Generalized Interfacial Assembly of 2D Mesoporous Heterostructures for High‐Energy Solid‐State Micro‐Supercapacitors DOI
Jieqiong Qin, Hongtao Zhang,

Tiesheng Bai

et al.

Advanced Functional Materials, Journal Year: 2024, Volume and Issue: unknown

Published: June 5, 2024

Abstract 2D materials have garnered considerable interest in various applications from catalysis to energy storage. However, the self‐stacking and poor air stability of (e.g., MXene) leads serious performance degradation, particular, micro‐supercapacitors (MSCs) with narrow working voltage low density. Here, a universal confined interfacial assembly strategy is demonstrated for controllably synthesizing series mesoporous heterostructures high‐voltage high‐energy ionogel‐based MSCs. This process reveals accurate controllability extraordinary versatility, endowing highly adjustable mesopore size (7–22 nm), tunable thickness (15–29 variable carbon precursors (including oligochitosan, glucose, sucrose), replaceable substrates MXene, graphene, BN, MoS 2 ). As proof concept, carbon@MXene based MSCs ionic liquid ionogel electrolyte deliver ultrahigh 3.7 V, superior areal density 181.3 µWh cm −2 , excellent flexibility 99% capacitance retention at 180°, modular self‐integration voltage/capacitance output, surpassing most reported MXene Therefore, this work will open novel available paradigm scalable fabrication target high‐performance functional microscale power source.

Language: Английский

Advancing MXene-based integrated microsystems with micro-supercapacitors and/or sensors: Rational design, key progress, and challenging perspectives DOI Creative Commons
Jin Jia, Yuanyuan Zhu, Pratteek Das

et al.

Journal of Materiomics, Journal Year: 2023, Volume and Issue: 9(6), P. 1242 - 1262

Published: Sept. 25, 2023

The escalating demand for micro/nano-sized devices, such as micro/nano-robots, intelligent portable/wearable microsystems, and implantable medical microdevices, necessitates the expeditious development of integrated microsystems incorporating energy conversion, storage, consumption. Critical bottlenecks in microscale storage/sensors their systems are being addressed by exploring new technologies materials, e.g., MXene, holding great potential developing lightweight deformable microdevices. This review summarizes latest progress milestones realization MXene-based micro-supercapacitors (MSCs) sensor arrays, thus discusses design fundamentals key advancements conversion-storage-consumption microsystems. Finally, we outline challenges fabricating MSCs/sensors self-powered which is crucial practical applications. Particularly, illuminate viable solutions to unsolved issues highlight exciting opportunities.

Language: Английский

Citations

22

Beyond conventional limits: Advancements and insights in broadening operating temperature ranges of supercapacitors DOI
Xin Jiang, Jin Jia, Yuanyuan Zhu

et al.

Energy storage materials, Journal Year: 2024, Volume and Issue: 70, P. 103462 - 103462

Published: May 8, 2024

Language: Английский

Citations

7

Flexible wood-based composite for solar water evaporation and waste heat power generation DOI

Jingyu Wu,

Tong Li, Qian Zhao

et al.

Sustainable materials and technologies, Journal Year: 2024, Volume and Issue: 40, P. e00950 - e00950

Published: April 24, 2024

Language: Английский

Citations

6

Aptamer‐Functionalized Magnetic Ti3C2 Based Nanoplatform for Simultaneous Enrichment and Detection of Exosomes DOI
Hongyuan Cui,

Tianfang Zheng,

Nana Qian

et al.

Small, Journal Year: 2024, Volume and Issue: 20(44)

Published: July 6, 2024

Exosomes are nanovesicles secreted by cells, which play a crucial role in various pathological processes. have shown great promise as tumor biomarkers because of the abundant secretion during formation. The development convenient, efficient, and cost-effective method for simultaneously enriching detecting exosomes is utmost importance both basic research clinical applications. In this study, an aptamer-functionalized magnetic Ti

Language: Английский

Citations

6

A dual-acetate synchronous catalysis-activation strategy towards regulable porous graphitic carbon for high-energy supercapacitor with acetate water-in-salt electrolyte DOI
Huanxi Liao, Longsheng Zhong,

Hejun Zeng

et al.

Carbon, Journal Year: 2023, Volume and Issue: 213, P. 118305 - 118305

Published: July 18, 2023

Language: Английский

Citations

15

Ti3−yNbyC2T MXenes as high-rate and ultra-stable electrode materials for supercapacitors DOI
Qiang Wang, Xiao Zhang, Zhipeng Chen

et al.

Journal of Alloys and Compounds, Journal Year: 2023, Volume and Issue: 954, P. 170128 - 170128

Published: April 14, 2023

Language: Английский

Citations

14

Stepwise Construction of MoS2@CoAl-LDH/NF 3D Core–Shell Nanoarrays with High Hole Mobility for High-Performance Asymmetric Supercapacitors DOI
Yue Yan,

Wenrui Wu,

Yang Yang

et al.

ACS Applied Materials & Interfaces, Journal Year: 2024, Volume and Issue: 16(25), P. 32434 - 32444

Published: June 11, 2024

Supercapacitors (SCs) have received widespread attention as excellent energy storage devices, and the design of multicomponent electrode materials construction ingenious structures are keys to enhancing performance SCs. In this paper, MoS2 nanorods were used carrier structure induce anchoring CoAl-LDH nanosheets grow on surface nickel foam (NF) in situ, thus obtaining a uniformly distributed nanorod@CoAl-LDH nanosheet core–shell nanoarray material (MoS2@CoAl-LDH/NF). On one hand, nanorod-structured core provides high conductivity support, accelerates electron transfer, avoids agglomeration nanosheets. other arrays abundant interfacially active sites, which accelerate electrolyte penetration enhance electrochemical activity. The synergistic effect two components unique nanostructure give MoS2@CoAl-LDH/NF capacity (14,888.8 mF cm–2 at 2 mA cm–2) long-term cycling (104.4% retention after 5000 charge/discharge cycles). integrated MoS2@CoAl-LDH/NF//AC device boasts voltage range spanning from 0 1.5 V, achieving peak density 0.19 mW h cm–2. Impressively, it maintains capacitance rate 84.6% enduring 10,000 cycles, demonstrating exceptional durability stability.

Language: Английский

Citations

5

A review on multi-scale structure engineering of carbon-based electrode materials towards dense energy storage for supercapacitors DOI
Dongyang Wu, Fei Sun, Min Xie

et al.

Journal of Energy Chemistry, Journal Year: 2024, Volume and Issue: unknown

Published: Nov. 1, 2024

Language: Английский

Citations

5

Phosphorus Doping Strategy-Induced Synergistic Modification of Interlayer Structure and Chemical State in Ti3C2Tx toward Enhancing Capacitance DOI Creative Commons
Lihong Chen,

Yifan Bi,

Yunqi Jing

et al.

Molecules, Journal Year: 2023, Volume and Issue: 28(13), P. 4892 - 4892

Published: June 21, 2023

Heteroatom doping is considered an effective method to substantially improve the electrochemical performance of Ti

Language: Английский

Citations

12

Molecular dynamics simulations of ionic liquids confined into MXenes DOI
Abner Massari Sampaio, Sheng Bi, Mathieu Salanne

et al.

Energy storage materials, Journal Year: 2024, Volume and Issue: 70, P. 103502 - 103502

Published: May 31, 2024

Language: Английский

Citations

4