Lead-free metal–halide perovskite nanocrystals: synthesis and optical properties [Review] DOI
Yuliya A. Timkina, Ivan D. Skurlov, Aleksandr P. Litvin

et al.

Journal of Optical Technology, Journal Year: 2024, Volume and Issue: 91(6), P. 429 - 429

Published: June 1, 2024

Subject of study. Lead-free perovskite nanocrystals (LFPNCs), their main characteristics, synthesis methods, and optical properties are examined. Aim The aim is to analyze the state-of-the-art research data on methods LFPNCs. In addition, formation processes LFPNCs, dependence nanocrystal size photoluminescence quantum yield (PLQY) parameters (such as method, temperature, ligand type) determined. Main results. LFPNCs analyzed based LaMer cluster growth models. According data, primary for preparing these (NCs) hot-injection ligand-assisted reprecipitation (LARP). Evidently, average increases with increasing reaction temperature. For NCs synthesized by LARP, temperature 100°C leads a slight decrease in yield. However, prepared hot-injection, PLQY remains independent Additionally, using oleic acid results narrow distribution NCs, whereas mixture ligands exhibiting highest PLQY. Practical significance. literature analysis show that LARP method most promising synthesizing owing its ease implementation, energy efficiency, scalability. produced this can be applied active materials sensor technologies, photovoltaics, optoelectronic devices.

Language: Английский

Multicolor luminescence of carbon Dots: From mechanisms to applications DOI

Man Jiang,

Yuzhu Sun, Mingyue Chen

et al.

Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: 496, P. 153761 - 153761

Published: July 5, 2024

Language: Английский

Citations

18

Designing carbon dots for enhanced photo-catalysis: Challenges and opportunities DOI
Lukáš Zdražil, Alejandro Cadranel, Miroslav Medveď

et al.

Chem, Journal Year: 2024, Volume and Issue: 10(9), P. 2700 - 2723

Published: Aug. 19, 2024

Language: Английский

Citations

10

Machine learning-assisted carbon dots synthesis and analysis: state of the art and future directions DOI
Fanyong Yan, Ruixue Bai, Juanru Huang

et al.

TrAC Trends in Analytical Chemistry, Journal Year: 2025, Volume and Issue: unknown, P. 118141 - 118141

Published: Jan. 1, 2025

Language: Английский

Citations

1

Aggregated carbon dots endow them with room-temperature phosphorescence in aqueous environments: Mechanisms, properties, and applications DOI
Shuai Ye, Shujian Ji,

Minghao Kang

et al.

Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: 495, P. 153653 - 153653

Published: July 1, 2024

Language: Английский

Citations

7

Machine Learning for Carbon Dots Synthesis and Applications DOI Creative Commons
Ali Nabi Duman, Almaz S. Jalilov

Materials Advances, Journal Year: 2024, Volume and Issue: 5(18), P. 7097 - 7112

Published: Jan. 1, 2024

One of the hottest topics in nanoparticles research right now is carbon dots (CDs).

Language: Английский

Citations

6

Exploring Carbon Dots: Green Nanomaterials for Unconventional Lasing DOI Creative Commons
Gianluca Minervini, Annamaria Panniello, Carlo Nazareno Dibenedetto

et al.

Small, Journal Year: 2024, Volume and Issue: 20(47)

Published: Aug. 20, 2024

In recent years, the progress toward lighting miniaturization is focused on luminescent nanomaterials. Among them, fluorescent carbon dots (CDs) are receiving increasing attention thanks to their astonishing optical properties complemented by intrinsic biocompatibility and low toxicity. The CDs can be easily dispersed in water, organic solvents or incorporated polymeric matrices, preserving emission properties. However, relationship between structural still not fully elucidated, motivating a consistent research effort for comprehension of features. Nevertheless, demonstrate efficient gain materials lasing, high quantum yield (QY), tunability visible near infrared (NIR) range, short lifetimes, absorption cross section, even if synthetic reproducibility, reaction spectral width may limit effective exploitation. This review summarizes latest advancements investigation characteristic that make laser action possible, illustrating geometries lasing random both solution solid state, few currently demonstrated breakthroughs. While journey application long, potential CD-based sources promising various technological fields futuristic perspectives will discussed.

Language: Английский

Citations

5

Effect of Gadolinium Doping on the Optical and Magnetic Properties of Red-Emitting Dual-Mode Carbon Dot-Based Probes for Magnetic Resonance Imaging DOI

Arina A. Efimova,

Zilya Badrieva, Ekaterina Brui

et al.

ACS Applied Bio Materials, Journal Year: 2025, Volume and Issue: 8(2), P. 1493 - 1502

Published: Jan. 31, 2025

Bioimaging probes based on carbon dots (CDs) can become a useful replacement for existing commercial probes, benefiting clinical diagnostics. While the development of dual-mode CD-based magnetic resonance imaging (MRI), which provides ability photoluminescence (PL) detection at same time, is ongoing, several challenges have to be addressed. First, most still emit shorter wavelengths (blue/green spectral range), harmful biological objects or very low PL intensity in window tissue transparency (red/near-infrared range). Second, relaxation characteristics proposed are similar only slightly larger than those contrast agents. Herein, we introduce probe allowing simultaneous and MRI analysis, CDs doped with gadolinium ions (Gd3+) peak red (640 nm), quantum yield up 24%, high longitudinal transverse relaxivities reaching 25.76 40.57 L mmol-1 s-1, respectively. Moreover, Gd-doped show good biocompatibility, was studied H9c2 4T1 cell lines viability above 70%. The developed red-emissive utilized as efficient nontoxic measurements carried out simultaneously.

Language: Английский

Citations

0

Computational Modeling of Properties of Quantum Dots and Nanostructures: From First Principles to Artificial Intelligence (A Review) DOI Creative Commons
Grzegorz Matyszczak, Krzysztof Krawczyk,

Albert Yedzikhanau

et al.

Nanomaterials, Journal Year: 2025, Volume and Issue: 15(4), P. 272 - 272

Published: Feb. 11, 2025

Nanomaterials, including quantum dots, have gained more and attention in the past few decades due to their extraordinary properties that make them useful for many applications, ranging from catalysis, energy generation storage, biotechnology, medicine informatics. Mathematical descriptions of phenomena which nanostructures are involved great demand because they may be utilized purpose controlling these (e.g., growth with certain sizes, shapes, other properties). Such models distinct nature, calculations first principles, ordinary partial differential equations, machine learning (including artificial intelligence) as well. The aim this article is review most important computational mathematical approaches description control processes involving nanostructures.

Language: Английский

Citations

0

Bottom-up carbon dots: purification, single-particle dynamics, and electronic structure DOI Creative Commons

Zhengyi Bian,

Eric J. Gomez,

Martin Gruebele

et al.

Chemical Science, Journal Year: 2025, Volume and Issue: 16(10), P. 4195 - 4212

Published: Jan. 1, 2025

The physico-chemical properties of 'bottom-up' carbon dots synthesized from small molecules feature both generalities, such as sp2-networked and core-surface energy transfer, heterogeneities, due to the unpredictable location heteroatoms often non-crystalline structure. Here we focus our review on three aspects these systems: (1) coupling characterization with bottom-up synthesis identify remove confounding byproducts or hydrogen-rich polymers; (2) single-particle obtain unambiguous information highlight distribution around ensemble average; (3) electronic structure how it can help elucidate origin important optical absorption fluorescence a heterogeneous dots.

Language: Английский

Citations

0

Machine learning algorithms for predicting the photoionization cross section of CdS/ZnSe core/shell spherical quantum dots surrounded by dielectric matrices DOI Creative Commons

A. Cherni,

N. Zeiri, N. Yahyaoui

et al.

Results in Physics, Journal Year: 2025, Volume and Issue: unknown, P. 108186 - 108186

Published: March 1, 2025

Language: Английский

Citations

0