Reply on RC1 DOI Creative Commons

Alexei Rozanov

Published: Aug. 15, 2024

Abstract. A new retrieval algorithm to obtain vertical profiles of the aerosol extinction coefficient from measurements scattered solar light in limb viewing geometry made by OMPS-LP instrument is presented. The method employs normalization radiances irradiance contrast a measurement at an upper tangent height, which used most other published limb-scatter retrievals. main advantage this approach nearly complete elimination dependence results on prior profile retrieval. This makes well suitable analyze observation scenes with highly elevated plumes as occurred after Hunga Tonga-Hunga Ha'apai volcanic eruption January 2022. were compared independent data SAGE III/ISS and OSIRIS. In general, agreement within 25 % between different products was observed although larger differences seen very strong eruptions wildfires. product investigate evolution plume eruption.

Language: Английский

Stratospheric Climate Anomalies and Ozone Loss Caused by the Hunga Tonga‐Hunga Ha'apai Volcanic Eruption DOI Creative Commons
Xinyue Wang, William J. Randel, Yunqian Zhu

et al.

Journal of Geophysical Research Atmospheres, Journal Year: 2023, Volume and Issue: 128(22)

Published: Nov. 22, 2023

Abstract The Hunga Tonga‐Hunga Ha'apai (HTHH) volcanic eruption in January 2022 injected unprecedented amounts of water vapor (H 2 O) and a moderate amount the aerosol precursor sulfur dioxide (SO ) into Southern Hemisphere (SH) tropical stratosphere. H O perturbations have persisted during early 2023 dispersed throughout atmosphere. Observations show large‐scale SH stratospheric cooling, equatorward shift Antarctic polar vortex slowing Brewer‐Dobson circulation. Satellite observations substantial ozone reductions over winter midlatitudes that coincide with largest circulation anomalies. Chemistry‐climate model simulations forced by realistic HTHH inputs SO qualitatively reproduce observed evolution plumes first year, exhibits changes effects similar to behavior. agreement demonstrates are caused influences.

Language: Английский

Citations

32

Siege in the Southern Stratosphere: Hunga Tonga‐Hunga Ha'apai Water Vapor Excluded From the 2022 Antarctic Polar Vortex DOI Creative Commons
G. L. Manney, M. L. Santee, A. Lambert

et al.

Geophysical Research Letters, Journal Year: 2023, Volume and Issue: 50(14)

Published: July 25, 2023

Abstract We use Aura Microwave Limb Sounder (MLS) trace gas measurements to investigate whether water vapor (H 2 O) injected into the stratosphere by Hunga Tonga‐Hunga Ha'apai (HTHH) eruption affected 2022 Antarctic stratospheric vortex. Other MLS‐measured long‐lived species are used distinguish high HTHH H O from that descending in vortex upper‐stratospheric peak. reached southern latitudes June–July but was effectively excluded strong transport barrier at its edge. MLS O, nitric acid, chlorine species, and ozone within polar were near average; large, strong, long‐lived, not exceptionally so. There is thus no clear evidence of influence on or composition. Substantial impacts vortices expected succeeding years since has spread globally.

Language: Английский

Citations

31

The Estimated Climate Impact of the Hunga Tonga‐Hunga Ha'apai Eruption Plume DOI Creative Commons
M. R. Schoeberl, Yi Wang, Rei Ueyama

et al.

Geophysical Research Letters, Journal Year: 2023, Volume and Issue: 50(18)

Published: Sept. 26, 2023

Abstract On 15 January 2022, the Hunga Tonga‐Hunga Ha'apai (HT) eruption injected SO 2 and water into middle stratosphere. The is rapidly converted to sulfate aerosols. aerosol vapor anomalies have persisted in Southern Hemisphere throughout 2022. anomaly increases net downward IR radiative flux whereas layer reduces direct solar forcing. reduction larger than increased flux. Thus, tropospheric forcing will be negative. changes peak July August diminish thereafter. Scaling observed cooling after 1991 Pinatubo eruption, HT would cool 2022 Hemisphere's average surface temperatures by less 0.037°C.

Language: Английский

Citations

28

Strong Evidence of Heterogeneous Processing on Stratospheric Sulfate Aerosol in the Extrapolar Southern Hemisphere Following the 2022 Hunga Tonga‐Hunga Ha'apai Eruption DOI Creative Commons
M. L. Santee, A. Lambert,

L. Froidevaux

et al.

Journal of Geophysical Research Atmospheres, Journal Year: 2023, Volume and Issue: 128(16)

Published: Aug. 2, 2023

Abstract The January 2022 eruption of Hunga Tonga‐Hunga Ha'apai (HT‐HH) caused the largest enhancement in stratospheric aerosol loading decades and produced an unprecedented water vapor, leading to strong cooling that turn induced changes large‐scale circulation. Here we use satellite measurements gas‐phase constituents together with extinction investigate extent which thick aerosol, excess moisture, enabled heterogeneous chemical processing. In southern tropics, unambiguous signatures substantial chlorine nitrogen repartitioning appear over a broad vertical domain almost immediately after eruption, depletion N 2 O 5 , NO x HCl accompanied by HNO 3 ClO, ClONO . After initially rising steeply, ClO plateau, maintaining fairly constant abundances for several months. These patterns are consistent saturation hydrolysis, suggesting this reaction is primary mechanism observed composition changes. midlatitudes subtropics show similar but weaker enhancements those regions, however, effects anomalous transport dominate evolution HCl, obscuring signs Perturbations species considerably than measured midlatitude stratosphere 2020 following Australian New Year's fires. moderate HT‐HH‐induced reactive seen throughout middle low‐latitude stratosphere, far smaller typical winter polar vortices, do not lead appreciable ozone loss; rather, extrapolar lower‐stratospheric remains primarily controlled dynamical processes.

Language: Английский

Citations

24

Unexpectedly rapid aerosol formation in the Hunga Tonga plume DOI Creative Commons
Elizabeth Asher, Michael A. Todt, K. H. Rosenlof

et al.

Proceedings of the National Academy of Sciences, Journal Year: 2023, Volume and Issue: 120(46)

Published: Oct. 30, 2023

The Hunga Tonga–Hunga Ha’apai (HT-HH) volcanic eruptions on January 13 and 15, 2022, produced a plume with the highest signal in stratospheric aerosol optical depth observed since eruption of Mt. Pinatubo 1991. Suites balloon-borne instruments series launches from Réunion Island intercepted HT-HH between 7 10 d eruptions, yielding observations number size distribution sulfur dioxide (SO 2 ) water vapor (H O) concentrations. measurements reveal an unexpected abundance large particles plume, constrain total injected to approximately 0.2 Tg, provide information altitude injection, indicate that formation sulfuric acid was complete within 3 wk. Large H O enhancements contributed as much ~30% ambient surface area likely accelerated SO oxidation rates three times faster than under normal conditions.

Language: Английский

Citations

18

Chemistry Contribution to Stratospheric Ozone Depletion After the Unprecedented Water‐Rich Hunga Tonga Eruption DOI Creative Commons
Jun Zhang, Douglas E. Kinnison, Yunqian Zhu

et al.

Geophysical Research Letters, Journal Year: 2024, Volume and Issue: 51(7)

Published: April 1, 2024

Abstract Following the Hunga Tonga–Hunga Ha'apai (HTHH) eruption in January 2022, stratospheric ozone depletion was observed at Southern Hemisphere mid‐latitudes and over Antarctica during 2022 austral wintertime springtime, respectively. The injected sulfur dioxide unprecedented amounts of water vapor into stratosphere. This work examines chemistry contribution volcanic materials to using chemistry‐climate model simulations with nudged meteorology. Simulated nitrogen oxide (NO x = NO + 2 ) anomalies show good agreement satellite observations. We find that yields up 4% destruction near ∼70 hPa August 20% ∼80 October. Most is attributed internal variability dynamical changes forced by eruption. Both modeling observations a significant reduction associated HTHH aerosol plume, indicating enhanced dinitrogen pentoxide hydrolysis on sulfate aerosol.

Language: Английский

Citations

8

Retrieval of stratospheric aerosol extinction coefficients from OMPS-LP measurements DOI Creative Commons
Alexei Rozanov, Christine Pohl, Carlo Arosio

et al.

Published: Feb. 8, 2024

Abstract. A new retrieval algorithm to obtain vertical profiles of the aerosol extinction coefficient from measurements scattered solar light in limb viewing geometry made by OMPS-LP instrument is presented. The method employs normalization radiances irradiance contrast a measurement at an upper tangent height, which used most other published limb-scatter retrievals. main advantage this approach nearly complete elimination dependence results on prior profile retrieval. This makes well suitable analyze observation scenes with highly elevated plumes as occurred after Hunga Tonga-Hunga Ha'apai volcanic eruption January 2022. were compared independent data SAGE III/ISS and OSIRIS. In general, agreement within 25 % between different products was observed although larger differences seen very strong eruptions wildfires. product investigate evolution plume eruption.

Language: Английский

Citations

7

Evolution of the Climate Forcing During the Two Years After the Hunga Tonga‐Hunga Ha'apai Eruption DOI Creative Commons
M. R. Schoeberl, Yi Wang, Ghassan Taha

et al.

Journal of Geophysical Research Atmospheres, Journal Year: 2024, Volume and Issue: 129(14)

Published: July 24, 2024

Abstract We calculate the climate forcing for 2 ys after 15 January 2022, Hunga Tonga‐Hunga Ha'apai (Hunga) eruption. use satellite observations of stratospheric aerosols, trace gases and temperatures to compute tropopause radiative flux changes relative climatology. Overall, net downward decreased compared The water vapor anomaly initially increases infrared flux, but this diminishes as disperses. aerosols cause a solar reduction that dominates change over most yrs period. induced temperature produce decrease in long‐wave flux. ozone short‐wave creating small sub‐tropical increase total from mid‐2022 2023. By end 2023, have disappeared. There is some disagreement measured aerosol optical depth (SAOD) which we view measure uncertainty; however, SAOD uncertainty does not alter our conclusion that, overall, dominate changes.

Language: Английский

Citations

6

OMPS-LP aerosol extinction coefficients and their applicability in GloSSAC DOI Creative Commons
Mahesh Kovilakam, L. W. Thomason, Magali Verkerk

et al.

Atmospheric chemistry and physics, Journal Year: 2025, Volume and Issue: 25(1), P. 535 - 553

Published: Jan. 16, 2025

Abstract. The Global Space-based Stratospheric Aerosol Climatology (GloSSAC) is essential for understanding and modeling the climatic impacts of stratospheric aerosols. It relies primarily on data from Gas Experiment (SAGE) satellite series, supplemented by Optical Spectrograph Infrared Imaging System (OSIRIS) Cloud-Aerosol Lidar Pathfinder Satellite Observations (CALIPSO). GloSSAC currently provides aerosol extinction coefficients optical depths at 525 1020 nm. With CALIPSO decommissioned OSIRIS nearing end its operational life, SAGE III/ISS (International Space Station) will soon become sole source GloSSAC, but it only be available as long ISS operational, until around 2030. Therefore, incorporating other measurements, such those Ozone Mapping Profiler Suite Limb (OMPS-LP), critical. OMPS-LP has provided continuous coefficient measurements since 2012 with a retrieval algorithm developed NASA, i.e., OMPS(NASA). However, OMPS(NASA) been shown to overestimate coefficients, particularly after 2022 Hunga Tonga eruption, compared tomographic OMPS University Saskatchewan (OMPS(SASK)) III/ISS. Our analysis shows that indeed exhibits consistently high bias (>50 %) following large volcanic eruptions pyrocumulonimbus plumes intense wildfires, while OMPS(SASK) reasonable agreement between 40° S N. This overestimation leads an effective radiative forcing (ERF) associated model-simulated global surface temperature response factor about 2.

Language: Английский

Citations

0

Retrieval of stratospheric aerosol extinction coefficients from sun-normalized Ozone Mapper and Profiler Suite Limb Profiler (OMPS-LP) measurements DOI Creative Commons
Alexei Rozanov, Christine Pohl, Carlo Arosio

et al.

Atmospheric measurement techniques, Journal Year: 2024, Volume and Issue: 17(22), P. 6677 - 6695

Published: Nov. 25, 2024

Abstract. A new retrieval approach for obtaining vertical profiles of the aerosol extinction coefficient from measurements scattered solar light in limb-viewing geometry made by Ozone Mapper and Profiler Suite Limb (OMPS-LP) instrument is presented. In contrast to many other published limb-scatter retrievals, our algorithm does not employ normalization a limb measurement at an upper tangent height. Instead, measured radiances are normalized irradiance. The main advantage this almost complete elimination dependence results on prior profile used retrieval. This makes better suited analysis observation scenes with highly elevated plumes, such as those that occurred after Hunga Tonga–Hunga Ha′apai volcanic eruption January 2022. were compared coefficients retrieved Stratospheric Aerosol Gas Experiment III International Space Station (SAGE III/ISS) Optical Spectrograph InfraRed Imaging System (OSIRIS). general, agreement within 25 % between different data products was observed 18–23 km altitude range, although larger differences seen very strong eruptions wildfires. comparison OSIRIS, high southern latitudes (above 60° S). product investigate evolution plume eruption.

Language: Английский

Citations

3