Design of an injectable, self-adhesive, and highly stable hydrogel electrode for sleep recording DOI Creative Commons
Ju-Chun Hsieh,

Weilong He,

Dhivya Venkatraghavan

et al.

Device, Journal Year: 2023, Volume and Issue: 2(2), P. 100182 - 100182

Published: Dec. 5, 2023

High-quality and continuous electroencephalogram (EEG) monitoring is desirable for sleep research, monitoring, the evaluation treatment of disorders. Existing EEG technologies suffer from fragile connections, long-term stability, complex preparation electrodes under real-life conditions. Here, we report an injectable spontaneously cross-linked hydrogel electrode applications. Specifically, our have a low impedance on hairy scalp regions 17.53 kΩ more than 8 h recording, high adhesiveness skin 0.92 N cm

Language: Английский

Bioinspired polydopamine hydrogels: Strategies and applications DOI
Yuanting Xu, Junfei Hu, Jingjing Hu

et al.

Progress in Polymer Science, Journal Year: 2023, Volume and Issue: 146, P. 101740 - 101740

Published: Sept. 17, 2023

Language: Английский

Citations

110

Photoswitchable and Reversible Fluorescent Eutectogels for Conformal Information Encryption DOI
Changchun Li, Jize Liu, Xiaoyan Qiu

et al.

Angewandte Chemie International Edition, Journal Year: 2023, Volume and Issue: 62(46)

Published: Oct. 4, 2023

Smart fluorescent materials that can respond to environmental stimuli are of great importance in the fields information encryption and anti-counterfeiting. However, traditional usually face problems such as lack tunable fluorescence insufficient surface-adaptive adhesion, hindering their practical applications. Herein, inspired by glowing sucker octopus, we present a novel strategy fabricate reversible eutectogel with high transparency, adhesive self-healing performance for conformal Using anthracene luminescent unit, exhibits photoswitchable therefore be reversibly written/erased patterns non-contact stimulation. Additionally, different from mechanically irreversible adhesion via glue, adhere various irregular substrates over wide temperature range (-20 65 °C) conformally deform more than 1000 times without peeling off. Furthermore, exploiting transparency good stretchability eutectogel, dual achieved under UV stretching conditions further improve security level. This study should provide promising future development advanced intelligent anti-counterfeiting materials.

Language: Английский

Citations

87

Flexible Conformally Bioadhesive MXene Hydrogel Electronics for Machine Learning‐Facilitated Human‐Interactive Sensing DOI
Wei Wang,

Hailiang Zhou,

Zhishan Xu

et al.

Advanced Materials, Journal Year: 2024, Volume and Issue: 36(31)

Published: March 29, 2024

Wearable epidermic electronics assembled from conductive hydrogels are attracting various research attention for their seamless integration with human body conformally real-time health monitoring, clinical diagnostics and medical treatment, human-interactive sensing. Nevertheless, it remains a tremendous challenge to simultaneously achieve bioadhesive remarkable self-adhesiveness, reliable ultraviolet (UV) protection ability, admirable sensing performance high-fidelity epidermal electrophysiological signals along timely photothermal therapeutic performances after diagnostic sensing, as well efficient antibacterial activity hemostatic effect potential therapy. Herein, hydrogel-based sensor, featuring superior self-adhesiveness excellent UV-protection performance, is developed by dexterously assembling conducting MXene nanosheets network biological hydrogel polymer stably attaching onto skin high-quality recording of high signal-to-noise ratios (SNR) low interfacial impedance intelligent diagnosis smart human-machine interface. Moreover, sign language gesture recognition platform based on collected electromyogram (EMG) designed hassle-free communication hearing-impaired people the help advanced machine learning algorithms. Meanwhile, possesses capability, biocompatibility, effective hemostasis properties promising bacterial-infected wound bleeding.

Language: Английский

Citations

68

Solvent‐Free and Skin‐Like Supramolecular Ion‐Conductive Elastomers with Versatile Processability for Multifunctional Ionic Tattoos and On‐Skin Bioelectronics DOI Open Access

Wenwen Niu,

Qiong Tian, Zhiyuan Liu

et al.

Advanced Materials, Journal Year: 2023, Volume and Issue: 35(39)

Published: June 24, 2023

The development of stable and biocompatible soft ionic conductors, alternatives to hydrogels ionogels, will open up new avenues for the construction stretchable electronics. Here, a brand-new design, encapsulating naturally occurring ionizable compound by polymer via high-density hydrogen bonds, resulting in solvent-free supramolecular ion-conductive elastomer (SF-supra-ICE) that eliminates dehydration problem possesses excellent biocompatibility, is reported. SF-supra-ICE with high conductivity (>3.3 × 10-2 S m-1 ) exhibits skin-like softness strain-stiffening behaviors, elasticity, breathability, self-adhesiveness. Importantly, can be obtained simple water evaporation step solidify aqueous precursor into nature. Therefore, act as inks painted printed customized tattoos (I-tattoos) multifunctional on-skin bioelectronics. I-tattoos exhibit ultraconformal seamless contact human skin, enabling long-term high-fidelity recording various electrophysiological signals extraordinary immunity motion artifacts. Human-machine interactions are achieved exploiting transmit beings. Stretchable I-tattoo electrode arrays, manufactured printing method, demonstrated multichannel digital diagnosis health condition back muscles spine.

Language: Английский

Citations

65

Conductive hydrogels for bioenergy harvesting and self-powered application DOI
Chenyang Zhang, Md Osman Goni Nayeem, Zhiqi Wang

et al.

Progress in Materials Science, Journal Year: 2023, Volume and Issue: 138, P. 101156 - 101156

Published: June 23, 2023

Language: Английский

Citations

57

Hydrogel sensors for biomedical electronics DOI
Jingyun Ma, Jiaqi Zhong,

Fuqin Sun

et al.

Chemical Engineering Journal, Journal Year: 2023, Volume and Issue: 481, P. 148317 - 148317

Published: Dec. 23, 2023

Language: Английский

Citations

48

Fully Polymeric Conductive Hydrogels with Low Hysteresis and High Toughness as Multi‐Responsive and Self‐Powered Wearable Sensors DOI
Weiyi Wang,

Pengshan Guo,

Xin Liu

et al.

Advanced Functional Materials, Journal Year: 2024, Volume and Issue: 34(32)

Published: April 22, 2024

Abstract High mechanical strength, excellent toughness, low hysteresis, and robust resilience are of great importance for stretchable conductive hydrogels (CHs) to heighten their reliabilities self‐powered sensing applications. However, it still remains challenging simultaneously obtain the mutually exclusive performances. Herein, an intrinsically adhesive hydrogel is fabricated by one‐step radical polymerization acrylamide (AAm), three hydroxy groups together clustered‐N‐[tris(hydroxymethyl)methyl]acrylamide (THMA), cationic 1‐Butyl‐3‐Vinylimidazolium Bromide (ILs) dissolved in core‐shell structurally dispersed PEDOT:PSS (PP) solution. Owing abundant clustered hydrogen bonds, electrostatic interactions between PILs chains anionic PSS shells, polymer chain entanglements, CHs feature superior properties with a high tensile strength (0.25 MPa), fracture strain (1015%), toughness (1.22 MJ m ‐3 ), energy 36.5 kJ ‐2 extremely hysteresis (5%), display fatigue resistance. As result, indicate gauge factor up 10.46, broad range (1‐900%) pressure (0.05‐100 kPa), fast responsive rate, thus qualifying monitoring reliably accurately large tiny human movements daily life. Moreover, hydrogel‐assembled triboelectric nanogenerators (TENGs) exhibit stable electrical output performances, which greatly promising flexible wearable electronics.

Language: Английский

Citations

47

Extended H-bonds/π-bonds networks for boosting electron transfer over polydopamine-covered nanocellulose/g-C3N4 toward efficient photocatalytic H2O2 production DOI
Tianshang Shan, Yu Wang, Dan Luo

et al.

Applied Catalysis B Environment and Energy, Journal Year: 2024, Volume and Issue: 349, P. 123872 - 123872

Published: April 24, 2024

Language: Английский

Citations

31

Polydopamine interface-modulated MXene-based conductive antibacterial hydrogels for on-skin health monitoring and diabetic wound healing DOI
Dandan Liu, Siwei Bi, Haibo Wang

et al.

Composites Part A Applied Science and Manufacturing, Journal Year: 2024, Volume and Issue: 180, P. 108065 - 108065

Published: Feb. 8, 2024

Language: Английский

Citations

19

Multifunctional Conductive Hydrogel Interface for Bioelectronic Recording and Stimulation DOI
Hao Tang, Yuanfang Li,

Shufei Liao

et al.

Advanced Healthcare Materials, Journal Year: 2024, Volume and Issue: 13(22)

Published: May 22, 2024

The past few decades have witnessed the rapid advancement and broad applications of flexible bioelectronics, in wearable implantable electronics, brain-computer interfaces, neural science technology, clinical diagnosis, treatment, etc. It is noteworthy that soft elastic conductive hydrogels, owing to their multiple similarities with biological tissues terms mechanics, water-rich, functions, successfully bridged gap between rigid electronics biology. Multifunctional hydrogel emerging as a new generation promising material candidates, authentically established highly compatible reliable, high-quality bioelectronic particularly recording stimulation. This review summarizes basis design principles involved constructing systematically discusses fundamental mechanism unique advantages bioelectrical interfacing surface. Furthermore, an overview state-of-the-art manufacturing strategies for interfaces enhanced biocompatibility integration system presented. finally exemplifies unprecedented impetus toward stimulation, especially integrated systems, concludes perspective expectation bioelectronics biomedical applications.

Language: Английский

Citations

19