Application of smog chambers in atmospheric process studies DOI Creative Commons
Biwu Chu, Tianzeng Chen, Yongchun Liu

et al.

National Science Review, Journal Year: 2021, Volume and Issue: 9(2)

Published: June 13, 2021

Smog chamber experimental systems, which have been widely used in laboratory simulation for studying atmospheric processes, are comprehensively reviewed this paper. The components, development history, main research topics and achievements of smog chambers introduced. Typical the world, including their volumes, wall materials, light sources features, summarized compared. Key factors influences on environment discussed, loss, emission background pollutants. features next-generation application prospect future studies also outlined

Language: Английский

A phenomenology of new particle formation (NPF) at 13 European sites DOI Creative Commons
Dimitrios Bousiotis, Francis D. Pope, David C. S. Beddows

et al.

Atmospheric chemistry and physics, Journal Year: 2021, Volume and Issue: 21(15), P. 11905 - 11925

Published: Aug. 10, 2021

Abstract. New particle formation (NPF) events occur almost everywhere in the world and can play an important role as a source. The frequency characteristics of NPF vary spatially, this variability is yet to be fully understood. In present study, long-term size distribution datasets (minimum 3 years) from 13 sites various land uses climates across Europe were studied, events, deriving secondary not traffic-related nucleation, extracted analysed. was consistently found higher at rural background sites, while growth rates newly formed particles roadsides (though many cases differences between small), underlining importance abundance condensable compounds anthropogenic origin there. rate summer all studied. urban presented highest uncertainty due greater compared other two types site. incoming air masses specific conditions associated with them greatly affect events. general, cleaner probability for more polluted ones show rates. However, different patterns found, even close proximity (< 200 km), local each Region-wide also studied same although some which seasonality neighbouring sites. responsible increase number concentration ultrafine than 400 % on day their occurrence. degree enhancement less increased contribution sources within environment. It evident that, variables (such solar radiation intensity, relative humidity, or concentrations pollutants) appear have similar influence it impossible predict site using just these variables, crucial conditions.

Language: Английский

Citations

47

Atmospheric nanoparticle growth DOI
Dominik Stolzenburg, Runlong Cai, Sara M. Blichner

et al.

Reviews of Modern Physics, Journal Year: 2023, Volume and Issue: 95(4)

Published: Nov. 9, 2023

Atmospheric nanoparticles can serve as nuclei for cloud droplets, thereby inducing significant but uncertain effects on the radiative forcing of climate system. This article focuses physicochemical processes that govern growth these particles from formation molecular clusters until reach sizes where they act condensation nuclei. The review describes latest developments in measurement and modeling connects domains to large-scale simulations such Earth system models. authors recommend closer coordination among laboratory studies, atmospheric measurements, understand importance

Language: Английский

Citations

22

Road Traffic Emissions Lead to Much Enhanced New Particle Formation through Increased Growth Rates DOI Creative Commons
James Brean, Alex Rowell, David C. S. Beddows

et al.

Environmental Science & Technology, Journal Year: 2024, Volume and Issue: 58(24), P. 10664 - 10674

Published: June 8, 2024

New particle formation (NPF) is a major source of atmospheric aerosol particles, including cloud condensation nuclei (CCN), by number globally. Previous research has highlighted that NPF less frequent but more intense at roadsides compared to urban background. Here, we closely examine both background and roadside sites in Central Europe. We show the concentration oxygenated organic molecules (OOMs) greater roadside, OOMs along with sulfuric acid onto new particles sufficient explain growth sites. identify hitherto unreported traffic-related OOM contributing 29% 16% total background, respectively. Critically, this undiscovered an essential component NPF. Without their contribution rates subsequent enhancements survival, >50 nm produced would be reduced factor 21 site. Reductions hydrocarbon emissions from road traffic may thereby reduce numbers CCN counts.

Language: Английский

Citations

7

Influence of atmospheric conditions on the role of trifluoroacetic acid in atmospheric sulfuric acid–dimethylamine nucleation DOI Creative Commons
Ling Liu, Fangqun Yu,

Kaipeng Tu

et al.

Atmospheric chemistry and physics, Journal Year: 2021, Volume and Issue: 21(8), P. 6221 - 6230

Published: April 26, 2021

Abstract. Ambient measurements combined with theoretical simulations have shown evidence that the tropospheric degradation end-products of Freon alternatives, trifluoroacetic acid (TFA), one most important and abundant atmospheric organic substances, can enhance nucleation process based on sulfuric (SA) dimethylamine (DMA) in urban environments. However, TFA is widespread all over world under different conditions, such as temperature precursor concentration, which are factors potentially influencing thus inducing mechanisms. Herein, using density functional theory Atmospheric Cluster Dynamics Code, influence concentrations role SA–DMA has been investigated. The results indicate growth trends clusters involving increase decrease temperature. enhancement particle formation rate by contributions SA–DMA–TFA cluster to pathways be up 227-fold 95 %, respectively, at relatively low temperature, SA high DMA winter, boundary layer, or megacities far away from industrial sources sulfur-containing pollutants. These provide perspective realistic environments, revealing potential alternatives a wide range conditions.

Language: Английский

Citations

36

Application of smog chambers in atmospheric process studies DOI Creative Commons
Biwu Chu, Tianzeng Chen, Yongchun Liu

et al.

National Science Review, Journal Year: 2021, Volume and Issue: 9(2)

Published: June 13, 2021

Smog chamber experimental systems, which have been widely used in laboratory simulation for studying atmospheric processes, are comprehensively reviewed this paper. The components, development history, main research topics and achievements of smog chambers introduced. Typical the world, including their volumes, wall materials, light sources features, summarized compared. Key factors influences on environment discussed, loss, emission background pollutants. features next-generation application prospect future studies also outlined

Language: Английский

Citations

35