Inorganic Chemistry Communications, Journal Year: 2024, Volume and Issue: unknown, P. 113176 - 113176
Published: Sept. 1, 2024
Language: Английский
Inorganic Chemistry Communications, Journal Year: 2024, Volume and Issue: unknown, P. 113176 - 113176
Published: Sept. 1, 2024
Language: Английский
Science China Materials, Journal Year: 2024, Volume and Issue: 67(2), P. 484 - 492
Published: Jan. 12, 2024
Language: Английский
Citations
38Small, Journal Year: 2024, Volume and Issue: unknown
Published: Oct. 3, 2024
Abstract Graphitic carbon nitride (gC 3 N 4 ) is an attractive photocatalyst for solar energy conversion due to its unique electronic structure and chemical stability. However, gC generally suffers from insufficient light absorption rapid compounding of photogenerated charges. The introduction defects atomic doping can optimize the improve carrier separation efficiency. Herein, high efficiency photocatalysis hydrogen evolution in visible achieved by S‐modified double‐deficient site strategy. Defect engineering forms abundant unsaturated sites cyano (─C≡N), which promotes strong interlayer C─N bonding interactions accelerates charge transport . S tunes semiconductors, formation C─S─C bonds optimizes electron‐transfer paths bonding, enhances light. Meanwhile,C≡N acts as electron trap capture photoexcited electrons, providing active reduction H + hydrogen. photocatalytic SDCN (1613.5 µmol g −1 h 31.5 times higher than that pristine MCN (51.2 ). situation transfer mechanism photocatalysts are investigated detail a combination experimental theoretical calculations.
Language: Английский
Citations
10Journal of Colloid and Interface Science, Journal Year: 2023, Volume and Issue: 657, P. 309 - 319
Published: Nov. 23, 2023
Language: Английский
Citations
19ACS Catalysis, Journal Year: 2024, Volume and Issue: unknown, P. 15444 - 15455
Published: Oct. 3, 2024
Language: Английский
Citations
8Applied Catalysis B Environment and Energy, Journal Year: 2024, Volume and Issue: unknown, P. 124879 - 124879
Published: Nov. 1, 2024
Language: Английский
Citations
7Small, Journal Year: 2024, Volume and Issue: 20(45)
Published: Aug. 18, 2024
Graphitic carbon nitride (g-C
Language: Английский
Citations
6Applied Surface Science, Journal Year: 2024, Volume and Issue: 660, P. 160018 - 160018
Published: March 30, 2024
Language: Английский
Citations
5Surfaces and Interfaces, Journal Year: 2025, Volume and Issue: unknown, P. 105844 - 105844
Published: Jan. 1, 2025
Language: Английский
Citations
0Advanced Science, Journal Year: 2025, Volume and Issue: unknown
Published: March 5, 2025
Artificial photosynthesis for producing high-value hydrogen peroxide (H2O2) using carbon nitride-based systems holds immense potential. However, understanding the charge transfer dynamics in homojunction photocatalysts remains a significant challenge owing to limitations of current characterization techniques. Here, polymeric C3N5/C3N4 (CNHJ) is employed as model system probe interfacial electron transfer. Bimetallic cocatalysts serve sensitive probes, enabling situ tracking S-scheme between C3N5 and C3N4 via X-ray photoelectron spectroscopy. Leveraging unique advantages this S-scheme, CNHJ demonstrates substantially enhanced performance two-electron oxygen reduction reaction, achieving an impressive H2O2 production rate 8.78 mmol g-1 h-1 under visible light irradiation. Furthermore, robust continuous-flow setups, natural sunlight, photocatalytic disinfection tests, highlighting its practical This approach offers new insights into dynamic mechanisms paves way advancing artificial technologies.
Language: Английский
Citations
0Journal of Material Science and Technology, Journal Year: 2025, Volume and Issue: unknown
Published: March 1, 2025
Language: Английский
Citations
0