Abstract.
Gaseous
pollutants
at
the
ground
level
seriously
threaten
urban
air
quality
environment
and
public
health.
There
are
few
estimates
of
gaseous
that
spatially
temporally
resolved
continuous
across
China.
This
study
takes
advantage
big
data
artificial-intelligence
technologies
to
generate
seamless
daily
maps
three
major
ambient
pollutant
gases,
i.e.,
NO2,
SOµgâmâ3),
(10.7â2
rebounded
more
than
2
times
slower
due
emissions
residents'
increased
indoor
cooking
atmospheric
oxidation
capacity.
Surface
reached
their
peak
annual
concentrations
21.3â±â8.8ââ3,
23.1â±â13.3â±â0.29âmgâmâ3
2013,
then
continuously
declined
over
time
by
12â%,
55â%,
17â%,
respectively,
until
2020.
The
declining
rates
were
prominent
2017
sharper
reductions
anthropogenic
but
have
slowed
down
recent
years.
Nevertheless,
people
still
suffer
high-frequency
risk
exposure
eastern
China,
almost
World
Health
Organization
(WHO)
recommended
short-term
guidelines
(AQG)
since
2018,
benefiting
implemented
stricter
âultra-lowâ
emission
standards.
reconstructed
dataset
will
benefit
future
(especially
short-term)
pollution
environmental
health-related
studies.
Atmospheric chemistry and physics,
Journal Year:
2023,
Volume and Issue:
23(2), P. 1511 - 1532
Published: Jan. 26, 2023
Abstract.
Gaseous
pollutants
at
the
ground
level
seriously
threaten
urban
air
quality
environment
and
public
health.
There
are
few
estimates
of
gaseous
that
spatially
temporally
resolved
continuous
across
China.
This
study
takes
advantage
big
data
artificial-intelligence
technologies
to
generate
seamless
daily
maps
three
major
ambient
pollutant
gases,
i.e.,
NO2,
SO2,
CO,
China
from
2013
2020
a
uniform
spatial
resolution
10
km.
Cross-validation
between
our
observations
illustrated
high
on
basis
for
surface
CO
concentrations,
with
mean
coefficients
determination
(root-mean-square
errors)
0.84
(7.99
µg
m−3),
(10.7
0.80
(0.29
mg
respectively.
We
found
COVID-19
lockdown
had
sustained
impacts
pollutants,
where
recovered
its
normal
in
around
34th
day
after
Lunar
New
Year,
while
SO2
NO2
rebounded
more
than
2
times
slower
due
emissions
residents'
increased
indoor
cooking
atmospheric
oxidation
capacity.
Surface
reached
their
peak
annual
concentrations
21.3
±
8.8
m−3,
23.1
13.3
1.01
0.29
m−3
2013,
then
continuously
declined
over
time
by
12
%,
55
17
respectively,
until
2020.
The
declining
rates
were
prominent
2017
sharper
reductions
anthropogenic
but
have
slowed
down
recent
years.
Nevertheless,
people
still
suffer
high-frequency
risk
exposure
eastern
China,
almost
World
Health
Organization
(WHO)
recommended
short-term
guidelines
(AQG)
since
2018,
benefiting
implemented
stricter
“ultra-low”
emission
standards.
reconstructed
dataset
will
benefit
future
(especially
short-term)
pollution
environmental
health-related
studies.
Environmental Science & Technology,
Journal Year:
2023,
Volume and Issue:
57(46), P. 18282 - 18295
Published: April 28, 2023
Fine
particulate
matter
(PM2.5)
chemical
composition
has
strong
and
diverse
impacts
on
the
planetary
environment,
climate,
health.
These
effects
are
still
not
well
understood
due
to
limited
surface
observations
uncertainties
in
model
simulations.
We
developed
a
four-dimensional
spatiotemporal
deep
forest
(4D-STDF)
estimate
daily
PM2.5
at
spatial
resolution
of
1
km
China
since
2000
by
integrating
measurements
species
from
high-density
observation
network,
satellite
retrievals,
atmospheric
reanalyses,
Cross-validation
results
illustrate
reliability
sulfate
(SO42-),
nitrate
(NO3-),
ammonium
(NH4+),
chloride
(Cl-)
estimates,
with
high
coefficients
determination
(CV-R2)
ground-based
0.74,
0.75,
0.71,
0.66,
average
root-mean-square
errors
(RMSE)
6.0,
6.6,
4.3,
2.3
μg/m3,
respectively.
The
three
components
secondary
inorganic
aerosols
(SIAs)
account
for
21%
20%
14%
(NH4+)
total
mass
eastern
China;
we
observed
significant
reductions
40-43%
between
2013
2020,
slowing
down
2018.
Comparatively,
ratio
SIA
increased
7%
across
except
Beijing
nearby
areas,
accelerating
recent
years.
SO42-
been
dominant
component
China,
although
it
was
surpassed
NO3-
some
e.g.,
Beijing-Tianjin-Hebei
region
2016.
SIA,
accounting
nearly
half
(∼46%)
mass,
drove
explosive
formation
winter
haze
episodes
North
Plain.
A
sharp
decline
concentrations
an
increase
SIA-to-PM2.5
ratios
during
COVID-19
lockdown
were
also
revealed,
reflecting
enhanced
oxidation
capacity
particles.
Ecotoxicology and Environmental Safety,
Journal Year:
2023,
Volume and Issue:
264, P. 115491 - 115491
Published: Sept. 18, 2023
The
combine
effect
of
air
pollutant
mixture
on
atherosclerotic
cardiovascular
disease
(ASCVD)
remain
undefined.
This
study
aims
to
explore
the
association
between
long-term
exposure
pollutants
and
ASCVD,
focusing
mediating
role
lipids,
blood
pressure
BMI.This
was
based
CHCN-BTH
cohort
study.
annual
concentrations
PM2.5
constituents
were
sourced
from
in
Tracking
Air
Pollution
China
(TAP)
ChinaHighAirPollutants
(CHAP)
datasets
2014
2019.
A
Cox
mixed-effects
model
used
investigate
associations
ASCVD.
combined
impact
assessed
using
Quantile
g-Computation.
Stratified,
sensitivity,
mediation
analyses
conducted.A
total
27,134
participants
aged
18-80
recruited
present
We
found
that
each
IQR
increase
PM2.5,
PM1,
NO2,
O3,
BC,
SO42-,
OM
significantly
associated
with
incidence
hazard
ratios
(HRs)
95
%
confidence
interval
(CI)
1.55
(1.35,
1.78),
1.46
(1.27,
1.67),
1.30
(1.21,
1.39),
1.66
(1.41,1.95),
2.14
(1.63,
2.83),
1.65
(1.25,
2.17)
1.92(1.52,
2.45),
respectively.
ASCVD
1.79
(1.46,
2.20),
contributed
83.3
this
effect.
Mediation
models
suggested
might
be
mediated
through
SBP,
DBP,
HDL-C,
LDL-C,
hsCRP
BMI
(mediation
proportion
range
1.3
26.1
%),
Notably,
HDL-C
played
roles
11.3
(7.0
%,
18.4),
(17.7
38.1
%)
25.4
(15.4,
47.7
effects
PM1
respectively.Long-term,
high-level
significantly
an
elevated
risk
particularly
for
PM2.5.
Blood
pressure,
lipids
BMI,
especially
may
mediate
Environment International,
Journal Year:
2022,
Volume and Issue:
170, P. 107566 - 107566
Published: Oct. 5, 2022
Although
exposure
to
fine
particulate
matter
(PM2.5)
has
been
associated
with
cognitive
decline,
little
is
known
about
which
PM2.5
constituents
are
more
harmful.
Recent
study
on
the
association
between
and
sleep
quality
prompted
us
propose
that
may
mediate
adverse
effects
of
components
decline.
Understanding
function,
as
well
mediating
role
provides
a
future
intervention
target
for
improving
function.
Using
data
involving
1834
participants
from
multicenter
cross-sectional
in
nine
cities
Beijing-Tianjin-Hebei
(BTH)
region
China,
we
undertook
multivariable
linear
regression
analyses
quantify
annual
moving-average
its
chemical
function
assess
modifying
characteristic
this
association.
Besides,
examined
extent
was
mediated
via
by
mediation
analysis.
We
observed
significantly
negative
associations
an
increase
one
interquartile
range
[-0.876
(95
%
CI:
-1.205,
-0.548)],
organic
carbon
[-0.481
-0.744,
-0.219)],
potassium
[-0.344
-0.530,
-0.157)],
iron
[-0.468
-0.646,
-0.291)],
ammonium
ion
[-0.125
-0.197,
-0.052)]
However,
didn't
find
any
individual
harmful
than
PM2.5.
Poor
partially
estimated
associations,
were
explained
ranging
2.28
11.99
%.
Stratification
showed
people
living
areas
lower
greenspace
susceptible
specific
components.
Our
suggests
effect
suffering
pronounced
among
individuals
poor
quality,
amplifying
environmental
inequalities
health.
Besides
reducing
pollution,
be
another
measure
worth
considering
improve
cognition
if
our
research
confirmed
future.
Abstract.
Gaseous
pollutants
at
the
ground
level
seriously
threaten
urban
air
quality
environment
and
public
health.
There
are
few
estimates
of
gaseous
that
spatially
temporally
resolved
continuous
over
long
periods
in
China.
This
study
takes
advantage
big
data
artificial
intelligence
technologies
to
generate
seamless
daily
maps
three
major
pollutant
gases,
i.e.,
NO2,
SO2,
CO,
across
China
from
2013
2020
a
uniform
spatial
resolution
10
km.
Cross-validation
illustrated
high
on
basis
for
with
mean
out-of-bag
coefficients
determination
(root-mean-square
errors)
0.84
(7.99
μg/m3),
(10.7
0.80
(0.29
mg/m3),
respectively.
They
have
experienced
significant
declines
then
recoveries
during
after
COVID-19
lockdown
associated
changes
anthropogenic
emissions
eastern
China,
while
surface
CO
recovered
faster
than
SO2
NO2.
All
decreased
significantly
by
0.23,
2.01,
49
μg/m3
per
year
(p
<
0.001)
2013–2020,
especially
agglomerations.
The
declining
rates
were
larger
2013–2017
but
slowed
down
recent
years.
Both
areas
occurrence
probabilities
days
exceeding
standards
also
gradually
shrank
weakened
time,
which
almost
disappeared
2018–2020,
suggesting
improvements
reconstructed
dataset
pollutants,
ChinaHighNO2,
ChinaHighSO2,
ChinaHighCO,
will
benefit
future
(especially
short-term)
pollution
environmental
health-related
studies.