Highly efficient solar water evaporation by wood through one-step in-situ synthesis of carbon dots DOI Creative Commons
Chunyu Ji, Ting Wang, Yifeng Wang

et al.

Chemical Engineering Journal, Journal Year: 2023, Volume and Issue: 479, P. 147680 - 147680

Published: Dec. 3, 2023

Solar evaporation provides an effective solution to solve the scarcity of freshwater resources. Biomass-based solar evaporators have attracted significant interest, because their environmental safety. However, due high latent heat for water, most biomass-based exhibit low water vapor generation rates. In this work, we developed a wood-based evaporator (CDs-Wood) by just one step in-situ synthesis carbon dots (CDs) using lignin in wood as source, and CDs-Wood has significantly decreased from 2257.5 J g­1 1003.8 g­1, which resulted rate 2.86 kg m­2 h­1. exhibits extensive optical absorption capacity (95.3 %), steam conversion efficiency (80 adaptability low-temperature conditions, excellent salt resistance. This work efficient potentially scalable designing all-biomass-based evaporators.

Language: Английский

Recent advances in the design of afterglow materials: mechanisms, structural regulation strategies and applications DOI
Xin Yang, Geoffrey I. N. Waterhouse, Siyu Lu

et al.

Chemical Society Reviews, Journal Year: 2023, Volume and Issue: 52(22), P. 8005 - 8058

Published: Jan. 1, 2023

Afterglow materials have attracted widespread attention owing to their distinctive and long-lived optical emission properties which create exciting opportunities in various fields.

Language: Английский

Citations

177

Rational Design of Covalent Bond Engineered Encapsulation Structure toward Efficient, Long‐Lived Multicolored Phosphorescent Carbon Dots DOI
Yongqiang Zhang, Manyu Li, Siyu Lu

et al.

Small, Journal Year: 2022, Volume and Issue: 19(31)

Published: Nov. 27, 2022

Multicolored phosphorescent materials based on carbon dots (CDs) constructed using the same or similar precursors with long lifetimes are conducive to their wide range of practical applications due developed compatibility. Herein, a universal method is prepare long-lived multicolored CD-based composites for which heavy-metal doping not required. The CDs encapsulated in silica via silane hydrolysis, forms many covalent SiOC and SiC bonds; hence, vibrations rotations luminescent centers CD surfaces hindered. transformation more rigid moiety occurs during high-temperature calcination. Furthermore, calcination, collapses, resulting tightly CDs. synergistic effect these two calcination phenomena produces blue, green, yellow, red phosphorescence, at wavelengths spanning 465 680 nm up 2.11 s. Taking advantage superior phosphorescence performances, successfully applied 3D multichannel information storage encryption.

Language: Английский

Citations

74

Evolution and fabrication of carbon dot-based room temperature phosphorescence materials DOI Creative Commons
Jiurong Li, Yongzhong Wu, Xiao Gong

et al.

Chemical Science, Journal Year: 2023, Volume and Issue: 14(14), P. 3705 - 3729

Published: Jan. 1, 2023

Carbon dot-based room temperature phosphorescence materials are reported, mainly focusing on the outstanding contributions over years, emission, lifetime, preparation and application.

Language: Английский

Citations

74

Long‐Lived Dynamic Room Temperature Phosphorescence from Carbon Dots Based Materials DOI
Kaiti Wang, Lunjun Qu, Chaolong Yang

et al.

Small, Journal Year: 2023, Volume and Issue: 19(31)

Published: Jan. 6, 2023

Abstract As a type of room temperature phosphorescence (RTP) material, carbon dots (CDs) always show short lifetime and low efficiency. To counter these disadvantages, several strategies, such as embedding in rigid matrix, introducing heteroatom, crosslink‐enhanced emission, etc., are well developed. Consequently, lots CDs‐based RTP materials obtained. Doping CDs into various matrix is the dominant method for preparation long‐lived so far. The desired CDs@matrix composites display outstanding performances. Meanwhile, matrix‐free carbonized polymer dots‐based also widely Amounts possessing ultra‐long lived, multiple colored, dynamic emission successfully Herein, recent progress achieved corresponding efficient strategies mechanisms summarized reviewed detail. Due to possess excellent chemical stability, photostability biological toxicity, they exhibit great application potential fields anti‐counterfeiting, data encryption, monitoring. introduced this review. promising functional development long wavelength emitting with still challengeable, especially red near‐infrared materials.

Language: Английский

Citations

73

Recent Advances of Carbon Dots with Afterglow Emission DOI
Huixian Shi, Yang Wu, Jiahui Xu

et al.

Small, Journal Year: 2023, Volume and Issue: 19(31)

Published: Feb. 21, 2023

Abstract Carbon dots (CDs) have gradually become a new generation of nano‐luminescent materials, which received extensive attention due to excellent optical properties, wide source raw low toxicity, and good biocompatibility. In recent years, there are many reports on the luminescent phenomenon CDs, great progress has been achieved. However,there rarely systematic summaries CDs with persistent luminescence. Here, summary including luminous mechanism, synthetic strategies, property regulation, potential applications, is given. First, brief introduction given development materials. Then, mechanism afterglow from room temperature phosphorescence (RTP), delayed fluorescence (DF), long luminescence (LPL) discussed. Next, constructed methods materials summarized two aspects, matrix‐free self‐protected matrix‐protected CDs. Moreover, regulation properties color, lifetime, efficiency presented. Afterwards, applications such as anti‐counterfeiting, information encryption, sensing, bio‐imaging, multicolor display, LED devices, etc., reviewed. Finally, an outlook proposed.

Language: Английский

Citations

69

Polymer–Structure‐Induced Room‐Temperature Phosphorescence of Carbon Dot Materials DOI Creative Commons
Chengyu Zheng,

Songyuan Tao,

Bai Yang

et al.

Small Structures, Journal Year: 2023, Volume and Issue: 4(5)

Published: Feb. 2, 2023

As emerging carbon‐based nanomaterials, carbon dots (CDs) are widely studied with regard to their luminescent properties. CDs obtained by the bottom‐up method exhibit polymeric characteristics after crosslinking, polymerization, and incomplete carbonization processes, herein referred as carbonized polymer (CPDs). In recent years, large progress has been achieved on room‐temperature phosphorescence (RTP) properties of CPDs. The developments synthesis strategies for RTP CPD materials reviewed. However, less attention devoted influence structures materials. Polymer a common feature extensive key factors facilitating Herein, effects emission self‐protective matrix‐assisted discussed. It is considered that can effectively immobilize subluminophores protect triplet excited states facilitate crosslink‐enhanced (CEE) effect proposed further explain materials, which provide an effective strategy Benefiting from CEE effect, efficient be applications then briefly summarized.

Language: Английский

Citations

62

Time‐dependent Phosphorescence Color of Carbon Dots in Binary Salt Matrices through Activations by Structural Confinement and Defects for Dynamic Information Encryption DOI
Wenying Shi, Ruixing Wang, Jing Liu

et al.

Angewandte Chemie International Edition, Journal Year: 2023, Volume and Issue: 62(23)

Published: April 6, 2023

The emergence of time-dependent phosphorescence color (TDPC) materials has taken information encryption to high-security levels. However, due the only path exciton transfer, it is almost impossible obtain TDPC for chromophores with a single emission center. Theoretically, in inorganic-organic composites, transfer organic depends on inorganic structure. Here, we assign two structural effects NaCl by metal (Mg2+ or Ca2+ Ba2+ ) doping, which triggers performance carbon dots (CDs) resulting material used multi-level dynamic 3D coding achieve encryption. confinement activates green CDs; while defect tunneling-related yellow phosphorescence. Such simply doped matrices can be synthesized using periodic table cations, endowing tremendous control over properties. This demonstration extends design view luminescent materials.

Language: Английский

Citations

60

Aggregation-induced color fine-tunable carbon dot phosphorescence covering from green to near-infrared for advanced information encryption DOI
Qijun Li,

Dengke Cheng,

Hailing Gu

et al.

Chemical Engineering Journal, Journal Year: 2023, Volume and Issue: 462, P. 142339 - 142339

Published: March 9, 2023

Language: Английский

Citations

53

Application of room-temperature phosphorescent carbon dots in information encryption and anti-counterfeiting DOI
Linlin Shi,

Luyao Ding,

Yongqiang Zhang

et al.

Nano Today, Journal Year: 2024, Volume and Issue: 55, P. 102200 - 102200

Published: Feb. 13, 2024

Language: Английский

Citations

52

Phosphorescent carbon dots: Intermolecular interactions, properties, and applications DOI
Jie Li, Zhou Heng, Hao Qiu

et al.

Coordination Chemistry Reviews, Journal Year: 2024, Volume and Issue: 503, P. 215642 - 215642

Published: Jan. 2, 2024

Language: Английский

Citations

33