Paintable, Fast Gelation, Highly Adhesive Hydrogels for High‐fidelity Electrophysiological Monitoring Wirelessly DOI

Leqi Li,

Xinyuan Ye,

Zichong Ji

et al.

Small, Journal Year: 2024, Volume and Issue: unknown

Published: Oct. 25, 2024

High-fidelity wireless electrophysiological monitoring is essential for ambulatory healthcare applications. Soft solid-like hydrogels have received significant attention as epidermal electrodes because of their tissue-like mechanical properties and high biocompatibility. However, it challenging to develop a hydrogel electrode that provides robust contact adhesiveness with glabrous skin hairy scalp high-fidelity, continuous signal detection. Here, paintable, fast gelation, highly adhesive, conductive engineered high-fidelity monitoring. The hydrogel, consisting gelatin, gallic acid, sodium citrate, lithium chloride, glycerol, Tris-HCl buffer solution exhibits reversible thermal phase transition capability, which endows the attributes on-skin applicability in situ gelation 15 s, thereby addressing aforementioned limitations. introduction acid enhances adhesive facilitating secure attachment or scalp. To accentuate potential applications at-home health monitoring, are demonstrated electrocardiogram recording one hour during various daily activities, well simultaneous electroencephalogram 30 min nap.

Language: Английский

Mechanisms, design, and fabrication strategies for emerging electromagnetic wave-absorbing materials DOI Creative Commons
Geng Chen,

Zijing Li,

Limin Zhang

et al.

Cell Reports Physical Science, Journal Year: 2024, Volume and Issue: 5(7), P. 102097 - 102097

Published: July 1, 2024

The rapid development of intelligent devices imposes new demands on electromagnetic wave (EMW)-absorbing materials, especially concerning wide-spectrum absorption, frequency band manipulation, and multifunctional integration. However, conventional investigations EMW-absorbing materials face several challenges that collectively limit the effectiveness existing amid growing demands, including ambiguous (EM) loss mechanisms, impedance mismatches, deficiencies in integrated design. This review elucidates EM delineates key bridge mechanisms linking microscopic macroscopic factors, proposes dielectric polarization models to clarify mechanisms. Additionally, it delves into unique advantages core-shell structures porous optimization. Finally, introduces fabrication approaches integrate detailing design strategies exploring potential applications. By consolidating these cutting-edge achievements, this aims guide scientific advancement materials.

Language: Английский

Citations

58

Smart sensing hydrogel actuators conferred by MXene gradient arrangement DOI

Jiazhou Zeng,

Xin Jing,

Liya Lin

et al.

Journal of Colloid and Interface Science, Journal Year: 2024, Volume and Issue: 677, P. 816 - 826

Published: Aug. 16, 2024

Language: Английский

Citations

22

Biocomposite silk fibroin hydrogel with stretchability, conductivity and biocompatibility for wireless strain sensor DOI
Rongjie Wang, Qiaoyun Liu, Jingjiang Wei

et al.

Journal of Material Science and Technology, Journal Year: 2024, Volume and Issue: 210, P. 195 - 203

Published: May 28, 2024

Language: Английский

Citations

21

Wearable Pressure Sensor Based on Triboelectric Nanogenerator for Information Encoding, Gesture Recognition, and Wireless Real‐Time Robot Control DOI Open Access
Mengjia Guo, Yifan Xia, Jiaxuan Liu

et al.

Advanced Functional Materials, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 21, 2025

Abstract Wearable sensor has attracted a broad interesting in application prospect of human‐machine interaction (HMI). However, most sensors are assembled the shape gloves to accurately capture complex hand motion information, thereby seriously blocking complete tasks. Herein, wearable pressure based on drum‐structured triboelectric nanogenerator (DS‐TENG) is developed subtle signals for physiological signal detection, information encoding, gesture recognition, and wireless real‐time robot control. The DS‐TENG enables limit detection down 3.9 Pa pressure, which can sensitively human micromotion pulse, throat sounds, wrist muscles contraction. Especially, combined with microprocessor Morse code, worn detect single‐finger translate into regular voltage signals, employed encode 26 letters subsequently decode corresponding letters. Furthermore, an aid machine learning, array (2 × 2) successfully achieve recognition high accuracy 92% wirelessly perform Consequently, encoding control, demonstrates extreme potential field HMI artificial intelligence.

Language: Английский

Citations

4

MXenes in healthcare: synthesis, fundamentals and applications DOI Creative Commons
Zaheer Ud Din Babar, Vincenzo Iannotti, Giulio Rosati

et al.

Chemical Society Reviews, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 1, 2025

Since their discovery over a decade ago, MXenes have transformed the field of "materials for healthcare", stimulating growing interest in healthcare-related applications. These developments also driven significant advancements MXenes' synthesis. This review systematically examines synthesis and applications sensing biomedical fields, underscoring pivotal role addressing critical challenges modern healthcare. We describe experimental by combining appropriate laboratory modules with mechanistic principles underlying each step. In addition, we provide extensive details on parameters, considerations, essential instructions successful Various healthcare including sensing, imaging, synergistic therapies, regenerative medicine, wearable devices been explored. further highlight emerging trends MXenes, viz., as nanovehicles drug delivery, vectors gene therapy, tools immune profiling. By identifying important parameters that define utility applications, this outlines strategies to regulate profile, thereby serving valuable guide design application-specific properties. The final section integrates research theoretical studies comprehensive understanding field. It technologies, such artificial intelligence (AI) machine learning (ML), accelerating material discovery, structure-property optimization, automation. Complemented detailed supplementary information synthesis, stability, biocompatibility, environmental impact, insights, offers profound knowledge base diverse family 2D materials. Finally, compared potential other materials underscore existing prioritize interdisciplinary collaboration. synthesizing key from its current (especially 2018 onward), provides cohesive assessment MXene foundations prospects sector.

Language: Английский

Citations

4

Robust accurate fatigue assessment enabled by an ultrasoft and super-adhesive low-impedance conducting polymer hydrogel DOI
Qi Liu,

Xinye Xu,

Y L Zhang

et al.

Chemical Engineering Journal, Journal Year: 2025, Volume and Issue: unknown, P. 161207 - 161207

Published: March 1, 2025

Language: Английский

Citations

2

Hydrophobic and Adhesive Elastomer Encapsulation for Anti‐Drying, Non‐Swelling, and Adhesive Hydrogels DOI

Huixin Yuan,

Tang Zhu,

Yuchan Huang

et al.

Advanced Functional Materials, Journal Year: 2024, Volume and Issue: unknown

Published: July 25, 2024

Abstract Traditional hydrogels often face issues like dehydration, excessive swelling, and poor adhesion, limiting their practical applications. This study presents a facile universal method to create elastomer‐encapsulated with improved water retention, non‐swelling, enhanced adhesion. n‐Butyl acrylate (BA) 2,2,3,4,4,4‐hexafluorobutyl methacrylate (HFBMA) are utilized as the “soft” “hard” monomers, respectively, in situ construct elastomer coatings on hydrogel surface through surface‐confined copolymerization. The resulting transparent, hydrophobic, adhesive coating is tightly bound surface, conferring upon it robust defense against dehydration swelling various media, strong adhesion diverse substrates both aerial submerged conditions. Furthermore, this encapsulation strategy also augments mechanical attributes of bulk hydrogel, including its tensile properties puncture resistance, applicable wide array types configurations. Additionally, applied conductive results flexible sensors high sensitivity, reversible resistance change, exceptional sensing stability, significantly durability air underwater environments. These suggest potential applications harsh environments, such acoustic detection sonar scanning camouflage for submarines.

Language: Английский

Citations

12

Ultrasensitive and Breathable Hydrogel Fiber‐Based Strain Sensors Enabled by Customized Crack Design for Wireless Sign Language Recognition DOI
Dijie Yao, Weiyan Wang, Hao Wang

et al.

Advanced Functional Materials, Journal Year: 2024, Volume and Issue: unknown

Published: Nov. 26, 2024

Abstract Wearable strain sensors, capable of continuously detecting human movements, hold great application prospects in sign language gesture recognition to alleviate the daily communication barriers deaf and mute community. However, unsatisfactory sensing performance (such as low sensitivity, narrow detection range, etc.) wearing discomfort severely hinder their practical application. Here, high‐performance breathable hydrogel sensors are proposed by introducing an adjustable localized crack a closed‐loop connected fiber encapsulated porous elastomer films. Upon loading/unloading external strain, dynamic opening/closing pre‐cut causes rapid switching conductive path, resulting sharp changes resistance high sensitivity. Consequently, hydrogel‐based crack‐effect sensor exhibits superb sensitivity (GF up 3930), broad range (from 0.02% 80%), fast response/recovery time (78/52 ms), repeatability, structural stability. Based on capability accurately detect various strains across full wireless system is developed achieve accuracy 98.1% encoding decoding gestures with assistance machine learning, providing robust platform for efficient intelligibility barrier‐free communication.

Language: Английский

Citations

9

Skin‐Mountable Thermo‐responsive Structured Hydrogel for Optical and Adhesion Coupled Functional Sensing DOI Open Access

Xinqiang Xu,

Yang Lyu, Di Liu

et al.

Small, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 2, 2025

Smart hydrogel sensors with intrinsic responsiveness, such as pH, temperature, humidity, and other external stimuli, possess broad applications in innumerable fields biomedical diagnosis, environmental monitoring, wearable electronics. However, it remains a great challenge to develop structural hydrogels that simultaneously body temperature-responsive, adhesion-adaptable, transparency-tunable. Herein, an innovative skin-mountable thermo-responsive is fabricated, which endows tunable optical properties switchable adhesion at different temperatures. Interestingly, able exhibit lower critical solution temperature (LCST) adapt the human by altering acrylic acid(AAc) content network. The also displays high transparency strong low temperatures, while becomes opaque feeble Furthermore, highly sensitive sensor array structure constructed harnessing vat photopolymerization three-dimensional (3D) printing. As proof of concept, attached back hand capable detecting strain differences, integrating high-temperature monitoring alarm functions visual alteration. This work provides advanced manner fabricate structured responsive hydrogels, have potential application prospects field smart medical patches devices.

Language: Английский

Citations

1

Fully Stretchable and Self-Healing Graphene-Hydrogel E-Skin with Temperature-Strain Self-Calibration DOI
Wei Sheng, Jianxin Zhou, Wentao Li

et al.

ACS Applied Nano Materials, Journal Year: 2025, Volume and Issue: unknown

Published: Feb. 5, 2025

Language: Английский

Citations

1