Efficient Removal of Tetracyclines and Quinolones Enabled by Polyphenol-Mediated Supramolecular Coagulation DOI
Mengyue Wang, Yu Wang,

Nanjiong Pang

et al.

Langmuir, Journal Year: 2024, Volume and Issue: unknown

Published: Feb. 6, 2024

Ubiquitous antibiotics threaten human health and ecosystem sustainability, existing removal strategies, especially conventional multistep water treatments, are primarily limited by the antibiotic-specific capability. Here, we explore natural biomass, plant polyphenols, in capture of various with a facile treatment─polyphenol-mediated antibiotic-independent supramolecular coagulation (PMAC). The PMAC shows superior performance removing five tetracyclines quinolones (up to 98.54%), even under complex environmental parameters, including different pH, presence inorganic particles ionic strength, colloid-associated contaminants. Our mechanistic studies suggested that is capable exerting multiple molecular interactions antibiotics, coordination-driven self-assembly further destabilizes phenolic–antibiotic nanocomplexes, enabling an coagulation. Collectively, combination efficient remediation inexpensive biomass suggests simple scalable method for sustainable antibiotics. strategy great promise as cost-effective, approach eliminate being integrated into currently treatment systems.

Language: Английский

Occurrence and Distribution of Antibiotics in the Water, Sediment, and Biota of Freshwater and Marine Environments: A Review DOI Creative Commons

Zeinab Maghsodian,

Ali Mohammad Sanati, Tebogo Mashifana

et al.

Antibiotics, Journal Year: 2022, Volume and Issue: 11(11), P. 1461 - 1461

Published: Oct. 23, 2022

Antibiotics, as pollutants of emerging concern, can enter marine environments, rivers, and lakes endanger ecology human health. The purpose this study was to review the studies conducted on presence antibiotics in water, sediments, organisms aquatic environments (i.e., seas, lakes). Most reviewed were 2018 (15%) 2014 (11%). Antibiotics reported aqueous media at a concentration <1 ng/L−100 μg/L. results showed that highest number works Asian continent (seas: 74%, rivers: 78%, lakes: 87%, living organisms: 100%). water sea with frequency 49%, related fluoroquinolones. According results, amounts sediment 460 ng/L 406 ng/g, respectively. In sulfonamides had abundance (30%). Fluoroquinolones (with an 34%) lakes. Moreover, fluoroquinolones 68,000 39%. obtained it be concluded are among most dangerous due their high concentrations environment. This provides timely information regarding different which helpful for estimating ecological risks, contamination levels, management.

Language: Английский

Citations

100

Interfacial Si–O–Zr bonds induced well dispersed zirconia on magnetic mesoporous silicas for enhanced tetracycline removal DOI

Lijia Xie,

Tan Ying,

Yu-Qiu Ke

et al.

Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: 486, P. 150243 - 150243

Published: March 7, 2024

Language: Английский

Citations

26

Antibiotic-contaminated wastewater treatment and remediation by electrochemical advanced oxidation processes (EAOPs) DOI Creative Commons

Foysal Mahmud,

Tabassum Sunjida Banhi, Hridoy Roy

et al.

Groundwater for Sustainable Development, Journal Year: 2024, Volume and Issue: 25, P. 101181 - 101181

Published: April 26, 2024

Language: Английский

Citations

20

Antibiotic occurrence, environmental risks, and their removal from aquatic environments using microalgae: Advances and future perspectives DOI
Tufail Fayaz,

Nirmal Renuka,

Sachitra Kumar Ratha

et al.

Chemosphere, Journal Year: 2023, Volume and Issue: 349, P. 140822 - 140822

Published: Nov. 30, 2023

Language: Английский

Citations

40

Powerful combination of FeWO4/g-C3N4 heterostructures for solar light driven photocatalytic degradation of tetracycline and its antibacterial activity DOI Open Access

Kavitha Thangavelu,

Ranjith Rajendran, P. Senthilkumar

et al.

Materials Today Sustainability, Journal Year: 2023, Volume and Issue: 24, P. 100562 - 100562

Published: Oct. 4, 2023

Language: Английский

Citations

39

Boosting the adsorptive and photocatalytic performance of MIL-101(Fe) against methylene blue dye through a thermal post-synthesis modification DOI Creative Commons
Mehdi Fattahi,

Zohreh Niazi,

Fatemeh Esmaeili

et al.

Scientific Reports, Journal Year: 2023, Volume and Issue: 13(1)

Published: Sept. 4, 2023

Photocatalytic degradation under ultra-low powered light is a viable advanced oxidation process technique against extensive emerging contaminants. As new and remarkable class of nanoporous materials, metal-organic frameworks (MOFs), attract interest for the supreme adsorptive photocatalytic functionalities. An outstanding MOF, MIL-101(Fe) chosen as photocatalyst template synthesis α-Fe2O3 by simple thermal modification to improve structural properties toward methylene blue (MB) eradication. Octahedron-like (Modified MIL-101(Fe), M-MIL-101(Fe)) was superior in dispersion separation aqueous medium. Moreover, catalytic performance increased modified form ~ 7.3% 17.1% compared pristine respectively. Synergistic improvement MB removal achieved simultaneous adsorption/degradation 5-W LED irradiation. Parametric study indicated an 18.1% 44.5% observed increasing pH from 4 10, M-MIL-101(Fe) dose 0.2 1 g L-1, followed pseudo-second-order kinetics model efficiency dropped 38% concentration 5 20 mg L-1. Radical trapping tests revealed significant role [Formula: see text] electron radicals major participants dye degradation. A loss reusability that good further. In conclusion, post-synthesis on improved its structural, catalytic, MB.

Language: Английский

Citations

26

Key role of Fe(VI)-activated Bi2WO6 in the photocatalytic oxidation of sulfonamides: Mediated electron transfer mechanism DOI
Yudan Zhang, Ping Chen, Wenying Lv

et al.

Journal of Hazardous Materials, Journal Year: 2023, Volume and Issue: 458, P. 132009 - 132009

Published: July 6, 2023

Language: Английский

Citations

25

Combined use of strictly anaerobic MBBR and aerobic MBR for municipal wastewater treatment and removal of pharmaceuticals DOI

Athanasia Iliopoulou,

Olga S. Arvaniti,

Michalis Deligiannis

et al.

Journal of Environmental Management, Journal Year: 2023, Volume and Issue: 343, P. 118211 - 118211

Published: May 28, 2023

Language: Английский

Citations

23

Harnessing Activated Hydrochars: A Novel Approach for Pharmaceutical Contaminant Removal DOI Creative Commons
Manish Kumar Gautam, Tamal Mondal,

Rupashri Nath

et al.

C – Journal of Carbon Research, Journal Year: 2024, Volume and Issue: 10(1), P. 8 - 8

Published: Jan. 8, 2024

Water contamination is a pervasive global crisis, affecting over 2 billion people worldwide, with pharmaceutical contaminants emerging as significant concern due to their persistence and mobility in aquatic ecosystems. This review explores the potential of activated hydrochars, sustainable materials produced through biomass pyrolysis, revolutionize removal from water sources. These possess high surface area, porous structure, exceptional adsorption capabilities, making them promising solution. The impact on ecosystems human health far-reaching, biodiversity, quality, public health. To address this complex issue, diverse range techniques, including adsorption, biodegradation, advanced oxidation processes, are employed industry. Activated hydrochars offer substantial capacity, feedstock origins, minimal carbon footprint. highlights contaminant broader applications improving soil air resource recovery, waste management. Interdisciplinary collaboration development intelligent treatment systems essential fully unlock hydrochars. Regulatory support policy frameworks will facilitate responsible widespread application, cleaner more future. paper aims inform scientists, environmental experts, policymakers, industry stakeholders about role addressing challenges.

Language: Английский

Citations

12

A novel Fe-loaded porous hydrothermal biochar for removing tetracycline from wastewater: Performance, mechanism, and fixed-bed column DOI
Yu Deng, Jingfan Chen,

Ailun She

et al.

Journal of environmental chemical engineering, Journal Year: 2024, Volume and Issue: 12(2), P. 112256 - 112256

Published: Feb. 19, 2024

Language: Английский

Citations

12