Dynamic regulation of ferroelectric polarization using external stimuli for efficient water splitting and beyond DOI
Sundaram Chandrasekaran, Qingping Wang, Qiong Liu

et al.

Chemical Society Reviews, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 1, 2025

Regulating the ferroelectric polarization in catalysts is an emerging strategy to advance water splitting reactions, with merits of high charge transfer rate, creation real active sites, and optimizing chemisorption energy.

Language: Английский

Ultrasound-assisted piezoelectric photocatalysis: An effective strategy for enhancing hydrogen evolution from water splitting DOI
Fengyi Yang,

Piyan Wang,

Jiehui Hao

et al.

Nano Energy, Journal Year: 2023, Volume and Issue: 118, P. 108993 - 108993

Published: Oct. 12, 2023

Language: Английский

Citations

48

Electron spin-states reconfiguration induced by alternating temperature gradient for boosting photocatalytic hydrogen evolution on hollow core-shell FeS2/CuCo2O4 Z-scheme heterostructure DOI
Zuming He, Kai Lin, Ngie Hing Wong

et al.

Nano Energy, Journal Year: 2024, Volume and Issue: 124, P. 109483 - 109483

Published: March 11, 2024

Language: Английский

Citations

40

Research Advances in Magnetic Field‐Assisted Photocatalysis DOI
Ru Li,

Li‐Peng Qiu,

Shize Cao

et al.

Advanced Functional Materials, Journal Year: 2024, Volume and Issue: 34(33)

Published: March 21, 2024

Abstract Solar‐to‐chemical energy conversion thorugh photocatalytic technology has garnered significant attention due to its potential for clean hydrogen pro duction, pollutant degradation, and carbon dioxide reduction. However, relatively low solar‐to‐chemical efficiency hinders industrial development. External fields have currently emerged as a supplementary source augment the overall catalytic efficiency. Recently, performance been considerably enhanced through magnetic field modulation, which promotes separation transfer of photoexcited charge carriers. This article systematically reviews recent research progress field–assisted photocatalysis, discussing phenomena such negative magnetoresistance effect, Lorentz force, spin polarization. It comprehensively analyzes effect on critical processes in photocatalysis: light absorption, charge‐carrier separation, surface reactions. In particular, this review focuses spin‐relaxation mechanism, explains how electron lifetime is extended polarization, proposes design strategies spin‐polarized materials. Finally, discusses challenges opportunities enhancing The ultimate objective offer notable theoretical experimental insights that can guide development high‐performance photocatalysts systems.

Language: Английский

Citations

26

Electric effects reinforce charge carrier behaviour for photocatalysis DOI

Aoqiang Shu,

Chencheng Qin,

Miao Li

et al.

Energy & Environmental Science, Journal Year: 2024, Volume and Issue: 17(14), P. 4907 - 4928

Published: Jan. 1, 2024

Recent studies on enhancing charge carrier behavior through electric effects for efficient photocatalysis are summarized, evaluating the in-depth function of these effects. This provides unique perspectives to optimize photocatalytic processes.

Language: Английский

Citations

26

Magnetic-field-induced activation of S-scheme heterojunction with core–shell structure for boosted photothermal-assisted photocatalytic H2 production DOI
Pengyu Hao,

Pengnian Shan,

Jialin Lu

et al.

Fuel, Journal Year: 2024, Volume and Issue: 373, P. 132394 - 132394

Published: July 2, 2024

Language: Английский

Citations

23

Insight into synergy of Mn active sites and spin polarization electrons in Mn-incorporated ZnIn2S4 for boosting photocatalytic hydrogen evolution coupled with benzyl alcohol oxidation DOI
Zuming He, Yongmei Xia, Gang He

et al.

Chemical Engineering Journal, Journal Year: 2025, Volume and Issue: unknown, P. 159957 - 159957

Published: Jan. 1, 2025

Language: Английский

Citations

6

Insights into Operating Conditions on Electrocatalytic CO2 Reduction DOI Open Access
Zhaozhao Zhu, Wu Tang, Junjie Wang

et al.

Advanced Energy Materials, Journal Year: 2025, Volume and Issue: unknown

Published: Feb. 5, 2025

Abstract Electrocatalytic CO 2 reduction (CO RR) is rapidly emerging as a promising sustainable strategy for transforming into valuable fuels and chemical feedstocks, crucial step toward carbon‐neutral society. The efficiency, selectivity, stability of RR are heavily influenced by the chosen catalyst operating conditions used. Despite substantial advances in development catalysts, there scarcity comprehensive reviews focusing on influence different environments performance. This review offers detailed examination internal external environmental control strategies designed to enhance efficiency. fundamental reaction mechanisms through situ operational techniques, paired with theoretical analyses, discussed while also identifying key challenges future research directions technology. By delivering overview current state field, this highlights critical role control, mechanistic insights, practical considerations needed successful commercialization

Language: Английский

Citations

2

Review of photoelectrochemical water splitting: From quantitative approaches to effect of sacrificial agents, oxygen vacancies, thermal and magnetic field on (photo)electrolysis DOI
Mohamed El Ouardi, Ayoub El Idrissi, Madjid Arab

et al.

International Journal of Hydrogen Energy, Journal Year: 2023, Volume and Issue: 51, P. 1044 - 1067

Published: Sept. 26, 2023

Language: Английский

Citations

39

Constructing durable BiFeO3@SrBi2B2O7 p-n heterojunction for persulfate enhanced piezo-photocatalytic water purification DOI
Yinxu Wang, Jie Chen, Jian Wu

et al.

Separation and Purification Technology, Journal Year: 2023, Volume and Issue: 324, P. 124479 - 124479

Published: June 29, 2023

Language: Английский

Citations

28

Unification of hot spots and catalytic sites on isolated boron centers in porous carbon nitride nanosheets for efficient photocatalytic oxygen evolution DOI Creative Commons

Fengting He,

Shuling Wang,

Yang‐Ming Lu

et al.

Nano Energy, Journal Year: 2023, Volume and Issue: 116, P. 108800 - 108800

Published: Aug. 18, 2023

The quest for maximum photocatalysis necessitates the unification of hot spots and catalytic sites on photocatalysts. Herein, boron atoms were successfully incorporated into tri-s-triazine unit C3N4 (PCN-B-X), in form isolated B-N coordination. In-situ experimental simulation analyses collectively demonstrated that resulting atomic B centers cyano groups functioned as to amplify charge dynamics localized density. Concurrently, coordination served sites, reducing activation energy oxygen evolution reaction. Whereas, excessive precursor led partial B-B bonding, adversely affecting optical absorption separation. Consequently, optimal photocatalytic activity was achieved at an rate 248.9 µmol h−1 g−1 (λ > 420 nm), when harmoniously aligned PCN-B-20, surpassing by 5.2 times. This study provides insights mechanism suggests approaches develop robust metal-free photocatalysts solar fuel production.

Language: Английский

Citations

27