Polyphenol‐Mediated Multifunctional Human–Machine Interface Hydrogel Electrodes in Bioelectronics DOI Creative Commons
Lili Jiang, Donglin Gan, C. J. Xu

et al.

Small Science, Journal Year: 2024, Volume and Issue: 5(1)

Published: Nov. 21, 2024

Human-machine interface (HMI) electrodes enable interactions between humans and bioelectronic devices by facilitating electrical stimulation recording neural activity. However, reconciling the soft, hydrated nature of living human tissues with rigid, dry properties synthetic electronic systems is inherently challenging. Overcoming these significant differences, which critical for developing compatible, effective, stable interfaces, has become a key research area in materials science technology. Recently, hydrogels have gained prominence use HMI because are similar to can be tuned through incorporation nanofillers. This review examines functional requirements highlights recent progress development polyphenol-mediated multifunctional hydrogel-based bioelectronics. Furthermore, aspects such as mussel-inspired adhesion, underlying mechanisms, tissue-matching mechanical properties, electrochemical performance, biocompatibility, biofouling resistance, stability under physiological conditions, anti-inflammatory, antioxidant discussed. Finally, applications bioelectronics further perspectives outlined. Advances hydrogel expected facilitate unprecedented integration biological devices, potentially revolutionizing various biomedical fields enhancing capabilities performance devices.

Language: Английский

Transparent cellulose-lignin films containing Fe3+ with high UV absorption for thermal management DOI

Xin Fu,

Jianmin Peng, Xueren Qian

et al.

International Journal of Biological Macromolecules, Journal Year: 2025, Volume and Issue: 294, P. 139475 - 139475

Published: Jan. 5, 2025

Language: Английский

Citations

1
Thermally Responsive Hydroxypropyl Cellulose/Polyacrylamide Hydrogel with Programmable and Reversible Adhesion DOI
Yumin Wang,

Lide Xu,

Xiao Miao

et al.

ACS Applied Polymer Materials, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 6, 2025

The development of adhesives with switchable and programmable adhesion in both air water environments is highly desirable but still difficult to realize. Here, we have developed a smart hydrogel reversible behavior under thermal stimuli by introducing thermally responsive hydroxypropyl cellulose (HPC) polymer unit into the network. By alternately lowering raising temperature hydrogel, transition from sticky nonsticky state was achieved environments, wide switching range between high low adhesion, fast speed, durable efficiency. Accurate fine control dry wet strength can also be changing hydrogel. In addition performance, surface wettability, mechanical properties, optical transmission adapt programmed switched response change. exploiting its capacity, demonstrated as gripper for controllable capture release objects underwater environments. This study opens path design adhesives, materials, devices.

Language: Английский

Citations

0
In Situ Formation of Ion‐Clusters on Liquid Metals Surface for Simultaneously Improving Adhesive Toughness and Conductivity Toward Epidermal Electrodes DOI
Xinyu Chen, Yubing Fu, Xueling Yan

et al.

Advanced Functional Materials, Journal Year: 2025, Volume and Issue: unknown

Published: April 1, 2025

Abstract Developing epidermal electrodes that possess mechanic softness, tough adhesion, and high conductivity simultaneously is important but still remains challenging. Here, polyvinylpyrrolidone (PVP) introduced into poly(α‐thioctic acid) (PTA) to in situ generate ion‐clusters both PTA network on liquid metal particles (LMPs) surface, enhancing the mechanical strength toughness of PTA, as well its interfacial interaction with LMPs. As a result, poly(TA‐PVP)‐LMPs (noted PTPL) electrode reported softness (Young's modulus 175.86 kPa), adhesion (1604 J m −2 ), stretchability (>20 000%), rapid self‐healing, good biocompatibility. And attributed peel sintering LMPs, PTPL further exhibit electrical (26.19 mΩ sq −1 ) low skin impedance, providing signal‐to‐noise ratios (SNR 28.07 dB) accuracy monitoring multiple human electrophysiological signals. This work provides new strategy for balancing self‐adhesion, polymer materials fabrication.

Language: Английский

Citations

0
C-lignin-enabled multifunctional hydrogels for flexible wearable sensors DOI

Qingru Shen,

Meizhen Xie,

Shuizhong Wang

et al.

International Journal of Biological Macromolecules, Journal Year: 2025, Volume and Issue: 309, P. 142903 - 142903

Published: April 8, 2025

Language: Английский

Citations

0
Polyphenol‐Mediated Multifunctional Human–Machine Interface Hydrogel Electrodes in Bioelectronics DOI Creative Commons
Lili Jiang, Donglin Gan, C. J. Xu

et al.

Small Science, Journal Year: 2024, Volume and Issue: 5(1)

Published: Nov. 21, 2024

Human-machine interface (HMI) electrodes enable interactions between humans and bioelectronic devices by facilitating electrical stimulation recording neural activity. However, reconciling the soft, hydrated nature of living human tissues with rigid, dry properties synthetic electronic systems is inherently challenging. Overcoming these significant differences, which critical for developing compatible, effective, stable interfaces, has become a key research area in materials science technology. Recently, hydrogels have gained prominence use HMI because are similar to can be tuned through incorporation nanofillers. This review examines functional requirements highlights recent progress development polyphenol-mediated multifunctional hydrogel-based bioelectronics. Furthermore, aspects such as mussel-inspired adhesion, underlying mechanisms, tissue-matching mechanical properties, electrochemical performance, biocompatibility, biofouling resistance, stability under physiological conditions, anti-inflammatory, antioxidant discussed. Finally, applications bioelectronics further perspectives outlined. Advances hydrogel expected facilitate unprecedented integration biological devices, potentially revolutionizing various biomedical fields enhancing capabilities performance devices.

Language: Английский

Citations

2