity phase behavior (i.e., number type phases present in a particle) are properties that expected to impact several climate-relevant processes but remain highly uncertain. We studied using fluorescence microscopy showed comprise two (a hydrophobic hydrophilic phase) across wide range atmospheric relative humidity (RH). determined at room temperature photobleaching method possess different RH-dependent viscosities. is largely independent RH from 0 95%. use Vogel–Fulcher–Tamman equation extrapolate our results colder warmer temperatures, based on extrapolation, predicted be glassy (viscosity >1012 Pa s) temperatures less than 230 K RHs below 95%, with possible implications heterogeneous reaction kinetics formation atmosphere. Using kinetic multilayer model (KM-GAP), we investigated effect lifetime brown carbon within BBOA, which climate-warming agent. presence can increase planetary boundary layer polar regions compared previous modeling studies. Hence, lead an warming climate.

Language: Английский

Citations

18

On the importance of the model representation of organic aerosol in simulations of the direct radiative effect of Siberian biomass burning aerosol in the eastern Arctic DOI
I. B. Konovalov, Nikolai A. Golovushkin,

Matthias Beekmann

et al.

Atmospheric Environment, Journal Year: 2023, Volume and Issue: 309, P. 119910 - 119910

Published: June 21, 2023

Language: Английский

Citations

7

Biomass burning organic aerosol (BBOA) from wildfires has multiple phases and is more viscous than laboratory generated BBOA DOI Creative Commons
Nealan G. A. Gerrebos, Julia Zaks, Florence K. A. Gregson

et al.

Published: May 7, 2024

Biomass burning organic aerosol (BBOA) is a major contributor to in the atmosphere. The impacts of BBOA on climate and health depend strongly their physicochemical properties, including viscosity phase behaviour (number types phases); these relationships chemistry, are not yet fully characterized. We collected field samples during 2021 British Columbia wildfire season constrain at range relative humidities, compared them laboratory generated made from smoldering pine wood. Particles all exhibited two-phased with higher polarity hydrophilic core lower hydrophobic shell. used poke-flow technique estimate particles. found that both phases had viscosities >10 8 Pa s humidities up 50%, which more viscous than any or proxies previously measured. Aerosol mass spectrometry showed were oxidized those lab, likely explanation for viscosity. two high have implications how should be treated atmospheric models

Language: Английский

Citations

1

Model Analysis of Origination of Semidirect Radiative Effect of Siberian Biomass Burning Aerosol in the Arctic DOI
I. B. Konovalov, Nikolai A. Golovushkin

Atmospheric and Oceanic Optics, Journal Year: 2024, Volume and Issue: 37(3), P. 382 - 393

Published: June 1, 2024

Language: Английский

Citations

1

High Viscosity and Two Phases Observed over a Range of Relative Humidities in Biomass Burning Organic Aerosol from Canadian Wildfires DOI
Nealan G. A. Gerrebos, Julia Zaks, Florence K. A. Gregson

et al.

Environmental Science & Technology, Journal Year: 2024, Volume and Issue: unknown

Published: Nov. 28, 2024

Biomass burning organic aerosol (BBOA) is a major contributor to in the atmosphere. The impacts of BBOA on climate and health depend strongly upon their physicochemical properties, including viscosity phase behavior (number types phases); these properties are not yet fully characterized. We collected field samples during 2021 British Columbia wildfire season constrain at range relative humidities compared them previous studies BBOA. Particles from all exhibited two-phased with polar hydrophilic nonpolar hydrophobic phase. used poke-flow technique estimate particles. Both phases had viscosities >108 Pa s up 50%. Such high correspond mixing times within 200 nm particles >5 h. Two have implications for how should be treated atmospheric models.

Language: Английский

Citations

1

Application of the CHIMERE-WRF Model Complex to Study the Radiative Effects of Siberian Smoke Aerosol in the Eastern Arctic DOI Creative Commons
I. B. Konovalov, Nikolai A. Golovushkin, T. B. Zhuravleva

et al.

Atmospheric and Oceanic Optics, Journal Year: 2023, Volume and Issue: 36(4), P. 337 - 347

Published: Aug. 1, 2023

Abstract We describe a computational technology for studying the effects of aerosol-radiation interaction and calculating regional estimates direct (DRE) semidirect radiative (SDRE) biomass burning (BB) aerosol based on simulations with CHIMERE chemistry transport model coupled WRF meteorological model. The was applied to numerical Siberian in eastern Arctic period July 16–31, 2016. show that smokes, whole, had significant cooling effect atmosphere due DRE, value which at top was, average, −6.0 W m −2 , being minimal over snow-ice cover ocean (−1.2 ). At same time, contribution BB DRE balance is found be offset certain extent by SDRE, positive (2.0 ), average. SDRE formed as result multihour processes plays most important role covers, where it exceeds absolute value. It has been shown BBA our experiments mainly scattering (rather than absorption) radiation particles.

Language: Английский

Citations

3

Radiative Forcing of Smoke Aerosol Taking into Account the Photochemical Evolution of Its Organic Component: Impact of Illumination Conditions and Surface Albedo DOI
T. B. Zhuravleva, I. M. Nasrtdinov, I. B. Konovalov

et al.

Atmospheric and Oceanic Optics, Journal Year: 2022, Volume and Issue: 35(S1), P. S113 - S124

Published: Dec. 1, 2022

Language: Английский

Citations

4

Atmospheric and Ocean Optics: Atmospheric Physics III DOI Creative Commons
О. А. Romanovskii, О. V. Kharchenko

Atmosphere, Journal Year: 2022, Volume and Issue: 13(11), P. 1912 - 1912

Published: Nov. 17, 2022

This Special Issue aimed to collect novel papers presented at the 27th International Conference on “Atmospheric and Ocean Optics: Atmospheric Physics” (AOO—21) held from 5 9 July 2021 in Moscow, Russia [...]

Language: Английский

Citations

3

Dynamics of Microphysical Parameters of Pyrolysis Smoke Based on the Results of Inversion of Aerosol Scattering and Extinction Coefficients in the Big Aerosol Chamber of IAO SB RAS DOI

V. V. Veretennikov,

V. N. Uzhegov,

Vladimir P. Shmargunov

et al.

Atmospheric and Oceanic Optics, Journal Year: 2024, Volume and Issue: 37(3), P. 327 - 337

Published: June 1, 2024

Language: Английский

Citations

0

Microphysical parameters of smoke aerosols based on the results of inversion of aerosol scattering and extinction coefficients in a big aerosol chamber of IAO SB RAS DOI

V. V. Veretennikov,

V. N. Uzhegov,

Vladimir P. Shmargunov

et al.

27th International Symposium on Atmospheric and Ocean Optics, Atmospheric Physics, Journal Year: 2022, Volume and Issue: unknown, P. 177 - 177

Published: Dec. 8, 2022

Measurements of polarization scattering phase functions and spectral extinction coefficients were carried out in smoke aerosols formed as a result thermal decomposition wood materials, big aerosol chamber (BAC) the IAO SB RAS. The results are presented reconstructing parameters microstructure complex refractive index based on developed algorithm for inverting optical measurements. Temporal variability microphysical characteristics is studied.

Language: Английский

Citations

2