Carbon capture and storage (CCS): the way forward

Energy & Environmental Science, Journal Year: 2018, Volume and Issue: 11(5), P. 1062 - 1176

Published: Jan. 1, 2018

Carbon capture and storage (CCS) is vital to climate change mitigation, has application across the economy, in addition facilitating atmospheric carbon dioxide removal resulting emissions offsets net negative emissions. This contribution reviews state-of-the-art identifies key challenges which must be overcome order pave way for its large-scale deployment.

Language: Английский

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Carbon capture and conversion using metal–organic frameworks and MOF-based materials

Chemical Society Reviews, Journal Year: 2019, Volume and Issue: 48(10), P. 2783 - 2828

Published: Jan. 1, 2019

Rapidly increasing atmospheric CO2 concentrations threaten human society, the natural environment, and synergy between two. In order to ameliorate problem, carbon capture conversion techniques have been proposed. Metal-organic framework (MOF)-based materials, a relatively new class of porous materials with unique structural features, high surface areas, chemical tunability stability, extensively studied respect their applicability such techniques. Recently, it has become apparent that capabilities MOF-based significantly boost potential toward conversion. Furthermore, materials' well-defined structures greatly facilitate understanding structure-property relationships roles in this review, we provide comprehensive account significant progress design synthesis including MOFs, MOF composites derivatives, application Special emphases on capacities catalytic performances are discussed.

Language: Английский

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Industrial carbon dioxide capture and utilization: state of the art and future challenges

Chemical Society Reviews, Journal Year: 2020, Volume and Issue: 49(23), P. 8584 - 8686

Published: Jan. 1, 2020

This review covers the sustainable development of advanced improvements in CO₂capture and utilization.

Language: Английский

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Efficient, selective and sustainable catalysis of carbon dioxide

Green Chemistry, Journal Year: 2017, Volume and Issue: 19(16), P. 3707 - 3728

Published: Jan. 1, 2017

The efficient and selective conversion of CO₂as a sustainable C₁resource into valuable chemicals energy-related products through catalysis is reviewed.

Language: Английский

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Ionic-Liquid-Based CO₂ Capture Systems: Structure, Interaction and Process

Chemical Reviews, Journal Year: 2017, Volume and Issue: 117(14), P. 9625 - 9673

Published: July 7, 2017

The inherent structure tunability, good affinity with CO2, and nonvolatility of ionic liquids (ILs) drive their exploration exploitation in CO2 separation field, has attracted remarkable interest from both industries academia. aim this Review is to give a detailed overview on the recent advances IL-based materials, including pure ILs, solvents, membranes for capture viewpoint molecule engineering. effects anions, cations functional groups solubility selectivity as well studies degradability ILs are reviewed, developments functionalized also discussed. mechanism solvents explained by combining molecular simulation experimental characterization. Taking into consideration applications industrialization, achievements transport properties IL fluids process design processes highlighted. Finally, future research challenges perspectives commercialization materials posed.

Language: Английский

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Emerging trends in porous materials for CO₂capture and conversion

Chemical Society Reviews, Journal Year: 2020, Volume and Issue: 49(13), P. 4360 - 4404

Published: Jan. 1, 2020

The presence of an excessive concentration CO2 in the atmosphere needs to be curbed with suitable measures including reduction emissions at stationary point sources such as power plants through carbon capture technologies and subsequent conversion captured into non-polluting clean fuels/chemicals using photo and/or electrocatalytic pathways. Porous materials have attracted much attention for recent past; they witnessed significant advancements their design implementation conversion. In this context, emerging trends major porous adsorbents MOFs, zeolites, POPs, carbons, mesoporous are discussed. Their surface texture chemistry, influence various other features on efficiency, selectivity, recyclability explained compared thoroughly. scientific technical advances material structure versus provide deep insights designing effective materials. review concludes a summary, which compiles key challenges field, current critical development materials, future research directions combined possible solutions realising deployment

Language: Английский

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Are Ionic Liquids Chemically Stable?

Chemical Reviews, Journal Year: 2017, Volume and Issue: 117(10), P. 7113 - 7131

Published: Feb. 27, 2017

Ionic liquids have attracted a great deal of interest in recent years, illustrated by their applications variety areas involved with chemistry, physics, biology, and engineering. Usually, the stabilities ionic are highlighted as one outstanding advantages. However, really stable all cases? This review covers chemical liquids. It focuses on reactivity most popular imidazolium at structural positions, including C2 position, N1 N3 C4 C5 decomposition ring. Additionally, we discuss quaternary ammonium phosphonium hydrolysis nucleophilic reactions anions The aims to arouse caution potential provides guide for better utilization

Language: Английский

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The peculiar effect of water on ionic liquids and deep eutectic solvents

Chemical Society Reviews, Journal Year: 2018, Volume and Issue: 47(23), P. 8685 - 8720

Published: Jan. 1, 2018

Comprehensive review of unique effects water on ionic liquids and deep eutectic solvents observed in experimental theoretical studies.

Language: Английский

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Water-Lean Solvents for Post-Combustion CO₂Capture: Fundamentals, Uncertainties, Opportunities, and Outlook

Chemical Reviews, Journal Year: 2017, Volume and Issue: 117(14), P. 9594 - 9624

Published: June 19, 2017

This review is designed to foster the discussion regarding viability of postcombustion CO2 capture by water-lean solvents, separating fact from fiction for both skeptics and advocates. We highlight unique physical thermodynamic properties notable with a how such could translate efficiency gains compared aqueous amines. The scope this ranges purely fundamental molecular-level processes that govern solvent behavior bench-scale testing, through process engineering projections performance cost. Key discussions higher than expected mass transfer, water tolerance, compatibility current infrastructure are presented along limitations suggested areas where further development needed. conclude an outlook status field assess solvents capture.

Language: Английский

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Carbon dioxide capture using liquid absorption methods: a review

Environmental Chemistry Letters, Journal Year: 2020, Volume and Issue: 19(1), P. 77 - 109

Published: Sept. 18, 2020

Language: Английский

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