Shear-Induced Fabrication of Cellulose Nanofibril/Liquid Metal Nanocomposite Films for Flexible Electromagnetic Interference Shielding and Thermal Management DOI

Ning Ren,

Yusen Ai,

Yue Ning

et al.

ACS Applied Materials & Interfaces, Journal Year: 2024, Volume and Issue: 16(14), P. 17904 - 17917

Published: March 21, 2024

To address electromagnetic interference (EMI) pollution in modern society, the development of ultrathin, high-performance, and highly stable EMI shielding materials is desired. Liquid metal (LM) based conductive have received enormous amounts attention. However, processing approach LM/polymer composites represents great challenges due to high surface tension cohesive energy LMs. In this study, we develop a universal one-step fabrication strategy directly process containing LMs cellulose nanofibrils (CNFs) successfully fabricate flexible, films with an average specific efficiency (EMI SE) value 429 dB/mm small thickness only 70 μm wide frequency range 8.2–18 GHz. addition, resulting also exhibit excellent mechanical performance flexibility, which endow film ability withstand repeated folding, bending, folding into complex shapes without producing cracks or fractures. Besides, display thermal conductivity λ 4.90 W/(m K) α 3.17 mm2/s. Thus, presented shows potential fabricating advanced for applications.

Language: Английский

Gallium Liquid Metal: Nanotoolbox for Antimicrobial Applications DOI
Vi Khanh Truong, Andrew Hayles, Richard Bright

et al.

ACS Nano, Journal Year: 2023, Volume and Issue: 17(15), P. 14406 - 14423

Published: July 28, 2023

The proliferation of drug resistance in microbial pathogens poses a significant threat to human health. Hence, treatment measures are essential surmount this growing problem. In context, liquid metal nanoparticles promising. Gallium, post-transition notable for being at physiological temperature, has drawn attention its distinctive properties, high antimicrobial efficacy, and low toxicity. Moreover, gallium demonstrate anti-inflammatory properties immune cells. Gallium can alloy with other metals be prepared various composites modify tailor characteristics functionality. More importantly, the bactericidal mechanism could sidestep emerging mechanisms. Building on rationale, gallium-based enable impactful innovative strategic pathways battle against resistance. This review outlines nanoscale their corresponding mechanisms provide comprehensive yet succinct overview current applications. addition, challenges opportunities that require further research efforts have been identified discussed.

Language: Английский

Citations

67

3D Printing of Liquid‐Metal‐in‐Ceramic Metamaterials for High‐Efficient Microwave Absorption DOI
Ruizhe Xing,

G. Xu,

Ning Qu

et al.

Advanced Functional Materials, Journal Year: 2023, Volume and Issue: 34(31)

Published: Sept. 8, 2023

Abstract This work reports a gallium indium alloy (EGaIn)‐doped SiBOC ceramic that possesses unique liquid‐metal‐in‐ceramic feature. The low‐viscosity liquid nature of gallium‐based metals (Ga‐LMs) and the reactive core‐shell structure provide possibilities for phase engineering inside polymer‐derived ceramics. As demonstration, EGaIn nanoparticles (NPs) are directly mixed with UV‐curable precursor (UV‐PBS) to obtain resin suitable digital light processing 3D‐printing. After pyrolysis at 800–1200 °C, ceramics uniformly distributed NP domains (Si(GaIn)BOC) obtained. plays key role in promoting carbonization preventing crack formation during polymer‐to‐ceramic process, resulting an increase both yield mechanical strength. NPs also found have (EGaIn@(GaxIn1‐ x )2O3@SiBOC) matrix, which significantly enhances dielectric properties improves interfacial polarization. result, excellent electromagnetic wave absorption performance is achieved across C, X, Ku bands, respectively. Through rational design, novel metastructure design based on Schwarz P minimal surface proposed, exhibits ultrawide effective band extending up 11.36 GHz (within C‐Ku bands).

Language: Английский

Citations

53

Permeable, three-dimensional integrated electronic skins with stretchable hybrid liquid metal solders DOI
Qiuna Zhuang, Kuanming Yao, Chi Zhang

et al.

Nature Electronics, Journal Year: 2024, Volume and Issue: 7(7), P. 598 - 609

Published: July 1, 2024

Language: Английский

Citations

47

Lignocellulose‐Mediated Functionalization of Liquid Metals toward the Frontiers of Multifunctional Materials DOI Open Access

Wei Li,

Liyu Zhu,

Ying Xu

et al.

Advanced Materials, Journal Year: 2024, Volume and Issue: unknown

Published: Nov. 21, 2024

Lignocellulose-mediated liquid metal (LM) composites, as emerging functional materials, show tremendous potential for a variety of applications. The abundant hydroxyl, carboxyl, and other polar groups in lignocellulose facilitate the formation strong chemical bonds with LM surfaces, enhancing wettability adhesion improved interface compatibility. Beyond serving supportive matrix, can be tailored to optimize microstructure adapting them diverse This review comprehensively summarizes fundamental principles recent advancements lignocellulose-mediated highlighting advantages composite fabrication, including facile synthesis, versatile interactions, inherent functionalities. Key modulation strategies LMs innovative synthesis methods functionalized composites are discussed. Furthermore, roles structure-performance relationships these electromagnetic shielding, flexible sensors, energy storage devices systematically summarized. Finally, obstacles prospective pertaining thoroughly scrutinized deliberated upon. is expected provide basic guidance researchers boost popularity applications useful references design state-of-the-art LMs.

Language: Английский

Citations

33

Malleable, printable, bondable, and highly conductive MXene/liquid metal plasticine with improved wettability DOI Creative Commons
Haojie Jiang, Bin Yuan,

Hongtao Guo

et al.

Nature Communications, Journal Year: 2024, Volume and Issue: 15(1)

Published: July 20, 2024

Integration of functional fillers into liquid metals (LM) induces rheology modification, enabling the free-form shaping LM at micrometer scale. However, integrating non-chemically modified low-dimensional materials with to form stable and uniform dispersions remain a great challenge. Herein, we propose solvent-assisted dispersion (SAD) method that utilizes fragmentation reintegration in volatile solvents engulf disperse fillers. This successfully integrates MXene uniformly LM, achieving better internal connectivity than conventional dry powder mixing (DPM) method. Consequently, MXene/LM (MLM) coating exhibits high electromagnetic interference (EMI) shielding performance (105 dB 20 μm, which is 1.6 times coatings prepared by DPM). Moreover, rheological characteristic MLM render it malleable facilitates direct printing adaptation diverse structures. study offers convenient for assembling materials, paving way development multifunctional soft devices.

Language: Английский

Citations

31

Flexible solid-liquid bi-continuous electrically and thermally conductive nanocomposite for electromagnetic interference shielding and heat dissipation DOI Creative Commons
Yue Sun, Yunting Su,

Ziyuan Chai

et al.

Nature Communications, Journal Year: 2024, Volume and Issue: 15(1)

Published: Sept. 6, 2024

Language: Английский

Citations

28

4D printing roadmap DOI Creative Commons
Mahdi Bodaghi, Linlin Wang, Fenghua Zhang

et al.

Smart Materials and Structures, Journal Year: 2024, Volume and Issue: 33(11), P. 113501 - 113501

Published: June 26, 2024

Abstract Four-dimensional (4D) printing is an advanced manufacturing technology that has rapidly emerged as a transformative tool with the capacity to reshape various research domains and industries. Distinguished by its integration of time dimension, 4D allows objects dynamically respond external stimuli, setting it apart from conventional 3D printing. This roadmap been devised, contributions 44 active researchers in this field 32 affiliations world-wide, navigate swiftly evolving landscape printing, consolidating recent advancements making them accessible experts across diverse fields, ranging biomedicine aerospace, textiles electronics. The roadmap’s goal empower both enthusiasts, facilitating exploitation printing’s potential create intelligent, adaptive are not only feasible but readily attainable. By addressing current future challenges proposing science technology, sets stage for revolutionary progress numerous industries, positioning future.

Language: Английский

Citations

27

Fibres—threads of intelligence—enable a new generation of wearable systems DOI
Chao Dang, Zhixun Wang, Theodore Hughes‐Riley

et al.

Chemical Society Reviews, Journal Year: 2024, Volume and Issue: 53(17), P. 8790 - 8846

Published: Jan. 1, 2024

Fabrics represent a unique platform for seamlessly integrating electronics into everyday experiences. The advancements in functionalizing fabrics at both the single fibre level and within constructed have fundamentally altered their utility. revolution materials, structures, functionality enables intimate imperceptible integration, rapidly transforming fibres next-generation wearable devices systems. In this review, we explore recent scientific technological breakthroughs smart fibre-enabled fabrics. We examine common challenges bottlenecks physics, chemistry, fabrication strategies, applications that shape future of electronics. propose closed-loop fabric ecosystem encompassing proactive sensing, interactive communication, data storage processing, real-time feedback, energy harvesting, intended to tackle significant technology. Finally, envision computing as sophisticated platforms with system-level attributes management, machine learning, artificial intelligence, intelligent networks.

Language: Английский

Citations

25

Magnetically driven formation of 3D freestanding soft bioscaffolds DOI Creative Commons
Ruoxiao Xie, Yuanxiong Cao, Rujie Sun

et al.

Science Advances, Journal Year: 2024, Volume and Issue: 10(5)

Published: Feb. 2, 2024

3D soft bioscaffolds have great promise in tissue engineering, biohybrid robotics, and organ-on-a-chip engineering applications. Though emerging three-dimensional (3D) printing techniques offer versatility for assembling biomaterials, challenges persist overcoming the deformation or collapse of delicate structures during fabrication, especially overhanging thin features. This study introduces a magnet-assisted fabrication strategy that uses magnetic field to trigger shape morphing provide remote temporary support, enabling straightforward creation with overhangs thin-walled 3D. We demonstrate effectiveness our through replicate complex topology branching vascular systems. Furthermore, we engineered hydrogel-based support actuators capable walking motion triggered by cardiomyocytes. approach opens new possibilities shaping hydrogel materials into morphologies, which will further empower broad range biomedical

Language: Английский

Citations

21

Interfacial engineering of liquid metal nanoparticles for the fabrication of conductive hydrogels: A review DOI
Yanbo Zhao, Kai Zhao,

Rong Qian

et al.

Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: 486, P. 150197 - 150197

Published: March 6, 2024

Language: Английский

Citations

21