ACS Applied Materials & Interfaces,
Journal Year:
2023,
Volume and Issue:
15(3), P. 4549 - 4558
Published: Jan. 16, 2023
3D
printed
silicones
have
demonstrated
great
potential
in
diverse
areas
by
combining
the
advantageous
physiochemical
properties
of
with
unparalleled
design
freedom
additive
manufacturing.
However,
their
low-temperature
performance,
which
is
particular
importance
for
polar
and
space
applications,
has
not
been
addressed.
Herein,
a
silicone
foam
unprecedented
elasticity
presented,
featured
extraordinary
fatigue
resistance,
excellent
shape
recovery,
energy-absorbing
capability
down
to
low
temperature
−60
°C
after
extreme
compression
(an
intensive
load
over
66000
times
its
own
weight).
The
achieved
direct
writing
phenyl
silicone-based
pseudoplastic
ink
embedded
sodium
chloride
as
sacrificial
template.
During
water
immersion
process
create
pores
filaments,
unique
osmotic
pressure-driven
morphing
strategy
also
reported,
offers
an
attractive
alternative
traditional
4D
hydrogels
virtue
favorable
mechanical
robustness
material.
underlying
mechanisms
are
discussed
detail.
Nature Communications,
Journal Year:
2023,
Volume and Issue:
14(1)
Published: Feb. 14, 2023
The
growing
demand
for
complex
three-dimensional
(3D)
micro-/nanostructures
has
inspired
the
development
of
corresponding
manufacturing
techniques.
Among
these
techniques,
3D
fabrication
based
on
mechanically
guided
assembly
offers
advantages
broad
material
compatibility,
high
designability,
and
structural
reversibility
under
strain
but
is
not
applicable
nanoscale
device
printing
because
bottleneck
at
nanofabrication
design
technique.
Herein,
a
configuration-designable
suggested
through
robust
nanotransfer
methodology
substrate's
mechanical
characteristics.
Covalent
bonding-based
two-dimensional
allowing
nanostructure
elastomer
substrates
used
to
address
problems,
while
feasibility
configuration
modulation
characteristics
examined
using
analytical
calculations
numerical
simulations,
various
nanostructures.
printed
nanostructures
exhibit
strain-independent
electrical
properties
are
therefore
fabricate
stretchable
H2
NO2
sensors
with
performances
stable
external
strains
30%.
Advanced Functional Materials,
Journal Year:
2023,
Volume and Issue:
34(35)
Published: Nov. 15, 2023
Abstract
Freshwater
scarcity
has
become
a
critical
global
challenge
affecting
some
of
the
most
vulnerable
populations.
In
response,
significant
effort
focused
on
ways
to
increase
access
this
precious
resource.
Within
context
geographical,
cultural,
political,
and
technological
factors
governing
freshwater
availability,
atmospheric
water
harvesting
(AWH)
demonstrated
tremendous
promise
help
address
these
shortages.
Specifically,
mesh‐based
fog
harvesters
have
received
considerable
attention
for
their
passive
qualities
compared
with
energy‐dependent
siblings
(sorbents,
condensation,
etc.),
yet
specific
yield
(SY)
developed
only
modestly
in
recent
decades.
While
plant
animal
kingdom
provide
diverse
examples
collection,
science
remarkable
understanding
processes,
much
knowledge
be
translated
practically
at
scale.
This
is
partially
due
challenges
mass‐producing
complex
(often
micro‐scale)
structures
observed
nature.
Fortunately,
manufacturing
technology
catching
up
scientific
understanding,
especially
scale
mesh
design.
To
end,
review
begins
by
surveying
bioinspired
research
harvesting.
Afterward,
study
identifies
milestones
developing
meshes,
concluding
discussion
future
opportunities
connecting
bioinspiration
emerging
advanced
techniques.
Deleted Journal,
Journal Year:
2024,
Volume and Issue:
3(2), P. 200137 - 200137
Published: April 21, 2024
The
ability
of
organisms
to
adjust
environmental
changes
offers
valuable
insights
into
the
development
and
creation
innovative
smart
systems.
As
requirements
increase,
materials
change
their
shapes
has
become
a
broader
aim
beyond
original
capabilities.
In
contrast
conventional
manufacturing
methods,
additive
(AM)
skillfully
combines
precise
three-dimensional
structures
intricate
response
mechanisms
biological
with
materials.
This
combination
enables
production
bionic
programmable
features.
Trends
such
as
dynamic
modulation,
responsiveness
multiple
stimuli,
integration
functions
are
emerging
significant
in
structures.
review
first
presents
that
nature
designed
built
various
organisms,
highlighting
relationship
between
structural
characteristics
patterns
deformation.
then
discusses
how
developed
using
AM
techniques
respond
different
stimuli.
Additionally,
potential
uses
biomedicine,
intelligent
robotics,
origami
construction,
aerospace
discussed.
Finally,
challenges
future
prospects
for
examined
goal
offering
solutions
creating
next
generation
systems
through
interdisciplinary
research.
Advanced Functional Materials,
Journal Year:
2024,
Volume and Issue:
34(37)
Published: March 19, 2024
Abstract
Engineering
or
mimicking
living
materials
found
in
nature
has
the
potential
to
transform
use
of
materials.
Unlike
classic
synthetic
which
are
typically
optimized
for
static
properties,
economics,
and
recently
also
sustainability,
life
dynamic,
feedback‐controlled,
evolving,
adaptive.
Although
do
not
exhibit
such
complicated
functionalities,
researchers
increasingly
challenging
this
viewpoint
expanding
material
concepts
toward
dynamic
systems
inspired
by
selected
life‐like
functions.
Herein,
it
is
suggested
that
can
be
approached
from
two
perspectives:
through
engineering
biological
organisms
their
functions
provide
basis
new
materials,
producing
with
rudimentary
life‐inspired
Current
advances
discussed
perspectives
(i)
features
based
on
built‐in
memory
associative
learning,
(ii)
emergent
structures
self‐regulated
designs
using
non‐equilibrium
systems,
(iii)
interfacing
non‐living
form
cellular
community
control
growth
open
routes
fabrication.
Strategies
combining
(i)–(iii)
responses
applications
interactive
autonomous
devices,
helping
realize
next‐generation
sensors,
soft
robots,
external
over
bioproduction
self‐organizing
structural
Advanced Functional Materials,
Journal Year:
2025,
Volume and Issue:
unknown
Published: Feb. 26, 2025
Abstract
Auxetic
metamaterials
refer
to
materials
and
structures
with
extraordinary
deformation,
i.e.,
transverse
expansion
(contraction)
under
uniaxial
tension
(compression).
In
recent
decades,
a
very
wide
range
of
innovative
functional
performance
has
been
discovered
stemming
from
this
behavior.
This
desirable
exhibition
adaptivity,
programmability,
functionality
provides
great
potential
in
soft
intelligent
systems.
However,
thus
far,
the
mainstream
research
on
auxetic
focused
subjective
design,
monotonic
mechanical
properties,
passive
tunability.
review
thorough
overview
classical
properties
applications,
primary
objective
proposing
new
roadmap
auxetics
for
advances
interdisciplinary
field.
The
fundamental
works
are
categorized
different
configurations
mechanisms.
particular,
integration
shape
morphing,
actuation,
sensing,
multiphysical
response,
inverse
design
is
reviewed
detail.
To
accelerate
development
smart
structural
systems,
applications
generalized
into
robotics
(outside
body),
human–machine
interaction
(surrounding
healthcare
devices
(inside
body).
Finally,
several
significant
topics
emphasized
theory,
material
choice,
manufacturing
technique,
applications.
Biology,
Journal Year:
2023,
Volume and Issue:
12(5), P. 653 - 653
Published: April 26, 2023
Spinal
cord
injury
(SCI)
represents
a
significant
medical
challenge,
often
resulting
in
permanent
disability
and
severely
impacting
the
quality
of
life
for
affected
individuals.
Traditional
treatment
options
remain
limited,
underscoring
need
novel
therapeutic
approaches.
In
recent
years,
multipotent
mesenchymal
stem
cells
(MSCs)
have
emerged
as
promising
candidate
SCI
due
to
their
multifaceted
regenerative
capabilities.
This
comprehensive
review
synthesizes
current
understanding
molecular
mechanisms
underlying
MSC-mediated
tissue
repair
SCI.
Key
discussed
include
neuroprotection
through
secretion
growth
factors
cytokines,
promotion
neuronal
regeneration
via
MSC
differentiation
into
neural
cell
types,
angiogenesis
release
pro-angiogenic
factors,
immunomodulation
by
modulating
immune
activity,
axonal
driven
neurotrophic
glial
scar
reduction
modulation
extracellular
matrix
components.
Additionally,
examines
various
clinical
applications
MSCs
treatment,
such
direct
transplantation
injured
spinal
cord,
engineering
using
biomaterial
scaffolds
that
support
survival
integration,
innovative
cell-based
therapies
like
MSC-derived
exosomes,
which
possess
neuroprotective
properties.
As
field
progresses,
it
is
crucial
address
challenges
associated
with
MSC-based
therapies,
including
determining
optimal
sources,
intervention
timing,
delivery
methods,
well
developing
standardized
protocols
isolation,
expansion,
characterization.
Overcoming
these
will
facilitate
translation
preclinical
findings
practice,
providing
new
hope
improved
individuals
living
devastating
consequences
Advanced Functional Materials,
Journal Year:
2023,
Volume and Issue:
34(14)
Published: Dec. 24, 2023
Abstract
4D
printing
is
the
3D
of
objects
that
change
chemically
or
physically
in
response
to
an
external
stimulus
over
time.
Photothermally
responsive
shape
memory
materials
are
attractive
for
their
ability
undergo
remote
activation.
While
photothermal
methods
using
gold
nanorods
(AuNRs)
used
recovery,
patterning
these
into
with
complex
geometries
degradable
not
addressed.
Here,
fabrication
printed
bioplastics
photo‐activated
recovery
reported.
Protein‐based
nanocomposites
based
on
bovine
serum
albumin
(BSA),
poly
(ethylene
glycol)
diacrylate
(PEGDA),
and
AuNRs
developed
vat
photopolymerization.
These
mechanically
deformed
under
high
loads,
proteins
served
as
mechano‐active
elements
unfolded
energy‐dissipating
mechanism
prevented
fracture
thermoset.
The
bioplastic
object
maintained
its
metastable
shape‐programmed
state
ambient
conditions.
Subsequently,
up
99%
achieved
within
1
min
irradiation
near‐infrared
(NIR)
light.
Mechanical
characterization
small
angle
X‐ray
scattering
(SAXS)
analysis
suggest
unfold
during
programming
step
may
refold
recovery.
composites
promising
biodegradable
shape‐morphing
devices
robotics
medicine.
RSC Sustainability,
Journal Year:
2024,
Volume and Issue:
2(6), P. 1708 - 1737
Published: Jan. 1, 2024
Chemical
modifications
of
vegetable
oil
and
their
3D
printing
applications
are
discussed.
Acrylate
resin
compatibility
with
methods
presented.
printed
products
using
oil-derived
materials,
providing
insights
into
future
opportunities
explored.
Proceedings of the National Academy of Sciences,
Journal Year:
2023,
Volume and Issue:
120(33)
Published: Aug. 7, 2023
Biocompatible
and
morphable
hydrogels
capable
of
multimode
reprogrammable,
adaptive
shape
changes
are
potentially
useful
for
diverse
biomedical
applications.
However,
existing
systems
often
rely
on
complicated
structural
designs
involving
cumbersome
energy-intensive
fabrication
processes.
Here,
we
report
a
simple
electric-field-activated
protein
network
migration
strategy
to
reversibly
program
silk-protein
with
controllable
reprogrammable
complex
transformations.
The
application
low
electric
field
enables
the
convergence
net
negatively
charged
cross-linking
networks
toward
anode
(isoelectric
point
plane)
due
pH
gradient
generated
in
process,
facilitating
formation
structure
suitable
three-dimensional
change.
These
tunable
can
be
reprogrammed
or
permanently
fixed
by
control
polymorphic
transitions.
We
show
that
these
morphing
conformally
interfacing
biological
tissues
programming
bimorph
consisting
aligned
carbon
nanotube
multilayers
silk
was
assembled
illustrate
utility
as
an
implantable
bioelectronic
device
localized
low-voltage
electrical
stimulation
sciatic
nerve
rabbit.