Trends in Chemistry, Journal Year: 2022, Volume and Issue: 4(9), P. 822 - 834
Published: July 28, 2022
Language: Английский
CHINESE JOURNAL OF CATALYSIS (CHINESE VERSION), Journal Year: 2022, Volume and Issue: 43(2), P. 178 - 214
Published: Jan. 17, 2022
Language: Английский
Citations
633
Energy & environment materials, Journal Year: 2021, Volume and Issue: 5(4), P. 1012 - 1036
Published: Sept. 12, 2021
The number of lithium‐ion batteries (LIBs) is steadily increasing in order to meet the ever‐growing demand for sustainable energy and a high quality life humankind. At same time, resulting large LIB waste certainly poses safety hazards if it not properly disposed will seriously harm environment due its inherent toxicity use toxic substances. Moreover, consumption many scarce precious metal resources behind mass production batteries. In light severe environmental, resources, recycling problems, spent LIBs have become an essential urgently needed action achieve social development. This review therefore critically analyses value need from variety environment. A range existing technologies reusing LIBs, such as pretreatment, pyrometallurgy, hydrometallurgy, direct recycled methods, subsequently summarized exclusively. addition, benefits problems methods described above are analyzed detail. It also introduces progress other components, anodes, separators, electrolytes, well high‐value cathode. Finally, prospects addressed four ways (government, users, battery manufacturers, recyclers). should contribute development used particularly support industrialization processes.
Language: Английский
Citations
280
ACS Catalysis, Journal Year: 2022, Volume and Issue: 12(8), P. 4659 - 4679
Published: April 5, 2022
Plastics are indispensable, but their pollution is triggering a global environmental crisis. Although many end-of-life catalytic options have involved converting plastics into valuable products, deep understanding of the relationship between polymer structure and recycling performance significant urgently needed. Here, we start with primer polymeric chain structures on chemical discuss structure–performance polymer, catalyst, reaction. Specifically, development challenges re/upcycling waste PET polyolefins discussed in-depth. In addition, also present some prospects for innovations in catalyst synthesis reaction engineering basis relationship. The discussion ends brief perspective future plastic re/upcycling. Overall, intelligent catalysis design necessary incentivizing relieving burden plastics.
Language: Английский
Citations
221
Applied Surface Science, Journal Year: 2022, Volume and Issue: 610, P. 155346 - 155346
Published: Oct. 30, 2022
Language: Английский
Citations
210
Science Bulletin, Journal Year: 2021, Volume and Issue: 67(4), P. 389 - 397
Published: Oct. 20, 2021
Language: Английский
Citations
117
Small, Journal Year: 2022, Volume and Issue: 18(25)
Published: May 9, 2022
Heteroatom doping can endow MXenes with various new or improved electromagnetic, physicochemical, optical, and structural properties. This greatly extends the arsenal of materials their potential for a spectrum applications. article comprehensively critically discusses syntheses, properties, emerging applications growing family heteroatom-doped materials. First, strategies, synthesis methods, theoretical simulations high-performance are summarized. In order to achieve materials, mechanism atomic element from three aspects lattice optimization, functional substitution, interface modification is analyzed summarized, aiming provide clues developing controllable synthetic routes. The mechanisms underlying advantageous uses energy storage, catalysis, sensors, environmental purification biomedicine highlighted. Finally, future opportunities challenges study application multifunctional presented. work could open up prospects development MXenes.
Language: Английский
Citations
96
SusMat, Journal Year: 2022, Volume and Issue: 2(2), P. 161 - 185
Published: April 1, 2022
Abstract The mass production of disposable polyolefin products has led to serious plastic pollution and an imbalance between manufacturing recycling. Given these challenges, the chemical upcycling waste polyolefins attracted extensive attention due its high efficiency economic benefits. Herein, we review development in heterogeneous catalysis. status quo recycling is first discussed. We then introduce advanced strategies for view different value‐added discuss their challenges prospects. Our in‐depth analysis centers on catalytic mechanism design principle catalysts. Finally, outlook promising directions facilitate degradation process via polymer catalyst optimized engineering. Innovative are expected promote polyolefins, bringing great promise sustainable society.
Language: Английский
Citations
88
The Science of The Total Environment, Journal Year: 2023, Volume and Issue: 912, P. 169160 - 169160
Published: Dec. 10, 2023
Language: Английский
Citations
88
ACS Catalysis, Journal Year: 2022, Volume and Issue: 12(15), P. 9486 - 9493
Published: July 20, 2022
Rational engineering of metal–organic frameworks (MOFs) with maximum exposed highly active facets for photocatalytic CO2 reduction is desirable yet remains greatly challenging. Herein, ultrathin Ti-MOF NH2-MIL-125 nanosheets are successfully fabricated through a facile and efficient approach relying on the precursors directly. Importantly, surfaces dominated by {110} facet, which has more sites than {001} {111}. In contrast conventional catalysts {001}, {110}, {111} facets, nanosheet material reported here exhibits remarkably high photoreduction performance affording abundant augmented photoinduced electrons. The enhanced solar conversion activity attributed to favorable distribution photoexcited electrons over all Ti in outer surface nanosheet, as revealed density functional theory simulations.
Language: Английский
Citations
82
Journal of Material Science and Technology, Journal Year: 2023, Volume and Issue: 153, P. 205 - 218
Published: March 5, 2023
Language: Английский
Citations
79