Development of compatible photocatalyst-enzyme hybrid system via Intensifying enzyme tolerance for enhanced chiral alcohol synthesis DOI
Chun-Xian Cai,

Zi‐Wen Zhou,

Chunxiu Liu

et al.

Journal of Catalysis, Journal Year: 2024, Volume and Issue: unknown, P. 115932 - 115932

Published: Dec. 1, 2024

Language: Английский

In situ NADH regeneration coupled to enzymatic CO2 reduction: from fundamental concepts to recent advances DOI
Neha Gupta, Arpita Sarkar, Soumya Kanti Biswas

et al.

Journal of environmental chemical engineering, Journal Year: 2025, Volume and Issue: unknown, P. 116657 - 116657

Published: April 1, 2025

Language: Английский

Citations

0
Constructing Cu2+ active sites on pyrazole-decorated UiO-66-NH2 with high activity for photocatalytic CO2 reduction to HCOO− DOI

Xin Chen,

Ya‐Yu Zhao,

Meng-Qiang Deng

et al.

Materials Today Chemistry, Journal Year: 2025, Volume and Issue: 46, P. 102712 - 102712

Published: April 19, 2025

Language: Английский

Citations

0
Designing biomimetic catalytic systems for CO2 reduction to formate using NAD(P)H DOI

Chan-Woo Park,

Chul Han Kwon,

Young Hyun Hong

et al.

Inorganic Chemistry Frontiers, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 1, 2025

This review article focuses on current achievements and identifies future research directions by designing biomimetic catalytic systems for CO 2 reduction to formate using NAD(P)H.

Language: Английский

Citations

0
Nonporous and porous silica-polyethylene composite membrane attached FDH for carbon dioxide conversion to formate and its application in a photo-enzyme coupled system DOI
Shutao Gao, Qiyong Liao, Ruqing Chong

et al.

Separation and Purification Technology, Journal Year: 2025, Volume and Issue: unknown, P. 131656 - 131656

Published: Jan. 1, 2025

Language: Английский

Citations

0
Rh-functionalized Imino-pyridine Covalent Organic Framework Assembled on Ti3C2Tx (MXene) for Efficient NADH Regeneration and Photoenzymatic CO2 Reduction DOI

Hailong Zheng,

Zhipeng Huang,

Ping Wei

et al.

ACS Sustainable Chemistry & Engineering, Journal Year: 2025, Volume and Issue: unknown

Published: March 4, 2025

Nicotinamide adenine dinucleotide (NADH) regeneration is crucial for sustainable enzymatic CO2 reduction. In this study, Ti3C2Tx (MXene) and [Cp*Rh(bpy)(H2O)]2+ (labeled as [Cp*Rh]) were sequentially assembled onto imino-pyridine structured covalent organic frameworks (TD-COF) to construct Rh@TDM photocatalysts with dual cocatalyst. The photoelectrochemical tests temperature-dependent photoluminescence spectra suggest that the synergistic effect of incorporation [Cp*Rh] immobilization enables a reduction in exciton binding energy promotes carrier transfer. Consequently, optimized [email protected] photocatalyst achieves 95.0% NADH yield, significantly higher than TD-COF free (32.7%). Additionally, modification strategy applied also enhances selectivity 1,4-NADH. Therefore, turnover frequency 1,4-NADH 1.06 h–1, which 7.1 times (0.15 h–1). Subsequently, photoenzymatic cascade catalytic system, obtained remarkable formate generation rate 2137.7 μmol g–1 h–1. This work not only provides novel example using COF containing an structure immobilize but reveals synergetic MXene facilitates These findings offer new insights opportunities design application artificial systems

Language: Английский

Citations

0
Protein aggregates facilitated by polar aprotic solvents as carriers for enzyme immobilization DOI
Yitong Wang,

Huazong Liu,

Yan Chu

et al.

International Journal of Biological Macromolecules, Journal Year: 2025, Volume and Issue: 307, P. 142164 - 142164

Published: March 15, 2025

Language: Английский

Citations

0
Highly efficient photoenzymatic CO2 reduction via integrated structural design of porphyrin covalent organic framework on Ti3C2T (MXene) DOI
Zhipeng Huang, Shuli Bai,

Ping Wei

et al.

Separation and Purification Technology, Journal Year: 2025, Volume and Issue: unknown, P. 132943 - 132943

Published: April 1, 2025

Language: Английский

Citations

0
Highly efficient photoenzymatic CO2 reduction dominated by 2D/2D MXene/C3N5 heterostructured artificial photosynthesis platform DOI
Fengyi Yang,

Pengye Zhang,

Jiafu Qu

et al.

Journal of Colloid and Interface Science, Journal Year: 2024, Volume and Issue: 678, P. 1121 - 1131

Published: Aug. 22, 2024

Language: Английский

Citations

3
Electron-mediator-free efficient photocatalytic regeneration of coenzyme NAD(P)H via direct electron transfer using ultrathin Bi2MoO6 nanosheets DOI
Yao Chai,

Zirui Pang,

Heng Jiang

et al.

Green Chemistry, Journal Year: 2024, Volume and Issue: 27(3), P. 623 - 632

Published: Nov. 12, 2024

The direct electron transfer mechanism of single-layer Bi 2 MoO 6 ultrathin nanosheets promotes the efficient regeneration photocatalytic coenzyme NAD(P)H.

Language: Английский

Citations

1
Development of Compatible Photocatalyst-Enzyme Hybrid System Via Intensifying Enzyme Tolerance for Enhanced Chiral Alcohol Synthesis DOI
Chun-Xian Cai,

Zi‐Wen Zhou,

Chunxiu Liu

et al.

Published: Jan. 1, 2024

Language: Английский

Citations

0