Global perspectives on the biodegradation of LDPE in agricultural systems DOI Creative Commons
Jani E. Mendoza, Daniel Tineo, Beimer Chuquibala-Checan

et al.

Frontiers in Microbiology, Journal Year: 2025, Volume and Issue: 15

Published: Jan. 7, 2025

The increasing use of plastics globally has generated serious environmental and human health problems, particularly in the agricultural sector where low-density polyethylene (LDPE) other are widely used. Due to its low recycling rate slow degradation process, LDPE is a major source pollution. This paper addresses problem plastic accumulation agriculture, focusing on biodegradation strategies. studies reviewed include recent data methodologies used state-of-the-art technologies others that have been for decades, monitor measure degree each treatment applied can have, including SEM, GCMS, HPLC, microscopy. countries investigating these identified, while some developing them years, only begun address this years. microorganisms such as bacteria, fungi, algae, insect larvae influence decomposition highlighted. A workflow proposed carry out type research. Despite advances, challenges remain, optimizing conditions accelerate process need further research delves into microbial interactions various contexts.

Language: Английский

Microplastic detection and remediation through efficient interfacial solar evaporation for immaculate water production DOI Creative Commons

Zhen Yu,

Yang Li, Yaoxin Zhang

et al.

Nature Communications, Journal Year: 2024, Volume and Issue: 15(1)

Published: July 19, 2024

Freshwater scarcity and microplastics (MPs) pollution are two concerning intertwined global challenges. In this work, we propose a "one stone kills birds" strategy by employing an interfacial solar evaporation platform (ISEP) combined with MPs adsorbent. This aims to produce clean water simultaneously enhance removal. Unlike traditional predecessors, our ISEP generates condensed free from contamination. Additionally, the photothermally driven separation process significantly improves removal performance. We observed ratio increase of up 5.5 times compared previously reported adsorbents. Thus, rationally-designed holds promising potential not only mitigate existing issue but also remediate in natural environments.

Language: Английский

Citations

30

Enzymatic Mesoporous Metal Nanocavities for Concurrent Electrocatalysis of Nitrate to Ammonia Coupled with Polyethylene Terephthalate Upcycling DOI

Lizhi Sun,

Hao Lv, Jie Xiao

et al.

Advanced Materials, Journal Year: 2024, Volume and Issue: 36(27)

Published: April 9, 2024

Electrochemical upcycling of waste pollutants into high value-added fuels and/or chemicals is recognized as a green and sustainable solution that can address the resource utilization on earth. Despite great efforts, their progress has seriously been hindered by lack high-performance electrocatalysts. In this work, bimetallic PdCu mesoporous nanocavities (MCs) are reported new bifunctional enzymatic electrocatalyst realizes concurrent electrocatalytic nitrate wastewater polyethylene terephthalate (PET) plastic waste. Abundant metal mesopores open MCs provide confinement key intermediates for deeper electroreduction accelerate transport reactants/products within/out electrocatalyst, thus affording ammonia Faradic efficiency (FE

Language: Английский

Citations

19

Pseudomonas putida as a synthetic biology chassis and a metabolic engineering platform DOI Creative Commons
Esteban Martínez‐García, Vı́ctor de Lorenzo

Current Opinion in Biotechnology, Journal Year: 2023, Volume and Issue: 85, P. 103025 - 103025

Published: Dec. 7, 2023

The soil bacterium Pseudomonas putida, especially the KT2440 strain, is increasingly being utilized as a host for biotransformations of both industrial and environmental interest. foundations such performance include its robust redox metabolism, ability to tolerate wide range physicochemical stresses, rapid growth, versatile nonpathogenic nature, availability molecular tools advanced genetic programming. These attributes have been leveraged hosting engineered pathways production valuable chemicals or degradation/valorization pollutants. This has in turn pushed boundaries conventional enzymology toward previously unexplored reactions nature. Furthermore, modifications physical properties cells made enhance their catalytic performance. advancements establish P. putida bona fide chassis synthetic biology, on par with more traditional metabolic engineering platforms.

Language: Английский

Citations

33

Lifecycle Management for Sustainable Plastics: Recent Progress from Synthesis, Processing to Upcycling DOI
Shuangqiao Yang, Yijun Li, Min Nie

et al.

Advanced Materials, Journal Year: 2024, Volume and Issue: 36(33)

Published: June 13, 2024

Abstract Plastics, renowned for their outstanding properties and extensive applications, assume an indispensable irreplaceable role in modern society. However, the ubiquitous consumption of plastic items has led to a growing accumulation waste. Unreasonable practices production, utilization, recycling plastics have substantial energy resource depletion environmental pollution. Herein, state‐of‐the‐art advancements lifecycle management are timely reviewed. Unlike typical reviews focused on recycling, this work presents in‐depth analysis entire plastics, covering whole process from synthesis, processing, ultimate disposal. The primary emphasis lies selecting judicious strategies methodologies at each stage mitigate adverse impact waste plastics. Specifically, article delineates rationale, methods, realized various stages through both physical chemical pathways. focal point is attainment optimal rates thereby alleviating ecological burden By scrutinizing aims furnish comprehensive solutions reducing pollution fostering sustainability across all facets

Language: Английский

Citations

15

Recent advances in microbial and enzymatic engineering for the biodegradation of micro- and nanoplastics DOI Creative Commons
Jaewon Choi, Hong Bin Kim,

Yu‐Rim Ahn

et al.

RSC Advances, Journal Year: 2024, Volume and Issue: 14(14), P. 9943 - 9966

Published: Jan. 1, 2024

This review examines the escalating issue of plastic pollution, specifically highlighting detrimental effects on environment and human health caused by microplastics nanoplastics.

Language: Английский

Citations

14

Interface Engineering on Heterostructural Nanosheets for Efficient Electrocatalytic-Paired Upcycling of Waste Plastics and Nitrate DOI
Junhua Wu,

Xiaoxiao Cheng,

Yun Tong

et al.

ACS Catalysis, Journal Year: 2024, Volume and Issue: unknown, P. 18095 - 18106

Published: Nov. 22, 2024

Language: Английский

Citations

14

Compositional and temporal division of labor modulates mixed sugar fermentation by an engineered yeast consortium DOI Creative Commons
Jonghyeok Shin, Siqi Liao, Nurzhan Kuanyshev

et al.

Nature Communications, Journal Year: 2024, Volume and Issue: 15(1)

Published: Jan. 26, 2024

Synthetic microbial communities have emerged as an attractive route for chemical bioprocessing. They are argued to be superior single strains through division of labor (DOL), but the exact mechanism by which DOL confers advantages remains unclear. Here, we utilize a synthetic Saccharomyces cerevisiae consortium along with mathematical modeling achieve tunable mixed sugar fermentation overcome limitations single-strain fermentation. The involves two each specializing in glucose or xylose utilization ethanol production. By controlling initial community composition, allows fine tuning dynamics and product generation. altering inoculation delay, provides additional programmability parallelly regulate characteristics yield. Mathematical models capture observed experimental findings further offer guidance subsequent optimization. This study demonstrates functional potential bioprocessing insight into rational design engineered ecosystems various applications.

Language: Английский

Citations

11

Biochar immobilized hydrolase degrades PET microplastics and alleviates the disturbance of soil microbial function via modulating nitrogen and phosphorus cycles DOI
Huawen Han, Peizhi Song,

Yuchao Jiang

et al.

Journal of Hazardous Materials, Journal Year: 2024, Volume and Issue: 474, P. 134838 - 134838

Published: June 5, 2024

Language: Английский

Citations

11

A model-driven approach to upcycling recalcitrant feedstocks in Pseudomonas putida by decoupling PHA production from nutrient limitation DOI Creative Commons
Maria‐Tsampika Manoli, A. Gargantilla Becerra, Carlos del Cerro

et al.

Cell Reports, Journal Year: 2024, Volume and Issue: 43(4), P. 113979 - 113979

Published: March 22, 2024

Bacterial polyhydroxyalkanoates (PHAs) have emerged as promising eco-friendly alternatives to petroleum-based plastics since they are synthesized from renewable resources and offer exceptional properties. However, their production is limited the stationary growth phase under nutrient-limited conditions, requiring customized strategies costly two-phase bioprocesses. In this study, we tackle these challenges by employing a model-driven approach reroute carbon flux remove regulatory constraints using synthetic biology. We construct collection of Pseudomonas putida-overproducing strains at expense lignin-related compounds growth-coupling approaches. PHA was successfully achieved during phase, resulting in up 46% PHA/cell dry weight while maintaining balanced carbon-to-nitrogen ratio. Our additionally validated an upcycling scenario enzymatically hydrolyzed polyethylene terephthalate feedstock. These findings potential revolutionize address global plastic crisis overcoming complexities traditional

Language: Английский

Citations

8

Upcycling of polyethylene terephthalate to 1,4-cyclohexanedimethanol in water DOI

Shuhui Fang,

Zhiwen Gao,

Xinrui Shi

et al.

Science China Chemistry, Journal Year: 2025, Volume and Issue: unknown

Published: Jan. 3, 2025

Language: Английский

Citations

1