Experimental Study on Early Fire Smoke Characteristics in a High-Volume Space: A Fire Detection Perspective DOI Creative Commons
Li Wang, Xi Zhang, Liming Li

et al.

Fire, Journal Year: 2024, Volume and Issue: 7(9), P. 298 - 298

Published: Aug. 23, 2024

High-volume space structures are characterized by high combustible loads, rapid fire development, difficulty in firefighting, and potential building collapse risks, making early detection particularly crucial. The effectiveness of technologies relies on their ability to adapt the characteristics smoke-dominant combustion products protected space. However, there is a lack targeted research smoke generated during low-power stages fires high-volume spaces, which has not supported development for such environments. To address this, this paper presents an experimental study that, first time, collects data parameters as temperature, velocity, concentration, particle size at heights ranging from 6.5 m 18.5 using lightweight sensors. analyzes characteristic correlations these impact spaces presenting variation patterns plume velocity distribution with height. It identifies three distribution, contrasting previous studies, offers qualitative explanation findings. This enhances understanding signals large valuable insights developing more accurate efficient strategies technologies.

Language: Английский

Microphysical properties of atmospheric soot and organic particles: measurements, modeling, and impacts DOI Creative Commons
Weijun Li, Nicole Riemer, Liang Xu

et al.

npj Climate and Atmospheric Science, Journal Year: 2024, Volume and Issue: 7(1)

Published: March 8, 2024

Abstract Atmospheric soot and organic particles from fossil fuel combustion biomass burning modify Earth’s climate through their interactions with solar radiation modifications of cloud properties by acting as condensation nuclei ice nucleating particles. Recent advancements in understanding individual microscopic composition have led to heightened interest microphysical properties. This review article provides an overview current advanced measurements offers insights into future avenues for studying these To quantify morphology ageing, fractal dimension ( D f ) is a commonly employed quantitative metric which allows characterize morphologies aggregates relation ageing factors like internal mixing state, core-shell structures, phase, heterogeneity. Models been developed incorporate diversity metrics aged particles, enabling assessment optical absorption radiative forcing effects. The are complex they influenced particle sources, process, meteorological conditions. Furthermore, soluble exhibit diverse forms can engage liquid–liquid phase separation sulfate nitrate components. Primary carbonaceous such tar balls warrant further attention due strong light absorbing properties, presence toxic constituents, small size, impact human health. Future research needs include both atmospheric modeling approaches, focusing on changes the structures ensembles, effects dynamics

Language: Английский

Citations

24

Recent advances in soot formation mechanisms: Oxidation and oxidation-induced fragmentation DOI
Huaqiang Chu,

Run Hong,

Wenlong Dong

et al.

Fuel, Journal Year: 2024, Volume and Issue: 371, P. 132046 - 132046

Published: June 1, 2024

Language: Английский

Citations

21

Effective density of inhaled environmental and engineered nanoparticles and its impact on the lung deposition and dosimetry DOI Creative Commons
Denisa Lizoňová,

Amogh Nagarkar,

Philip Demokritou

et al.

Particle and Fibre Toxicology, Journal Year: 2024, Volume and Issue: 21(1)

Published: Feb. 17, 2024

Airborne environmental and engineered nanoparticles (NPs) are inhaled deposited in the respiratory system. The dose of such NPs their deposition location lung determines impact on health. When calculating NP using particle inhalation models, a common approach is to use bulk material density, ρ

Language: Английский

Citations

11

Validation of cantilever-enhanced photoacoustic particle-size-resolved light absorption measurement using nigrosin reference particles and Mie modelling DOI Creative Commons
Joel Kuula, Juho Karhu, Tommi Mikkonen

et al.

Aerosol Research, Journal Year: 2025, Volume and Issue: 3(1), P. 1 - 13

Published: Jan. 13, 2025

Abstract. Particle light absorption enhancement, also known as the lensing effect, is a complex phenomenon where particles undergo optical transformation they age. This process influenced by several factors, including particle size. To investigate this study introduces and validates novel method for size-resolved measurements using nigrosin model system. The combines three-wavelength cantilever-enhanced photoacoustic spectrometer (CEPAS) with differential mobility analyser (DMA) to achieve particle-size-resolved measurements. Nigrosin, well-characterised, spherically shaped, water-soluble material, was selected demonstrate feasibility precision of approach. system showed strong agreement (R2>0.94) Mie-modelled absorption, confirming its reliability. While broader motivation work lies in advancing techniques studying ageing, coating, enhancement black carbon other atmospheric aerosols, present serves foundational step validating methodology controlled simplified context. Future studies will expand application systems, coated aggregated particles, explore phenomena such enhancement.

Language: Английский

Citations

1

Simultaneous Inversion of Particle Size Distribution, Thermal Accommodation Coefficient, and Temperature of In-Flame Soot Aggregates Using Laser-Induced Incandescence DOI Open Access
Jun-You Zhang, Juqi Zhang, Xing Huang

et al.

Materials, Journal Year: 2024, Volume and Issue: 17(3), P. 634 - 634

Published: Jan. 28, 2024

Measuring the size distribution and temperature of high-temperature dispersed particles, particularly in-flame soot, holds paramount importance across various industries. Laser-induced incandescence (LII) stands out as a potent non-contact diagnostic technology for although its effectiveness is hindered by uncertainties associated with pre-determined thermal properties. To tackle this challenge, our study proposes multi-parameter inversion strategy—simultaneous particle distribution, accommodation coefficient, initial soot aggregates using time-resolved LII signals. Analyzing responses different heat transfer sub-models to rise demonstrates necessity incorporating sublimation thermionic emission accurately reproducing signals particles. Consequently, we selected particular model strategy. Our research reveals that LII-based sizing sensitive biases in particles (equivalent flame temperature), underscoring need proposed Numerical results obtained at two typical temperatures, 1100 K 1700 K, illustrate selecting an appropriate laser fluence enables simultaneous temperatures high accuracy confidence technique.

Language: Английский

Citations

4

Bayesian inversion of emissions from large urban fire using in situ observations DOI
Emilie Launay,

Virginie Hergault,

Marc Bocquet

et al.

Atmospheric Environment, Journal Year: 2024, Volume and Issue: 323, P. 120391 - 120391

Published: Feb. 5, 2024

Language: Английский

Citations

4

Effective density and packing of compacted soot aggregates DOI Creative Commons
Timothy A. Sipkens, Joel C. Corbin

Carbon, Journal Year: 2024, Volume and Issue: 226, P. 119197 - 119197

Published: April 28, 2024

The mass concentration of soot aggregates is often estimated from mobility size distributions using a mobility-based effective density, ρeff. This ρeff changes with aggregate morphology. In particular, the core increases when it becomes compacted by surface tension condensing coatings, such as combustion-related vapours, secondary aerosols, and cloud water. extent this compaction function coating volume, up to an asymptotic limit complete compaction. While has previously been shown correspond universal, scale-invariant packing factor for sufficiently large aggregates, not explicitly quantified. Here, we critically reanalyze multiple datasets compiled literature on completely compact soot. We show that, regardless material, generally become following 5-fold increase in volume. final shape more simply described than diameter or factor. Below 140 nm (about 20 monomers), obeys power law; above nm, reaches constant value 651 ± 8 kg m–3. 3 times larger that freshly-produced at nm. provide parameterization estimation after coating, or, conversely, use benchmark estimate restructuring. Our can be easily adapted other nanoparticle whose material density known.

Language: Английский

Citations

4

Theoretical and experimental validation of the aerosol electrical mobility separator electrometer DOI Creative Commons
Joshua S. Hassim, Simone Hochgreb,

Kingsley Reavell

et al.

Aerosol Science and Technology, Journal Year: 2025, Volume and Issue: unknown, P. 1 - 25

Published: Jan. 3, 2025

In this work, we introduce and validate a novel device, the Mobility Separator Electrometer (MSE). The MSE classifies particles by their electrical mobility, separating into two electrometer outlets. Automatic adjustment of voltage set-point to achieve equal currents enables autonomous measurement aerosol population's average mobility. transfer function device was experimentally validated, demonstrating good agreement with theory once calibrated for an effective length. power occurs when integrating it in tandem system involving Unipolar Diffusion Charger, upstream classifier such as Centrifugal Particle Mass Analyzer (CPMA) or Aerodynamic Aerosol Classifier (AAC) Condensation Counter (CPC). These combinations provide mass, aerodynamic diameter mobility diameter, enabling particle density. Using numerical simulations, show density various aerosols can be determined within 5% using aforementioned systems over extremely wide size range (30 nm

Language: Английский

Citations

0

Investigation of the Morphology and Composition of Aerosols from Plant Burning DOI
Bruno Martinent,

Santoni Paul-Antoine,

A. Coppalle

et al.

Published: Jan. 1, 2025

Language: Английский

Citations

0

Fractal Scaling in the Gas‐Phase Agglomeration of Nanowires DOI Open Access
Nabil Abomailek,

Isabel Gómez‐Palos,

Cristian Carnicero

et al.

Small, Journal Year: 2025, Volume and Issue: unknown

Published: Feb. 5, 2025

Abstract Assembling 1D nanoparticles (nanowires (NW) or nanotubes) as networks enables bridging multiple scales to form macroscopic materials such fibers, sheets and electrodes. This can be done directly in the gas phase from nanoparticle aerosols grown by floating catalyst chemical vapor deposition (FCCVD). In FCCVD nanowires/nanotubes grow high aspect ratios (10 2 –10 6 ) a stream agglomerate an aerogel. work studies agglomeration of Si nanowires scanning electron microscopy samples taken downstream reaction zone, through simulations with Brownian collision algorithm models. experimental analysis over 312 no individualized NWs are found, only agglomerates. is consistent fast binary rates 0.24 s estimated. The agglomerates show “fractal” scaling, fractional dimension D f 1.8 size increasing number power 1/D , diffusion limited cluster aggregation process. Formation nanowire aerogel involves percolation agglomerates, therefore occurring at much lower volume fraction than for particles considering excluded theory. Compared carbon nanotubes higher ratio, these SiNWs require longer residence time gelation.

Language: Английский

Citations

0