Durable Antibacterial Photothermal Membrane Using Melanin-Inspired Cu-Doped Polynorepinephrine for Water Remediation DOI
Heng Zhang, Wenxin Qi,

Shang Liu

et al.

Nano Letters, Journal Year: 2024, Volume and Issue: unknown

Published: Nov. 22, 2024

Solar-driven interfacial evaporation is an efficient approach to addressing water scarcity due its environmental sustainability. However, the prolonged use of solar evaporators causes microbial contamination from wastewater. Inspired by antifouling properties polydopamine, we develop a series mono- and dual-metal-loaded poly(norepinephrine) (PNE) nanoparticles pre-doping multiple metal ions. Metal doping enhances photothermal conversion efficiency (∼60%) PNE reducing energy bandgap imparts antimicrobial properties. Cu

Language: Английский

Ultimate water capillary evaporation in bamboo-inspired evaporator DOI Creative Commons
Kefan Shi, Marliyana Aizudin,

Meilan Pan

et al.

Materials Horizons, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 1, 2025

The chimney-assisted enclosed cavity structure significantly enhances water capillary evaporation and thermal localization, setting new performance records beyond those of traditional natural evaporators.

Language: Английский

Citations

3

Emerging Photothermal Materials from Lignin and Coal for Solar Vapor Generation DOI Open Access
Zhan‐Ku Li, Weidong Zhang,

Hong‐Lei Yan

et al.

Advanced Functional Materials, Journal Year: 2025, Volume and Issue: unknown

Published: Feb. 16, 2025

Abstract Solar vapor generation (SVG) garners significant attention as a technology for producing clean water owing to its high efficiency and zero carbon emissions. However, the widespread adoption of SVG is constrained by cost, low mechanical strength, complex fabrication processes current photothermal materials. Lignin coal, abundant in aromatic rings, C═O bonds, quinone structures, present natural advantages enhancing light absorption improving properties This review begins with an overview fundamentals strategies aimed at promoting efficiency. It then delves into structural characteristics conversion mechanisms lignin highlighting their unique contributions field. Further, latest advancements application lignin/coal‐based materials are comprehensively summarized. work not only lays systematic scientific foundation development next‐generation but also underscores potential value‐added utilization thereby contributing sustainable resource management.

Language: Английский

Citations

1

Advancing Efficiency in Solar-Driven Interfacial Evaporation: Strategies and Applications DOI
Lanlan Hou, Shuai Li,

Yingqun Qi

et al.

ACS Nano, Journal Year: 2025, Volume and Issue: unknown

Published: March 8, 2025

Solar-driven interfacial evaporation (SDIE) has emerged as a promising technology for addressing global water scarcity by utilizing solar-thermal conversion and at the air/material/water interface. The exceptional performance of these systems attracted significant interest; it is imperative to establish rigorous scientific standards evaluating effectiveness, optimizing system design, ensuring efficient practical applications. In this Review, we propose consensus criteria accurately assessing guiding future advancements. We then explore fundamental mechanisms driving synergy, emphasizing how material compositions, microscopic hierarchical structures, macroscopic three-dimensional spatial architecture designs enhance solar absorption photothermal conversion; balance heat confinement with pathway optimization; manage salt resistance; regulate enthalpy during vaporization. These matched coordination strategies are crucial maximizing target SDIE efficiency. Additionally, investigate applications technologies, focusing on cutting-edge progress versatile purification, combined atmospheric harvesting, collection, electric generation, deicing. Finally, highlight challenges exciting opportunities advancing research, efforts integrate principles, system-level collaboration, application-driven approaches boost sustainable highly energy technologies. By linking evaluation optimization influencing factors, offer comprehensive overview field outlook that promotes clean production synergistic

Language: Английский

Citations

1

Nanofibrous Hydrogel with Highly Salt‐Resistant Radial/Vertical‐Combined Structure for Efficient Solar Interfacial Evaporation DOI Open Access

Yong Wen,

Shengwu Deng,

Quanpei Xie

et al.

Small, Journal Year: 2025, Volume and Issue: unknown

Published: March 13, 2025

Abstract Hydrogel‐based solar interfacial evaporators, featuring various channels such as random, unidirectional, and radial array, are considered effective for seawater desalination owing to their porous structure, lower evaporation enthalpy, controllable water transport capacity. However, each individual array structure has its own strengths limitations, influencing transportation, thermal management, salt rejection. By combining the benefits of configuration into a single evaporator, performance can be maximized. Herein, study develops unique nanofibrous hydrogel‐based evaporator combined radical/vertical structure. This integrated with external internal vertical endows this excellent capability reduced heat loss, resulting in superior high salty resistance. The addition nanofibers hydrogels not only enhances hydrogel's stability but also facilitates transport. Under 1 sun illumination, achieve an impressive rate 4.62 kg m −2 h −1 energy efficiency 149.57%. After 12 20 wt.% NaCl solution, it still maintains average 3.98 minimal accumulation, thereby exhibiting exceptional resistance durability.

Language: Английский

Citations

1

Molecular engineering on self-floating phenolic aerogels for efficient solar vapor generation DOI
Junwei Pan, Yu Han, Xiangyang Xie

et al.

Separation and Purification Technology, Journal Year: 2025, Volume and Issue: unknown, P. 131733 - 131733

Published: Jan. 1, 2025

Language: Английский

Citations

0

Cellulose-derived hydrogel with low vaporization enthalpy enables highly efficient solar steam generation DOI
Junbo Chen, Yuanpeng Xie,

Maosong Tian

et al.

Carbohydrate Polymers, Journal Year: 2025, Volume and Issue: 356, P. 123385 - 123385

Published: Feb. 13, 2025

Language: Английский

Citations

0

Integration of Bio-Enzyme-Treated Super-Wood and AIE-Based Nonwoven Fabric for Efficient Evaporating the Wastewater with High Concentration of Ammonia Nitrogen DOI Creative Commons
Qian Ding,

Bingqi Jin,

Yong‐Fei Zheng

et al.

Nano-Micro Letters, Journal Year: 2025, Volume and Issue: 17(1)

Published: March 10, 2025

Abstract The treatment of ammonia nitrogen wastewater (ANW) has garnered significant attention due to the ecology, and even biology is under increasing threat from over discharge ANW. Conventional ANW methods often encounter challenges such as complex processes, high costs secondary pollution. Considerable progress been made in employing solar-induced evaporators for treatment. However, there remain notable barriers transitioning fundamental research practical applications, including insufficient evaporation rates inadequate resistance biofouling. Herein, we propose a novel evaporator, which comprises bio-enzyme-treated wood aerogel that serves water pumping storage layer, cost-effective multi-walled carbon nanotubes coated hydrophobic/hydrophilic fibrous nonwoven mat functioning photothermal aggregation-induced emission (AIE) molecules incorporated anti-biofouling agent. resultant bioinspired evaporator demonstrates rate 12.83 kg m −2 h −1 when treating simulated containing 30 wt% NH 4 Cl 1.0 sun illumination. AIE-doped exhibits remarkable photodynamic antibacterial activity against mildew bacteria, ensuring outstanding biofouling extended periods When enhanced by natural wind irradiation, achieves an impressive exceeding 20 . This advancement represents promising viable approach effective removal wastewater.

Language: Английский

Citations

0

Advances in Ice-Templated Graphene Aerogels: Fabrication, Properties, and Applications DOI
Meng Li, Yi Zheng, Hao Bai

et al.

ACS Applied Materials & Interfaces, Journal Year: 2025, Volume and Issue: unknown

Published: March 20, 2025

Graphene has been one of the most widely explored two-dimensional (2D) assemblies due to its outstanding mechanical, electrical, and thermal properties resulting from unique characteristics high anisotropy strong carbon-carbon bonds. Aerogels, characterized by their ultralow density ultrahigh specific surface area, stand out as leading porous materials. Therefore, integration graphene aerogels would boost development multifunctional Among various methods for fabrication aerogels, ice-templating received significant interest ecofriendly nature a physical process, broad applicability across material systems, proficiency in constructing abundant structures multifunctionalities. Consequently, become prevalent technique efficient assembly nanosheets into with inherited graphene, multifunctionality derived diverse constituents, well-controlled architecture. In this review, we systematically summarize progress ice-templated graphene-based aerogels. Initially, introduce process these elaborating each step precursor preparation freezing, drying, post-treatment. Subsequently, demonstrate applications macroarchitectures microstructures. Finally, review concludes straightforward summary, highlighting challenges opportunities associated This systematic aims offer new insights design innovative multiscale architecture multifunctionalities, which are crucial variety engineering applications.

Language: Английский

Citations

0

Biomass-Derived Gradient and Aligned Structured Aerogel for Sustainable Agricultural Irrigation DOI
Lanyue Zhang,

Zhanhong Yuan,

Xiaotong Fu

et al.

Nano Letters, Journal Year: 2025, Volume and Issue: unknown

Published: March 23, 2025

Interface evaporation-driven hydroelectric systems integrating water purification and energy collection offer the potential for sustainable agricultural irrigation. However, achieving high evaporation rates efficient harvesting poses challenges, particularly in optimizing transport. This study develops a gradient-aligned structured aerogel (GA aerogel), composed of biomass materials such as cellulose chitosan, which utilizes transport through aligned channels, unique ion management nanoscale chitosan's ability to reduce consumption, thereby enhancing performance. The GA achieves solar absorption rate 91.4%, an 2.5 kg m–2 h–1, output power 680 nW cm–2, stable operation over 120 h. Furthermore, by series array with capacitive storage, system harvested electrical irrigate plants purified water, promoting agriculture providing insights designing biomass-based evaporators.

Language: Английский

Citations

0

Scalable fabrication of sustainable, recyclable and multifunctional graphene−cellulose foam for efficient photothermal water evaporation DOI
Minjie Hou, Hui Xu, Li Xu

et al.

International Journal of Biological Macromolecules, Journal Year: 2025, Volume and Issue: 308, P. 142628 - 142628

Published: March 30, 2025

Language: Английский

Citations

0