Small‐Molecule Mixed Ionic‐Electronic Conductors for Efficient N‐Type Electrochemical Transistors: Structure‐Function Correlations DOI Creative Commons
Yongjoon Cho,

Lin Gao,

Yao Yao

et al.

Angewandte Chemie, Journal Year: 2024, Volume and Issue: unknown

Published: Sept. 23, 2024

Abstract The fundamental challenge in electron‐transporting organic mixed ionic‐electronic conductors (OMIECs) is simultaneous optimization of electron and ion transport. Beginning from Y6‐type/U‐shaped non‐fullerene solar cell acceptors, we systematically synthesize characterize molecular structures that address the aforementioned challenge, progressively introducing increasing numbers oligoethyleneglycol (OEG; g) sidechains 1 g to 3 g, affording OMIECs 1gY, 2gY, 3gY, respectively. crystal structure 1gY preserves key structural features Y n series: a U‐shaped/planar core, close π–π stacking, interlocked acceptor groups. Versus inactive Y6 Y11, all new glycolated compounds exhibit ion‐electron transport both conventional electrochemical transistor (cOECT) vertical OECT (vOECT) architectures. Notably, 3gY with highest OEG density achieves high transconductance 16.5 mS, an on/off current ratio ~10 6 , turn‐on/off response time 94.7/5.7 ms vOECTs. Systematic optoelectronic, electrochemical, architectural, crystallographic analysis explains superior 3gY‐based performance terms denser gY content, increased crystallite dimensions decreased long‐range crystalline order, enhanced film hydrophilicity which facilitates efficient redox processes. Finally, demonstrate small‐molecule‐based complementary inverter using vOECTs, showcasing bioelectronic applicability these small‐molecule OMIECs.

Language: Английский

Metal nanowire-based transparent electrode for flexible and stretchable optoelectronic devices DOI
Yu Ding, Sixing Xiong, Lulu Sun

et al.

Chemical Society Reviews, Journal Year: 2024, Volume and Issue: 53(15), P. 7784 - 7827

Published: Jan. 1, 2024

This review provides the state-of-the-art solution-processed metal nanowire-based flexible transparent electrodes and their applications in optoelectronic devices.

Language: Английский

Citations

18

Bioinspired interfacial engineering for highly stretchable electronics DOI Creative Commons
Osman Gul, Myoung Song, Chang-Yeon Gu

et al.

Nature Communications, Journal Year: 2025, Volume and Issue: 16(1)

Published: Feb. 4, 2025

The seamless integration of rigid/flexible electronic components into stretchable substrates is imperative for the realization reliable electronics. However, transition from flexible-to-stretchable presents inherent challenges in interfacial behavior, predominantly arising disparities elastic moduli, thereby rendering their arduous practical deployment. Here, we introduce a bioinspired interface-engineered flexible island (BIEFI), which effectively facilitates creation highly electronics by optimizing interface with mechanical interlocking mechanisms, resilient to physical deformations. Various components, such as light-emitting diodes (LEDs) and solar cells, are affixed onto island, showcasing its versatility robust platform rigid while ensuring entire substrate maintains high stretchability. Additionally, smart workout monitoring system demonstrated integrating resistance band platform. This approach seamlessly integrates wide range rigid, flexible, durability under diverse limited behavior. authors present an design deformations

Language: Английский

Citations

2

Superhydrophobic stretchable conductive composite textile with weft-knitted structure for excellent electromagnetic interference shielding and Joule heating performance DOI

Tai-Bao Yang,

Ji‐You Zong,

De‐Zhuang Jia

et al.

Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: 489, P. 151360 - 151360

Published: April 16, 2024

Language: Английский

Citations

15

Diving into Sweat: Advances, Challenges, and Future Directions in Wearable Sweat Sensing DOI Creative Commons

Andre Childs,

Beatriz Mayol, José A. Lasalde‐Ramírez

et al.

ACS Nano, Journal Year: 2024, Volume and Issue: 18(36), P. 24605 - 24616

Published: Aug. 26, 2024

Sweat analysis has advanced from diagnosing cystic fibrosis and testing for illicit drugs to noninvasive monitoring of health biomarkers. This article introduces the rapid development wearable flexible sweat sensors, highlighting key milestones various sensing strategies real-time analytes. We discuss challenges such as developing high-performance nanomaterial-based biosensors, ensuring continuous production sampling, achieving high sweat/blood correlation, biocompatibility. The potential machine learning enhance these sensors personalized healthcare is presented, enabling tracking prediction physiological changes disease onset. Leveraging advancements in electronics, nanomaterials, biosensing, data analytics, biosensors promise revolutionize management, prevention, prediction, promoting healthier lifestyles transforming medical practices globally.

Language: Английский

Citations

15

Pnipaam-based temperature responsive ionic conductive hydrogels for flexible strain and temperature sensing DOI

Tongda Lei,

Yongheng Wang, Yaya Feng

et al.

Journal of Colloid and Interface Science, Journal Year: 2024, Volume and Issue: 678, P. 726 - 741

Published: Sept. 17, 2024

Language: Английский

Citations

13

Recent progress in biocompatible miniature supercapacitors DOI Open Access
Pingping Luo, Qing Liu, Rui Chen

et al.

Energy Materials, Journal Year: 2025, Volume and Issue: 5(7)

Published: March 10, 2025

With the advancement of wearable and implantable health medical electronics, biocompatible miniature energy storage devices were developed rapidly. In particular, supercapacitors (BMSCs) have advantages conventional supercapacitors, such as high-power density, fast charging/discharging rate, long operating lifetime, well strong selectivity materials. They are expected to play an important role in personalized electronic integration systems. Biocompatibility involves biosafety materials relates mechanics geometrical forms. For example, BMSCs should be thin compact, ensuring ease portability comfort for users. also flexible stretchable conform skin or tissue, providing stable power electronics even under deformation. Furthermore, biodegradability/ bioabsorbability ensures they both body- environment-friendly. This review summarizes recent research progress devices, including basic requirements selection components. Additionally, advanced applications multifunctional systems real-time monitoring treatment introduced, along with associated challenges prospects.

Language: Английский

Citations

1

An Overview of Advances and Challenges in Developing Nanofiber Yarns for Wearable Technology DOI Creative Commons

Syamini Jayadevan,

Akshaya Kumar Aliyana,

George K. Stylios

et al.

Nano Energy, Journal Year: 2024, Volume and Issue: 129, P. 110034 - 110034

Published: July 23, 2024

Language: Английский

Citations

8

Combinatorial Bionic Hierarchical Flexible Strain Sensor for Sign Language Recognition with Machine Learning DOI

Xuanjie Zong,

Nianqiang Zhang, Jilai Wang

et al.

ACS Applied Materials & Interfaces, Journal Year: 2024, Volume and Issue: 16(29), P. 38780 - 38791

Published: July 16, 2024

Flexible strain sensors have been widely researched in fields such as smart wearables, human health monitoring, and biomedical applications. However, achieving a wide sensing range high sensitivity of flexible simultaneously remains challenge, limiting their further To address these issues, cross-scale combinatorial bionic hierarchical design featuring microscale morphology combined with macroscale base to balance the is presented. Inspired by combination serpentine butterfly wing structures, this study employs three-dimensional printing, prestretching, mold transfer processes construct sensor (CBH-sensor) serpentine-shaped inverted-V-groove/wrinkling-cracking structures. The CBH-sensor has 150% gauge factor up 2416.67. In addition, it demonstrates application array sign language gesture recognition, successfully identifying nine different gestures an impressive accuracy 100% assistance machine learning. exhibits considerable promise for use enabling unobstructed communication between individuals who those do not. Furthermore, wide-ranging possibilities field gesture-driven interactions human-computer interfaces.

Language: Английский

Citations

5

Strain-Sensor-In-Pixel Technology for Resolution-Sustainable Stretchable Displays DOI

Won Kyung Min,

Jong Bin An,

Byung Ha Kang

et al.

ACS Nano, Journal Year: 2024, Volume and Issue: 18(27), P. 17735 - 17748

Published: June 27, 2024

One of the limitations stretchable displays is severe degradation resolution or decrease in number pixels per unit area when stretched. Hence, we suggest a strain-sensor-in-pixel (S-SIP) system through adoption hidden that are activated only during stretch mode for maintaining density on-state pixels. For S-SIP system, gate and source electrodes InGaZnO thin-film transistors (TFTs) an existing pixel connected to resistive strain sensor facile selective deposition silver nanowires (AgNWs) via electrohydrodynamic-jet-printing. With this approach, integrated TFT functions as strain-triggered switch, which responds stretching along designated axes by finely tuning orientation cycles AgNW printing. The sensor-integrated remains off-state unstretched switches stretched, exhibiting large negative gauge factor -1.1 × 1010 superior mechanical stability enduring 6000 cycles, enables efficient structure operate without requiring additional signal processing. Furthermore, stable operation 5 5-pixel array demonstrated circuit simulation, implying outstanding applicability process compatibility conventional active-matrix display backplanes.

Language: Английский

Citations

4

Strain‐induced morphology evolution and charge transport in conjugated polymer films DOI Creative Commons
Zicheng Ding, Kui Zhao, Yanchun Han

et al.

Interdisciplinary materials, Journal Year: 2024, Volume and Issue: unknown

Published: Oct. 17, 2024

Abstract Stretchable conjugated polymer films are pivotal in flexible and wearable electronics. Despite significant advancements film stretchability through molecular engineering multicomponent blending, these often exhibit limited elastic ranges reduced carrier mobilities under large strain or after cyclic stretching. These limitations hinder their application Therefore, it is imperative to reveal the mechanical fatigue mechanisms incorporate multiple energy dissipation strategies enhance deformation electrical performance of stretched films. In this review, we begin by introducing typical behaviors Subsequently, discuss multiscale structural evolution various stretching conditions based on both in‐situ ex‐situ characterizations. This analysis further related diverse mechanisms. We next establish correlation between strain‐induced microstructure After that, propose develop highly constructing stable crosslinks promoting dynamics low‐crystalline Finally, highlight future opportunities for high‐performance mechanically devices stretchable

Language: Английский

Citations

4