Fragmentation engineering on the edge of hydroxy-functional COFs for the enhanced photocatalytic production of H2O2 and direct photo-oxidation of benzene to phenol in aqueous systems DOI
Shijian Zhou, Yuexin Shi, Guangyuan Chen

et al.

Chemical Engineering Journal, Journal Year: 2023, Volume and Issue: 477, P. 146946 - 146946

Published: Oct. 27, 2023

Language: Английский

Anthraquinones-based photocatalysis: A comprehensive review DOI Creative Commons
Cheng-Xin Chen, Shan-Shan Yang,

Ji-Wei Pang

et al.

Environmental Science and Ecotechnology, Journal Year: 2024, Volume and Issue: 22, P. 100449 - 100449

Published: July 5, 2024

In recent years, there has been significant interest in photocatalytic technologies utilizing semiconductors and photosensitizers responsive to solar light, owing their potential for energy environmental applications. Current efforts are focused on enhancing existing photocatalysts developing new ones tailored uses. Anthraquinones (AQs) serve as redox-active electron transfer mediators photochemically active organic photosensitizers, effectively addressing common issues such low light utilization carrier separation efficiency found conventional semiconductors. AQs offer advantages abundant raw materials, controlled preparation, excellent capabilities, photosensitivity, with applications spanning the energy, medical, sectors. Despite utility, comprehensive reviews AQs-based systems contexts lacking. this review, we thoroughly describe photochemical properties of photocatalysis, particularly key challenges like clean production, antibacterial action, pollutant degradation. However, face limitations practical due electrical conductivity solubility-related secondary contamination. To mitigate these issues, design synthesis graphene-immobilized highlighted a solution enhance Additionally, future research directions proposed deepen understanding AQs' theoretical mechanisms provide wastewater treatment. This review aims facilitate mechanistic studies improve technologies.

Language: Английский

Citations

9

Antibacterial Evaporator Based on Wood-Reduced Graphene Oxide/Titanium Oxide Nanocomposite for Long-Term and Highly Efficient Solar-Driven Wastewater Treatment DOI
Roya Mehrkhah, Mojtaba Mohammadi,

Alireza Zenhari

et al.

Industrial & Engineering Chemistry Research, Journal Year: 2022, Volume and Issue: 62(11), P. 4573 - 4586

Published: Sept. 15, 2022

Herein, we developed antifouling and highly efficient solar absorbers consisting of poplar wood coated with titanium dioxide (TiO2) reduced graphene oxide (RGO) nanocomposites (with different weight ratio TiO2 to RGO). The antibacterial activity all prepared against Staphylococcus aureus (S. aureus) Escherichia coli (E. coli) was investigated. results showed that T2G1 (a nanocomposite in which the RGO is 2:1) has highest among (MIC 0.08 mg mL–1 MBC 0.6 0.8 for E. S. aureus, respectively). Therefore, it considered be most photothermal material interfacial desalination solar-driven treatment wastewater. Because broad-band absorption by T2G1, absorber composed (denoted as T2G1-w) a high energy conversion efficiency 90.12% under 1 sun (1 kW m–2). T2G1-w also had stability long-term cycles. great performance freshwater production from contaminated water containing dye or heavy metals. concentration metals Zn2+, Pb2+, Fe2+, Ni2+, Cr6+ 1000 L–1 near zero presence absorber, indicating its potential application sewage treatment.

Language: Английский

Citations

36

Sustainable fabrication of Co-MOF@CNT nano-composite for efficient adsorption and removal of organic dyes and selective sensing of Cr(VI) in aqueous phase DOI

Khalil M. A. Qasem,

Shabnam Khan, Sampath Chinnam

et al.

Materials Chemistry and Physics, Journal Year: 2022, Volume and Issue: 291, P. 126748 - 126748

Published: Sept. 14, 2022

Language: Английский

Citations

31

Constructing an ultrastable imidazole covalent organic framework for concurrent uranium detection and recovery DOI Creative Commons
Wei‐Rong Cui, Wei Xu, Weibin Qiu

et al.

Ecotoxicology and Environmental Safety, Journal Year: 2023, Volume and Issue: 252, P. 114639 - 114639

Published: Feb. 13, 2023

Uranium is one of the most important strategic resources for development nuclear industry, but its unintended release has created potential environmental and health risks. It highly desired to explore new methods that enable concurrent uranium monitoring recovery protection sustainable industry. Here, first time, an imidazole fluorescent covalent organic framework (named PyTT-Tp) with ultrastable skeleton open nanopore channel synthesized by condensing ammonium acetate, 1,3,5-triformylphloroglucinol pyrene-4,5,9,10-tetrone. By precisely tailoring complexing ligands, PyTT-Tp shows excellent capacity 941.27 mg g-1 reached equilibrium within 60 min, which can be attributed dense selective binding sites on accessible skeleton. In addition, due signal amplification pyrene-imidazole skeleton, it ultra-low detection limit 4.92 nM UO22+ ultra-fast response time (2 s) suitable on-site content extracted water. modulating target this approach extended other nuclides.

Language: Английский

Citations

22

Fragmentation engineering on the edge of hydroxy-functional COFs for the enhanced photocatalytic production of H2O2 and direct photo-oxidation of benzene to phenol in aqueous systems DOI
Shijian Zhou, Yuexin Shi, Guangyuan Chen

et al.

Chemical Engineering Journal, Journal Year: 2023, Volume and Issue: 477, P. 146946 - 146946

Published: Oct. 27, 2023

Language: Английский

Citations

22