Advanced Functional Materials,
Journal Year:
2024,
Volume and Issue:
34(24)
Published: Feb. 20, 2024
Abstract
Intrinsically
flexible
photodetectors
are
compelling
building
blocks
for
next‐generation
wearable
optoelectronic
systems
owing
to
their
distinctive
advantages
of
reliable
structural
durability
and
versatile
scalability
large‐scale
production.
However,
practical
applications
still
impeded
by
the
inferior
photodetection
performance,
irreversible
device
failure
after
breakage,
serious
e‐waste
accumulation
service
life.
Herein,
a
high‐performance
intrinsically
flexible,
mechanically
durable,
self‐healable,
closed‐loop
recyclable,
screen‐printable
Te
NWs/MoS
2
nanosheets/polyimine
nanocomposite‐based
photodetector
designed
engineering‐ordered‐bridged
1D/2D
carrier
percolation
“fast
lanes”
in
dynamic
covalent
polyimine
matrix
via
flow‐designed
solution‐shearing
method.
Such
design
provides
sixfold,
20.1‐fold,
6.9‐fold
enhancement
mobility,
responsivity
(11.68
mA
W
−1
),
detectivity
(1.145
×
10
Jones),
respectively,
as
well
stable
photoresponse
over
eight
months
or
50
000
bending‐flattening
times.
Meanwhile,
this
presents
excellent
self‐healing
efficiency
repeatable
recyclability
reconfiguration.
Furthermore,
these
merits
can
be
fully
integrated
onto
textile
assembling
nacre‐like
/polyimine
nanocomposite
coatings
on
textiles
screen‐printing
processes,
enabling
programmable
patterning
arrays
large‐area
image
sensing.
This
work
viable
approach
shape‐tunable
optoelectronics
with
mechanical
customizable
functionalities,
demonstrating
tremendous
potential
systems.
Advanced Optical Materials,
Journal Year:
2024,
Volume and Issue:
12(27)
Published: July 15, 2024
Abstract
With
the
development
of
wearable
electronic
technology,
flexible
photodetectors
have
attracted
widespread
attention,
and
it
is
great
significance
to
develop
flexible,
eco‐friendly
low‐cost
photodetectors.
Cellulose
paper,
as
a
eco‐friendly,
low‐cost,
lightweight,
customizable,
biodegradable
renewable
material,
has
received
enthusiastic
attention
rapid
in
field
recent
years.
In
this
review,
focused
on
research
progress
paper‐based
(PB)
First,
fabrication
methods
PB
are
discussed,
including
electrode
materials
optoelectronic
functional
materials.
Then,
review
systematically
summarizes
analyzes
achievements
photoelectric
performances
(spectral
response
range,
responsivity,
detectivity,
response/recovery
times
on/off
ratio)
flexibility
characteristics
(bending
angle
bending
cycle).
terms
key
performance
indicators,
reported
so
far
can
detect
multiple
wavelengths
light
from
UV
near‐infrared
with
maximum
detectivity
10
13
Jones.
addition,
various
applications
reviewed
discussed.
Finally,
look
forward
future
methods,
performances,
applications.
hope
that
will
promoted
Advanced Materials,
Journal Year:
2024,
Volume and Issue:
36(33)
Published: June 20, 2024
Abstract
Xenes,
mono‐elemental
atomic
sheets,
exhibit
Dirac/Dirac‐like
quantum
behavior.
When
interfaced
with
other
2D
materials
such
as
boron
nitride,
transition
metal
dichalcogenides,
and
carbides/nitrides/carbonitrides,
it
enables
them
unique
physicochemical
properties,
including
structural
stability,
desirable
bandgap,
efficient
charge
carrier
injection,
flexibility/breaking
stress,
thermal
conductivity,
chemical
reactivity,
catalytic
efficiency,
molecular
adsorption,
wettability.
For
example,
BN
acts
an
anti‐oxidative
shield,
MoS
2
injects
electrons
upon
laser
excitation,
MXene
provides
mechanical
flexibility.
Beyond
precise
compositional
modulations,
stacking
sequences,
inter‐layer
coupling
controlled
by
parameters,
achieving
scalability
reproducibility
in
hybridization
is
crucial
for
implementing
these
consumer
applications.
However,
realizing
the
full
potential
of
hybrid
faces
challenges
air
gaps,
uneven
interfaces,
formation
defects
functional
groups.
Advanced
synthesis
techniques,
a
deep
understanding
behaviors,
control
over
interfacial
interactions,
awareness
cross‐correlations
among
factors
are
essential.
Xene‐based
hybrids
show
immense
promise
groundbreaking
applications
computing,
flexible
electronics,
energy
storage,
catalysis.
In
this
timely
perspective,
recent
discoveries
novel
Xenes
their
highlighted,
emphasizing
correlations
synthetic
structure,
It
anticipated
that
insights
will
revolutionize
diverse
industries
technologies.
Heliyon,
Journal Year:
2024,
Volume and Issue:
10(3), P. e24964 - e24964
Published: Jan. 26, 2024
2D
nanosheets
produced
using
liquid
phase
exfoliation
method
offers
scalable
and
cost
effective
routes
to
optoelectronics
devices.
But
this
technique
sometimes
yields
high
defect,
low
stability,
compromised
electronic
properties.
In
work,
we
employed
an
innovative
approach
that
improved
the
existing
for
fabricating
MoS2/graphene
heterostructure-based
photodetector
with
enhanced
optoelectronic
This
involves
hydrothermally
treating
MoS2
before
dispersing
it
in
a
carefully
chosen
environmentally
friendly
IPA/water
solvent
ultrasonication
through
optomechanical
approach.
Thereafter,
heterostructure
of
graphene
were
formed
sequential
deposition
fabrication
vertical
heterojunctions.
Furthermore,
achieved
vertically
stacked
bare
photodetector.
The
hybrid
characterized
spectroscopic
microscopic
techniques.
results
obtained
show
size
is
between
350
500
nm
on
average,
their
thickness
less
than
or
equal
5
nm,
crystallinity
2H
semiconducting
phase.
photocurrent,
photoresponsivity,
external
quantum
efficiency
(EQE),
specific
detectivity
at
4
V
bias
voltage
650
illumination
wavelength
3.55
μA,
39.44
mA/W,
7.54
%,
2.02
×
1010
Jones,
respectively,
are
0.55
6.11
1.16
3.4
109
Jones.
presented
indicate
photoresponse
performances
as-prepared
greatly
(about
7-fold)
compared
sole
MoS2.
Again,
fabricated
work
better
characteristics
as
similar
prepared
conventional
solution
processed
method.
provide
modest,
inexpensive,
efficient
fabricate
heterojunctions
performance.
Sensors,
Journal Year:
2025,
Volume and Issue:
25(4), P. 1042 - 1042
Published: Feb. 10, 2025
With
the
rapid
development
of
micro-nano
technology
and
wearable
devices,
flexible
photodetectors
(PDs)
have
drawn
widespread
interest
in
areas
such
as
healthcare,
consumer
electronics,
intelligence
interfaces.
Two-dimensional
(2D)
materials
with
layered
structures
excellent
optoelectronic
properties
mechanical
flexibility,
which
attract
a
great
deal
attention
applications.
Although
based
on
mechanically
exfoliated
2D
demonstrated
superior
performance
compared
to
traditional
Si-based
PDs,
large-scale
manufacturing
integration
remain
significant
challenges
for
achieving
industrial
production.
The
emerging
various
printing
provides
low-cost
highly
effective
method
integrated
manufacturing.
In
this
review,
we
comprehensively
introduce
most
recent
progress
printed
material
PDs.
We
first
reviewed
research
photodetectors,
discussion
is
focused
substrate
materials,
functional
figures
merits.
Furthermore,
solution
processing
coupled
film
strategies
produce
PDs
are
summarized.
Subsequently,
applications
image
sensors,
also
Finally,
point
out
potential
expect
work
inspire
promote
mass
process.
Advanced Materials,
Journal Year:
2023,
Volume and Issue:
35(38)
Published: June 8, 2023
With
molecularly
well-defined
and
tailorable
2D
structures,
covalent
organic
frameworks
(COFs)
have
emerged
as
leading
material
candidates
for
chemical
sensing,
storage,
separation,
catalysis.
In
these
contexts,
the
ability
to
directly
deterministically
print
COFs
into
arbitrary
geometries
will
enable
rapid
optimization
deployment.
However,
previous
attempts
been
restricted
by
low
spatial
resolution
and/or
post-deposition
polymerization
that
limits
range
of
compatible
COFs.
Here,
limitations
are
overcome
with
a
pre-synthesized,
solution-processable
colloidal
ink
enables
aerosol
jet
printing
micron-scale
resolution.
The
formulation
utilizes
low-volatility
solvent
benzonitrile,
which
is
critical
obtaining
homogeneous
printed
COF
film
morphologies.
This
also
other
nanomaterials,
thus
facilitating
integration
printable
nanocomposite
films.
As
proof-of-concept,
boronate-ester
integrated
carbon
nanotubes
(CNTs)
form
COF-CNT
films,
in
CNTs
enhance
charge
transport
temperature
sensing
performance,
ultimately
resulting
high-sensitivity
sensors
show
electrical
conductivity
variation
4
orders
magnitude
between
room
300
°C.
Overall,
this
work
establishes
flexible
platform
additive
manufacturing
accelerate
incorporation
technologically
significant
applications.
Small Methods,
Journal Year:
2024,
Volume and Issue:
unknown
Published: June 6, 2024
Abstract
To
simulate
biological
visual
systems
and
surpass
their
functions
performance,
it
is
essential
to
develop
high‐performance
optoelectronic
neuromorphic
electronics
with
broadband
response,
low
power
consumption,
fast
response
speed.
Among
these,
synaptic
transistors
have
emerged
as
promising
candidates
for
constructing
systems.
In
this
work,
flexible
printed
(from
275
1050
nm)
carbon
nanotube
good
stability,
high
speed
(3.14
ms),
low‐power
consumption
(as
0.1
fJ
per
event
the
nm
pulse
illumination)
using
PbS
quantum
dots
(QDs)
modified
semiconducting
single‐walled
nanotubes
(sc‐SWCNTs)
active
layers
are
developed.
optical
pulses
within
ultraviolet
near‐infrared
wavelength
range,
devices
exhibit
excitatory
postsynaptic
current,
paired‐pulse
facilitation,
a
transition
from
short‐term
plasticity
long‐term
plasticity,
other
behaviors.
Furthermore,
simplified
neural
morphology
array
developed
integrated
such
image
perception,
memory,
preprocessing.
More
importantly,
can
also
emulate
complicated
bionic
functions,
infrared
perception
of
salmon
eyes
warning
behavior
reindeer
in
different
environments.
This
work
holds
immense
significance
advancing
development
artificial
Small,
Journal Year:
2024,
Volume and Issue:
unknown
Published: July 19, 2024
Abstract
With
the
rapid
development
of
micro/nano
machining,
there
is
an
elevated
demand
for
high‐performance
microdevices
with
high
reliability
and
low
cost.
Due
to
their
outstanding
electrochemical,
optical,
electrical,
mechanical
performance,
carbon
materials
are
extensively
utilized
in
constructing
energy
storage,
sensing,
optoelectronics.
Carbon
machining
fundamental
carbon‐based
intelligent
microelectronics,
multifunctional
integrated
microsystems,
high‐reliability
portable/wearable
consumer
electronics,
portable
medical
diagnostic
systems.
Despite
numerous
reviews
on
materials,
a
comprehensive
overview
lacking
that
systematically
encapsulates
based
structures,
from
structural
design
manufacturing
strategies
specific
applications.
This
review
focuses
latest
progress
toward
miniaturized
device,
including
engineering,
large‐scale
fabrication,
performance
optimization.
Especially,
targets
in‐depth
evaluation
micro
storage
devices,
microsensors,
microactuators,
photoresponsive
electromagnetic
interference
shielding
devices.
Moreover,
it
highlights
challenges
opportunities
microdevices,
aiming
spark
further
exciting
research
directions
application
prospectives.
Sensors & Diagnostics,
Journal Year:
2024,
Volume and Issue:
3(9), P. 1406 - 1427
Published: Jan. 1, 2024
Non-contact,
maskless,
direct
writing
methods
allow
the
rapid,
large-scale
production
of
graphene
electrodes
with
high
design
flexibility,
showing
great
promise
for
point-of-care
electrochemical
sensing
applications.