ACS Sustainable Chemistry & Engineering,
Journal Year:
2022,
Volume and Issue:
10(11), P. 3546 - 3556
Published: March 8, 2022
Ti3C2Tx
MXene
has
drawn
remarkable
attention
in
electronic
sensors.
Existing
MXene-based
pressure
sensors
generally
have
a
narrow
linear
sensing
range,
which
limits
their
wide
application.
Moreover,
previous
studies
on
were
mainly
focused
increasing
sensitivity
via
various
microengineering
techniques,
but
little
been
paid
to
environmental
stability
and
biocompatibility
of
these
Herein,
highly
flexible,
biocompatible,
environmentally
stable
MXene/bamboo
cellulose
fiber
(BCF)/poly(dimethylsiloxane)
(PDMS)
composite
sensor
with
an
ultrawide
working
range
(up
2
MPa),
high
linearity
(R2
=
0.966),
long-term
is
demonstrated.
First,
the
MXene/BCF
(MB)
foam
well-optimized
porosity
connectivity
was
prepared
through
efficient
freeze-drying
method.
Then,
MB-based
piezoresistive
(PMB)
obtained
by
directly
embedding
MB
foams
into
PDMS
elastomers.
In
striking
contrast
composite-based
sensors,
PMB
exhibits
not
only
excellent
performance
good
also
prominent
work
reliability
resist
temperature
fluctuation,
moisture/water,
UV
irradiation.
Furthermore,
demonstrate
potential
sensor,
human
movements
under
both
ambient
harsh
conditions
monitored.
Finally,
successfully
integrated
soft
robotic
hands
show
its
great
tactile
sensation.
ACS Applied Materials & Interfaces,
Journal Year:
2022,
Volume and Issue:
14(13), P. 15504 - 15516
Published: March 28, 2022
The
universal
application
of
wearable
strain
sensors
in
various
situations
for
human-activity
monitoring
is
considerably
limited
by
the
contradiction
between
high
sensitivity
and
broad
working
range.
There
still
remains
a
huge
challenge
to
design
featuring
simultaneous
range
sensitivity.
Herein,
typical
bilayer-conductive
structure
Ti3C2Tx
MXene/carbon
nanotubes
(CNTs)/thermoplastic
polyurethane
(TPU)
composite
film
was
developed
simple
scalable
vacuum
filtration
process
utilizing
porous
electrospun
thermoplastic
mat
as
skeleton.
MXene/CNTs/TPU
sensor
composed
two
parts:
brittle
densely
stacked
MXene
upper
lamella
flexible
MXene/CNT-decorated
fibrous
network
lower
layer.
Benefiting
from
synergetic
effect
parts
along
with
hydrogen-bonding
interactions
TPU
fiber
sheets,
possesses
both
(up
330%)
(maximum
gauge
factor
2911)
well
superb
long-term
durability
(2600
cycles
under
50%).
Finally,
can
be
successfully
employed
human
movement
monitoring,
tiny
facial
expressions,
respiration,
pulse
beat
large-scale
finger
elbow
bending,
demonstrating
promising
attractive
devices
human-machine
interaction.
InfoMat,
Journal Year:
2022,
Volume and Issue:
4(4)
Published: Feb. 22, 2022
Abstract
Wearable
electronics
offer
incredible
benefits
in
mobile
healthcare
monitoring,
sensing,
portable
energy
harvesting
and
storage,
human‐machine
interactions,
etc.,
due
to
the
evolution
of
rigid
structure
flexible
stretchable
devices.
Lately,
transition
metal
carbides
nitrides
(MXenes)
are
highly
regarded
as
a
group
thriving
two‐dimensional
nanomaterials
extraordinary
building
blocks
for
emerging
platforms
because
their
excellent
electrical
conductivity,
enriched
surface
functionalities,
large
area.
This
article
reviews
most
recent
developments
MXene‐enabled
wearable
electronics.
Several
electronic
devices
designed
on
nanometric
scale
highlighted
by
drawing
attention
widely
developed
nonstructural
attributes,
including
3D
configured
devices,
textile
planer
substrates,
bioinspired
structures,
printed
materials.
Furthermore,
unique
progress
these
nanodevices
is
representative
applications
healthcare,
energy,
electromagnetic
interference
(EMI)
shielding,
humanoid
control
machines.
The
prospects
MXene
key
frontier
next‐generation
envisioned
design
challenges
systems
also
discussed,
followed
proposed
solutions.
image
Nature Communications,
Journal Year:
2022,
Volume and Issue:
13(1)
Published: Sept. 9, 2022
Abstract
Wearable
strain
sensors
that
detect
joint/muscle
changes
become
prevalent
at
human–machine
interfaces
for
full-body
motion
monitoring.
However,
most
wearable
devices
cannot
offer
customizable
opportunities
to
match
the
sensor
characteristics
with
specific
deformation
ranges
of
joints/muscles,
resulting
in
suboptimal
performance.
Adequate
design
is
highly
required
achieve
user-designated
working
windows
without
sacrificing
high
sensitivity,
accompanied
real-time
data
processing.
Herein,
Ti
3
C
2
T
x
MXene
modules
are
fabricated
in-sensor
machine
learning
(ML)
models,
either
functioning
via
wireless
streaming
or
edge
computing,
classifications
and
avatar
reconstruction.
Through
topographic
on
piezoresistive
nanolayers,
exhibited
ultrahigh
sensitivities
within
meet
all
joint
ranges.
By
integrating
a
ML
chip,
an
module
fabricated,
enabling
reconstruction
high-precision
animations
mimic
continuous
motions
average
determination
error
3.5
cm,
additional
computing
devices.
Nano-Micro Letters,
Journal Year:
2022,
Volume and Issue:
14(1)
Published: April 11, 2022
Delayed
diagnosis
of
cancer
using
conventional
diagnostic
modalities
needs
to
be
addressed
reduce
the
mortality
rate
cancer.
Recently,
2D
nanomaterial-enabled
advanced
biosensors
have
shown
potential
towards
early
The
high
surface
area,
functional
groups
availability,
and
excellent
electrical
conductivity
MXene
make
it
material
choice
for
fabrication
electrochemical
disease
diagnostics.
MXene-enabled
aptasensors
great
promise
detection
biomarkers
with
a
femtomolar
limit
detection.
Additionally,
stability,
ease
synthesis,
good
reproducibility,
specificity
offered
by
hold
mainstream
approach.
In
this
review,
design
MXene-based
been
discussed.
Besides,
various
synthetic
processes
useful
properties
MXenes
which
can
tuned
optimized
easily
efficiently
fabricate
sensitive
elucidated.
Further,
futuristic
sensing
applications
along
challenges
will
deliberated
herein.
Advanced Functional Materials,
Journal Year:
2023,
Volume and Issue:
33(44)
Published: July 7, 2023
Abstract
Electronic
skins
(E‐skins)
capable
of
biomechanical/bioelectrical
signal
acquisition
are
intensively
pursued
for
human‐centered
healthcare
daily
life.
For
practical
use,
it
is
highly
desired,
yet
challenging,
to
mass‐produce
E‐skins
that
soft
and
breathable
wearing
comfort,
skin‐adhesive
robust
acquisition,
multi‐signal
sensing
enhanced
data.
Herein,
a
scalable
fabrication
strategy
bioinspired
E‐skin
(SPRABE‐skin)
with
multi‐layered
architecture
reported
integrates
skin‐like
softness,
self‐protection,
self‐adhesion,
breathability,
bimodal
in
single
patch.
The
fibrous
thermoplastic
polyurethane
(TPU)
scaffold
endows
the
SPRABE‐skin
tissue‐like
softness
(Young's
modulus
3.36
MPa)
stretchability,
good
permeability
water
vapor,
self‐protection
against
adverse
loading
events.
A
strain
layer
composed
MXene‐carbon
nanotubes@TPU
(MXene‐CNT@TPU)
composition
exhibits
ultra‐high
sensitivity
wide
range
(gauge
factor
at
485%
reaches
63
494).
An
electrode
made
MXene‐waterborne
(MXene‐WPU)
provides
adhesive
electrode‐skin
interface,
which
enables
biopotentials,
such
as
electrocardiograph
(ECG),
electromyograph
(EMG),
electroencephalo‐graph
(EEG),
improved
fidelity
even
under
various
dynamic
interferences.
Finally,
based
system
demonstrated
realizes
wireless,
long‐duration,
monitoring
ECG
running
activities.
Advanced Materials Technologies,
Journal Year:
2022,
Volume and Issue:
8(1)
Published: Sept. 15, 2022
Abstract
Flexible
strain
sensors
have
received
widespread
attention
because
of
their
great
potential
in
many
fields.
Carbon
nanotubes
(CNTs)
been
used
as
conductive
materials
for
flexible
due
to
excellent
electrical
and
mechanical
properties,
the
fabricated
sensing
performance.
This
paper
systematically
summarizes
advances
resistance‐type
based
on
CNTs.
The
mechanisms
are
introduced,
including
crack
extension,
tunneling
effect,
disconnection
overlapping
materials.
performance
parameters
sensors,
sensitivity,
stretchability,
linearity,
hysteresis,
dynamic
durability,
transparency,
discussed
comprehensively.
coating
methods,
3D
printing
techniques,
chemical
vapor
deposition,
transfer
spinning
processes
fabricate
CNT
highlighted.
effect
isolated
porous
internal
structures,
folded
microcracked
surface
films
fabrics
macroscopic
structures
sensor
were
analyzed.
applications
medical
health,
motion
monitoring,
gesture
recognition,
human–computer
interaction,
soft
robotics
provided
detail.
Finally,
future
challenges
summarized
outlook
is
presented.
Although
made
progress
so
far,
there
still
problems
that
need
researchers’
solutions.
Advanced Materials,
Journal Year:
2023,
Volume and Issue:
35(13)
Published: Jan. 5, 2023
Mechanically
stretchable
strain
sensors
gain
tremendous
attention
for
bioinspired
skin
sensation
systems
and
artificially
intelligent
tactile
sensors.
However,
high-accuracy
detection
of
both
intensity
direction
with
simple
device/array
structures
is
still
insufficient.
To
overcome
this
limitation,
an
omnidirectional
perception
platform
utilizing
a
sensor
array
triangular-sensor-assembly
(three
tilted
by
45°)
coupled
machine
learning
(ML)
-based
neural
network
classification
algorithm,
proposed.
The
sensor,
which
constructed
strain-insensitive
electrode
regions
strain-sensitive
channel
region,
can
minimize
the
undesirable
electrical
intrusion
from
electrodes
strain,
leading
to
heterogeneous
surface
structure
more
reliable
sensing
characteristics.
exhibits
decent
sensitivity
gauge
factor
(GF)
≈8,
moderate
range
(≈0-35%),
relatively
good
reliability
(3000
stretching
cycles).
More
importantly,
employing
multiclass-multioutput
behavior-learned
cognition
highly
accurate
recognition
arbitrary
interpretating
correlated
signals
three-unit
its
algorithm
overall
accuracy
around
98%
±
2%
over
≈0-30%
in
various
stimuli
environments.