Abstract.
In
situ
cloud
probe
data
from
the
NASA
ObseRvations
of
Aerosols
above
CLouds
and
their
intEractionS
(ORACLES)
field
campaign
were
used
to
estimate
effective
radius
(Re),
optical
thickness
class="inline-formula">Ï),
droplet
concentration
class="inline-formula">Nc)
for
marine
stratocumulus
over
southeast
Atlantic
Ocean.
The
in
Re,
class="inline-formula">Ï,
class="inline-formula">Nc
compared
with
co-located
Moderate
Resolution
Imaging
Spectroradiometer
(MODIS)
retrievals
class="inline-formula">Re
class="inline-formula">Ï
MODIS-derived
class="inline-formula">Nc.
For
145
profiles,
a
MODIS
retrieval
was
time
gap
less
than
1âh.
On
average,
(11.3âµm
11.7)
1.6âR)
0.77
0.73,
respectively.
average
(151.5âcmâ3)
within
1âcmâ3
an
class="inline-formula">R
0.90.
profiles
classified
into
67
contact
where
aerosol
class="inline-formula">Na)
greater
500âcmNa
up
tops.
Contact
had
(by
88âcmâ3),
2.5),
lower
2.2âµm)
profiles.
These
differences
associated
aerosolâcloud
interactions
(ACI),
estimates
5âcmâ3,
0.5,
0.2âRe>15âÏ>25
removed.
agreement
between
changes
ACI
driven
by
small
biases
properties
relative
measurements
across
different
regimes.
Thus,
combined
location
concentration,
can
be
study
larger
domains
longer
timescales
possible
using
data.
Atmospheric chemistry and physics,
Journal Year:
2022,
Volume and Issue:
22(12), P. 8259 - 8285
Published: June 27, 2022
Abstract.
The
cloud
drop
effective
radius
(Re)
of
the
size
distribution
derived
from
passive
satellite
sensors
is
a
key
variable
used
in
climate
research.
Validation
these
products
has
often
taken
place
under
stratiform
conditions
that
favor
assumption
horizontal
homogeneity
by
retrieval
techniques.
However,
many
studies
have
noted
concerns
with
respect
to
significant
biases
retrieved
Re
arising
heterogeneity,
for
example,
cumulus
fields.
Here,
we
examine
data
collected
during
2019
“Cloud,
Aerosol
and
Monsoon
Processes
Philippines
Experiment”
(CAMP2Ex),
which,
part,
targeted
objective
providing
first
detailed
evaluation
across
multiple
platforms
techniques
congestus
region.
Our
consists
cross-comparisons
between
Moderate
Resolution
Imaging
Spectroradiometer
(MODIS)
onboard
Terra
satellite,
Research
Scanning
Polarimeter
(RSP)
NASA
P-3
aircraft,
situ
measurements
both
Learjet
aircraft
are
all
close
spatiotemporal
proximity
same
A
particular
advantage
our
approach
lies
capability
RSP
retrieve
using
bi-spectral
MODIS
polarimetric
approach,
which
allows
retrievals
an
airborne
perspective
samples.
Averaged
over
flight
segments
examined
here
warm
clouds,
method,
bias-adjusted
method
Fu
et
al.
(2019)
show
comparable
median
(mean
±
standard
deviation)
samples
9.6
(10.2
4.0)
µm,
11.0
(13.6
11.3)
10.4
(10.8
3.8)
respectively.
These
values
far
lower
than
15.1
(16.2
5.5)
µm
17.2
(17.7
5.7)
MODIS,
Similar
results
observed
when
segregated
cloud-top
height
case
studies.
clouds
sampled
CAMP2Ex
consist
mostly
small
transect
length
∼
1.4
km)
low
1
km),
had
more
numerous
trade
wind
cumuli
past
field
campaigns
such
as
Rain
Shallow
Cumulus
Ocean
(RICO)
Indian
Experiment
(INDOEX).
overestimates
technique
compared
increased
optical
depth
decreased.
Drizzle,
bumpiness,
solar
zenith
angle,
however,
not
closely
correlated
overestimate
Re.
For
shallow
dominated
liquid
cover
region
period,
3-D
radiative
transfer
particularly
optically
thin
appear
be
leading
cause
large
positive
retrievals.
Because
this
bias
varies
underlying
structure
field,
caution
continues
warranted
use
Atmospheric measurement techniques,
Journal Year:
2025,
Volume and Issue:
18(4), P. 981 - 1011
Published: Feb. 27, 2025
Abstract.
Satellite
remote
sensing
retrievals
of
cloud
effective
radius
(CER)
are
widely
used
for
studies
aerosol–cloud
interactions.
Such
retrievals,
however,
rely
on
forward
radiative
transfer
(RT)
calculations
using
simplified
assumptions
that
can
lead
to
retrieval
errors
when
the
real
atmosphere
deviates
from
model.
Here,
coincident
airborne
and
in
situ
observations
obtained
during
NASA's
ObseRvations
Aerosols
above
CLouds
their
intEractionS
(ORACLES)
field
campaign
evaluate
CER
marine
boundary
layer
stratocumulus
clouds
explore
impacts
RT
model
other
confounding
factors.
Specifically,
spectral
Enhanced
MODIS
Airborne
Simulator
(eMAS)
Research
Scanning
Polarimeter
(RSP)
compared
with
polarimetric
RSP
derived
droplet
size
distributions
(DSDs)
observed
by
Phase
Doppler
Interferometer
(PDI)
a
combination
Cloud
Aerosol
Spectrometer
(CAS)
Two-Dimensional
Stereo
Probe
(2D-S).
The
sensitivities
eMAS
about
DSD
variance
(CEV)
liquid
water
complex
index
refraction
explored.
CEV
inferred
reflectance
backscatter
glory
provide
additional
context
retrievals.
agreement
is
case
dependent,
updating
assumptions,
including
as
constraint,
yields
mixed
results
tied
differing
vertical
heterogeneity.
Moreover,
probes,
often
benchmark
assessments,
themselves
do
not
agree,
PDI
DSDs
yielding
values
1.3–1.6
µm
larger
than
CAS
roughly
50
%–60
%
smaller
CAS.
Implications
interpretation
discussed.
Atmosphere,
Journal Year:
2022,
Volume and Issue:
13(4), P. 586 - 586
Published: April 5, 2022
Changes
in
marine
boundary
layer
cloud
(MBLC)
radiative
properties
response
to
aerosol
perturbations
are
largely
responsible
for
uncertainties
future
climate
predictions.
In
particular,
the
relationship
between
droplet
number
concentration
(Nd,
a
proxy
aerosol)
and
liquid
water
path
(LWP)
remains
challenging
quantify
from
observations.
this
study,
satellite
observations
multiple
polar-orbiting
platforms
2006–2011
used
combination
with
atmospheric
reanalysis
data
regional
machine
learning
model
predict
changes
LWP
MBLCs
Southeast
Atlantic.
The
impact
of
predictor
variables
on
output
is
analysed
using
Shapley
values
as
technique
explainable
learning.
Within
model,
precipitation
fraction,
top
height,
Nd
identified
important
state
predictors
LWP,
dynamical
proxies
sea
surface
temperature
(SST)
being
most
environmental
predictors.
A
positive
nonlinear
found,
weaker
sensitivity
at
high
concentrations.
This
found
be
dependent
other
model:
Nd–LWP
higher
precipitating
clouds
decreases
increasing
SSTs.
Atmospheric measurement techniques,
Journal Year:
2022,
Volume and Issue:
15(21), P. 6329 - 6371
Published: Nov. 3, 2022
Abstract.
Data
are
presented
from
intercomparisons
between
two
research
aircraft,
the
FAAM
BAe-146
and
NASA
Lockheed
P3,
surface-based
DOE
(Department
of
Energy)
ARM
(Atmospheric
Radiation
Measurement)
Mobile
Facility
at
Ascension
Island
(8∘
S,
14.5∘
W;
a
remote
island
in
mid-Atlantic).
These
took
place
17
August
to
5
September
2017,
during
African
biomass
burning
(BB)
season.
The
primary
motivation
was
give
confidence
use
data
multiple
platforms
with
which
evaluate
numerical
climate
models.
three
were
involved
CLouds–Aerosol–Radiation
Interaction
Forcing
for
Year
2017
(CLARIFY-2017),
ObseRvations
Aerosols
above
CLouds
their
intEractionS
(ORACLES),
Layered
Atlantic
Smoke
Interactions
Clouds
(LASIC)
field
experiments.
Comparisons
flight
segments
on
6
d
where
flew
alongside
facility
presented,
along
comparisons
wing-tip-to-wing-tip
P3
18
2017.
intercomparison
sampled
relatively
clean
atmosphere
overlying
moderately
polluted
boundary
layer,
while
six
fly-bys
site
both
conditions
2–4
km
upwind.
We
compare
validate
characterisations
aerosol
physical,
chemical
optical
properties
as
well
atmospheric
radiation
cloud
microphysics
platforms.
assess
performance
measurement
instrumentation
field,
under
sampling
not
tightly
controlled
laboratory
measurements
calibrations
performed.
Solar
compared
enough
permit
radiative
closure
studies.
Optical
absorption
coefficient
all
within
uncertainty
limits,
although
absolute
magnitudes
too
low
(<10
Mm−1)
fully
support
comparison
Ångström
exponents.
Aerosol
airborne
more
comparable
than
aircraft-to-ground
observations.
Scattering
observations
adequately
platforms,
but
agreement
ground-based
worse,
potentially
caused
by
small
differences
or
actual
population
over
land.
Chemical
composition
followed
similar
pattern,
better
Thermodynamics,
microphysical
generally
agreed
given
uncertainties.
Atmospheric Science Letters,
Journal Year:
2024,
Volume and Issue:
25(5)
Published: Jan. 11, 2024
Abstract
Aerosols
significantly
affect
cloud
microphysics
and
energy
budget
in
different
ways.
The
contribution
of
the
direct,
semi‐direct,
indirect
effects
aerosols
on
radiation
are
here
investigated
over
North
Atlantic
tropical
ocean
under
aerosol
loadings.
Weather
Research
Forecasting
Model
is
used
to
perform
a
set
numerical
idealized
experiments,
which
forced
with
prescribed
profiles.
We
evaluate
modeled
shallow
clouds
surface
radiative
budget.
results
indicate
that
large
loadings
associated
enhanced
cloudiness
reduced
precipitation.
While
change
rainfall
mainly
due
larger
number
smaller
droplets,
attributed
absorbing
aerosols,
dust
particles,
responsible
for
rise
temperature
feeds
back
onto
specific
humidity.
As
boundary
layer
increase
moisture
dominates,
net
effect
higher
relative
humidity,
favors
formation
thin
low
non‐precipitating
clouds.
feedback
accounts
dynamical
lower
troposphere:
shortwave
absorption
increases
at
top
marine
atmospheric
boundary‐layer
reduces
entrainment
warm
dry
air,
increasing
level
content.
Despite
overall
cloudiness,
daytime
cover
reduced.
semi‐direct
warming
surface,
opposite
effect.
Atmospheric chemistry and physics,
Journal Year:
2022,
Volume and Issue:
22(19), P. 12923 - 12943
Published: Oct. 7, 2022
Abstract.
In
situ
cloud
probe
data
from
the
NASA
ObseRvations
of
Aerosols
above
CLouds
and
their
intEractionS
(ORACLES)
field
campaign
were
used
to
estimate
effective
radius
(Re),
optical
thickness
(τ),
droplet
concentration
(Nc)
for
marine
stratocumulus
over
southeast
Atlantic
Ocean.
The
in
Re,
τ,
Nc
compared
with
co-located
Moderate
Resolution
Imaging
Spectroradiometer
(MODIS)
retrievals
Re
τ
MODIS-derived
Nc.
For
145
profiles,
a
MODIS
retrieval
was
time
gap
less
than
1
h.
On
average,
(11.3
µm
11.7)
1.6
2.3
higher
Pearson's
correlation
coefficients
(R)
0.77
0.73,
respectively.
average
(151.5
cm−3)
within
cm−3
an
R
0.90.
profiles
classified
into
67
contact
where
aerosol
(Na)
greater
500
sampled
100
m
tops
78
separated
Na
up
tops.
Contact
had
(by
88
cm−3),
2.5),
lower
2.2
µm)
profiles.
These
differences
associated
aerosol–cloud
interactions
(ACI),
estimates
5
cm−3,
0.5,
0.2
when
Re>15
or
τ>25
removed.
agreement
between
changes
ACI
driven
by
small
biases
properties
relative
measurements
across
different
regimes.
Thus,
combined
location
concentration,
can
be
study
larger
domains
longer
timescales
possible
using
data.
Scientific Data,
Journal Year:
2023,
Volume and Issue:
10(1)
Published: July 20, 2023
Abstract
In-situ
marine
cloud
droplet
number
concentrations
(CDNCs),
condensation
nuclei
(CCN),
and
CCN
proxies,
based
on
particle
sizes
optical
properties,
are
accumulated
from
seven
field
campaigns:
ACTIVATE;
NAAMES;
CAMP
2
EX;
ORACLES;
SOCRATES;
MARCUS;
CAPRICORN2.
Each
campaign
involves
aircraft
measurements,
ship-based
or
both.
Measurements
collected
over
the
North
Central
Atlantic,
Indo-Pacific,
Southern
Oceans,
represent
a
range
of
clean
to
polluted
conditions
in
various
climate
regimes.
With
extensive
environmental
sampled,
this
data
collection
is
ideal
for
testing
satellite
remote
detection
methods
CDNC
environments.
Remote
measurement
vital
expanding
available
these
difficult-to-reach
regions
Earth
improving
our
understanding
aerosol-cloud
interactions.
The
includes
composition
continental
tracers
identify
potential
contributing
sources.
Several
campaigns
include
High
Spectral
Resolution
Lidar
(HSRL)
polarimetric
imaging
measurements
retrievals
that
will
be
basis
next
generation
space-based
sensors
and,
thus,
can
utilized
as
surrogates.
Atmospheric chemistry and physics,
Journal Year:
2024,
Volume and Issue:
24(18), P. 10323 - 10347
Published: Sept. 18, 2024
Abstract.
The
aerosol–cloud–precipitation
interactions
within
the
cloud-topped
marine
boundary
layer
(MBL)
are
examined
using
aircraft
in
situ
measurements
from
Aerosol
and
Cloud
Experiments
Eastern
North
Atlantic
(ACE-ENA)
Southern
Ocean
Clouds,
Radiation,
Transport
Experimental
Study
(SOCRATES)
field
campaigns.
SOCRATES
clouds
exhibit
a
larger
number
concentration
smaller
cloud
droplet
effective
radius
(148.3
cm−3
8.0
µm)
compared
to
ACE-ENA
summertime
(89.4
9.0
wintertime
(70.6
9.8
µm).
clouds,
especially
during
winter,
feature
stronger
drizzle
formation
via
growth
through
enhanced
collision–coalescence
that
is
attributed
relatively
cleaner
environment
deeper
layer.
Furthermore,
aerosol–cloud
interaction
(ACI)
indices
two
campaigns
distinct
sensitivities,
indicating
different
microphysical
responses
aerosols.
winter
season
features
fewer
aerosols,
which
more
likely
activated
into
droplets
under
conditions
of
sufficient
water
vapor
availability
strong
turbulence.
enriched
aerosol
loading
summer
generally
leads
competing
for
limited
exhibiting
ACI.
Notably,
precipitation
susceptibilities
than
in-cloud
behavior
significantly
alters
sub-cloud
condensation
nuclei
(CCN)
budgets
coalescence-scavenging
effect
and,
turn,
impacts
ACI
assessments.
results
this
study
can
enhance
understanding
aid
future
model
simulation
assessment
interaction.