Exploring Pyrazine‐Based Organic Redox Couples for Enhanced Thermoelectric Performance in Wearable Energy Harvesters DOI

Chia‐Yu Lee,

Ching‐Chieh Hsu,

Chia‐Hsin Wang

et al.

Small, Journal Year: 2024, Volume and Issue: unknown

Published: Oct. 2, 2024

Abstract Thermoelectric generators (TEGs) based on thermogalvanic cells can convert low‐temperature waste heat into electricity. Organic redox couples are well‐suited for wearable devices due to their nontoxicity and the potential enhance ionic Seebeck coefficient through functional‐group modifications. Pyrazine‐based organic with different functional groups is comparatively analyzed cyclic voltammetry under varying temperatures. The results reveal substantial differences in entropy changes temperature highlight 2,5‐pyrazinedicarboxylic acid dihydrate (PDCA) as optimal candidate. How of pyrazine compounds impact examined, by calculating electrostatic density theory. To evaluate thermoelectric properties, PDCA integrated concentrations a double‐network hydrogel comprising poly(vinyl alcohol) polyacrylamide. resulting champion device exhibits an impressive ( S i ) 2.99 mV K −1 , thermal conductivities ≈67.6 µS cm ≈0.49 W m respectively. Finally, TEG constructed connecting 36 pieces 20 × 10 −3 PDCA‐soaked series. It achieves maximum power output ≈0.28 µW gradient 28.3 °C small light‐emitting diode. These findings significant TEGs devices.

Language: Английский

Ionic thermoelectric gels and devices: Progress, opportunities, and challenges DOI
Yu Mao, Huan Li, Yuchen Li

et al.

EnergyChem, Journal Year: 2024, Volume and Issue: 6(3), P. 100123 - 100123

Published: March 19, 2024

Language: Английский

Citations

26

Solar interfacial evaporation systems with multi-field synergies boost water purification and blue energy harvesting technologies DOI
Baichun Wang, Xinyu Huang, Zhe Liu

et al.

Energy & Environmental Science, Journal Year: 2024, Volume and Issue: 17(20), P. 7600 - 7626

Published: Jan. 1, 2024

Water purification and blue energy harvest based on SIES in synergies with light field, thermal field hydrochemical field.

Language: Английский

Citations

14

Photothermal Material‐Based Solar‐Driven Cogeneration of Water and Electricity: An Efficient and Promising Technology DOI Open Access

Xiaoqing Bao,

Haopeng Luo,

Tingyi Weng

et al.

Small, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 19, 2025

Abstract With the increasing demand for fresh‐water and electricity in modern society, various technologies are being explored to obtain electricity. Due advances materials science, solar‐driven interfacial evaporation (SDIE) systems have attracted widespread attention because they require only solar energy, possess a high rate little pollution. The researchers combined energy harvesting measures into system output electricity, further improving utilization. However, more in‐depth research review remain on using SDIE efficient water‐electricity cogeneration. Therefore, mechanisms of different photothermal that utilize produce thermal first summarized this paper. Subsequently, mechanism application thermal, mechanical, chemical, electrical power cogeneration discussed. Concurrently, vital mathematical equations widely used simulation methods performance evaluation practical applications presented. design operation based analyzed summarized. Based understanding these aspects, future development direction is proposed address problems faced basic applications.

Language: Английский

Citations

1

Carbon material-based thermoelectric ultra-high-performance alkali-activated concrete DOI
Rongzhen Piao, Dongsun Lee,

Seong Yun Woo

et al.

Composites Part B Engineering, Journal Year: 2025, Volume and Issue: unknown, P. 112279 - 112279

Published: Feb. 1, 2025

Language: Английский

Citations

1

Electrode-dependent thermoelectric effect in ionic hydrogel fiber for self-powered sensing and low-grade heat harvesting DOI
Yunling Dai, Hongbo Wang, Kun Qi

et al.

Chemical Engineering Journal, Journal Year: 2024, Volume and Issue: 497, P. 154970 - 154970

Published: Aug. 23, 2024

Language: Английский

Citations

6

Recent advances in ionic thermoelectric systems and theoretical modelling DOI Creative Commons

Nazish Jabeen,

Muhammad Muddasar,

Nicolás Menéndez

et al.

Chemical Science, Journal Year: 2024, Volume and Issue: 15(35), P. 14122 - 14153

Published: Jan. 1, 2024

Converting waste heat from solar radiation and industrial processes into useable electricity remains a challenge due to limitations of traditional thermoelectrics. Ionic thermoelectric (i-TE) materials offer compelling alternative thermoelectrics their excellent ionic thermopower, low thermal conductivity, abundant material options. This review categorizes i-TE thermally diffusive thermogalvanic types, with an emphasis on the former its superior thermopower. also highlights for creating supercapacitors (ITESCs) that can generate significantly higher voltages low-grade sources compared conventional technologies. Additionally, it explores cells combined devices, discussing key optimization parameters theoretical modeling approaches maximizing device performance. Future directions aim enhance performance address energy density challenges flexible wearable applications. Herein, cutting-edge are comprehensively outlined, empowering researchers develop next-generation harvesting technologies more sustainable future.

Language: Английский

Citations

6

Lattice Architectures for Thermoelectric Energy Harvesting DOI
Danwei Zhang,

Natalie Ngoh Yen Qi,

Samantha Faye Duran Solco

et al.

ACS Energy Letters, Journal Year: 2024, Volume and Issue: 9(5), P. 2240 - 2247

Published: April 17, 2024

Tapping on waste heat for green electricity is a welcomed goal, especially in an energy-scarce era. For more than 200 years, the optimization of thermoelectric modules has been through either materials efficiency or device topology (fill factor, aspect ratio, etc.). Now, there pressing need re-examination its design higher power performance modules. Specifically, have recent reports potential leg geometries increased output power, but progress hampered by current fabrication methods. In this Perspective, we offer fresh take how lattice architectural legs are cost-effective strategy that can drastically improve output. We will discuss extent to which lightweight and trade-offs with mechanical conclude strategies realize them industrial applications.

Language: Английский

Citations

4

Insights Into Janus Interfaces with Ordered Micro/Nanostructures for Low‐Temperature Differential Evaporation DOI
Bing‐Da Sun, Mengyuan Wu,

Xuguang Zhao

et al.

Advanced Functional Materials, Journal Year: 2024, Volume and Issue: unknown

Published: July 14, 2024

Abstract Low‐temperature differential evaporation constitutes a promising direction for energy‐saving desalination. Herein, novel Janus interfacial structure with well‐ordered micro/nanopores is developed. Fabricated can weak the water intermolecular forces and pump to hydrophilic–hydrophobic junction. Within nanochannels, increased curvature of meniscus increases ratio thin layers, thereby enhancing microscale heat transfer at heated walls; in addition, smaller nanopores limit development vortices liquid–gas interface prevent back mixing intermediate interface, which possess nanoscale effect on intensifying evaporation. These effects are validated by theoretical experimental studies. Optimized (20 nm) 95°/25° exhibits fluxes up 2.4 kg m −2 h −1 45 °C (feed side)/25 (permeate side, ambient pressure), as enthalpy only 30% that direct The unique simultaneously inhibits salt accumulation achieve self‐cleaning, maintaining steady performance during 480 continuous desalination 50 cycles batch operation. This work highlights structural design strategy separation materials specific micro/nanoscopic topologies high thermally driven applications.

Language: Английский

Citations

4

Liquid-flow thermocells with high hybrid entropy for low-grade heat harvesting DOI
Hongwei Chen,

Haoyu Zou,

Fanghao Zhong

et al.

Nano Energy, Journal Year: 2024, Volume and Issue: 129, P. 109992 - 109992

Published: July 14, 2024

Language: Английский

Citations

4

Giant gateable thermoelectric conversion by tuning the ion linkage interactions in covalent organic framework membranes DOI Creative Commons

Shijie Yin,

Jianguo Li,

Zhuozhi Lai

et al.

Nature Communications, Journal Year: 2024, Volume and Issue: 15(1)

Published: Sept. 17, 2024

Language: Английский

Citations

4