Degradable and Recyclable Solar Desalination Membranes Based on Naturally Occurring Building Blocks DOI
Ning Li, Yuan Zou, Xueqian Zhang

et al.

Chemistry of Materials, Journal Year: 2022, Volume and Issue: 34(23), P. 10399 - 10408

Published: Nov. 21, 2022

Solar steam generation is a robust and environmentally friendly way to obtain fresh water alleviate the shortage problem. Although wide variety of devices have been well documented, most fabricated materials are often only suitable for one device generally difficult be removed, resulting in disposable device. This may raise serious concerns about total cost issues, particularly those with complex well-tailored microstructures. Thus, it urgent develop dynamic photothermal coating that can easily removed flexibly switched between different installations stable conversion ability. In this work, we report degradable recyclable metal-phenolic network-based assembled from two kinds naturally occurring building blocks [gallic acid (GA) Fe(III)]. Hydrophilic poly(vinylidene fluoride) (PVDF) was selected as substrate, GA@Fe(III)@PVDF membrane, which achieve high evaporation rate 1.539 kg m–2 h–1 superb efficiency 90.2% under 1 sun illumination. Impressively, GA@Fe(III) degraded acidic condition rapidly, recovered PVDF recoated by networks again. The performance remain over 150 degrading recoating cycles. We believed work could offer opportunities fabricate low-cost, sustainable, coatings solar generation.

Language: Английский

Bioinspired polydopamine hydrogels: Strategies and applications DOI
Yuanting Xu, Junfei Hu, Jingjing Hu

et al.

Progress in Polymer Science, Journal Year: 2023, Volume and Issue: 146, P. 101740 - 101740

Published: Sept. 17, 2023

Language: Английский

Citations

110

A robust and 3D-printed solar evaporator based on naturally occurring molecules DOI
Xueqian Zhang, Yan Yu, Ning Li

et al.

Science Bulletin, Journal Year: 2023, Volume and Issue: 68(2), P. 203 - 213

Published: Jan. 1, 2023

Language: Английский

Citations

107

Programmed microalgae-gel promotes chronic wound healing in diabetes DOI Creative Commons
Yong Kang, Lingling Xu,

Jinrui Dong

et al.

Nature Communications, Journal Year: 2024, Volume and Issue: 15(1)

Published: Feb. 3, 2024

Abstract Chronic diabetic wounds are at lifelong risk of developing foot ulcers owing to severe hypoxia, excessive reactive oxygen species (ROS), a complex inflammatory microenvironment, and the potential for bacterial infection. Here we develop programmed treatment strategy employing live Haematococcus (HEA). By modulating light intensity, HEA can be perform variety functions, such as antibacterial activity, supply, ROS scavenging, immune regulation, suggesting its use in therapy. Under high intensity (658 nm, 0.5 W/cm 2 ), green (GHEA) with efficient photothermal conversion mediate wound surface disinfection. decreasing 0.1 photosynthetic system GHEA continuously produce oxygen, effectively resolving problems hypoxia promoting vascular regeneration. Continuous irradiation induces astaxanthin (AST) accumulation cells, resulting gradual transformation from red hue (RHEA). RHEA scavenges excess ROS, enhances expression intracellular antioxidant enzymes, directs polarization M2 macrophages by secreting AST vesicles via exosomes. The living hydrogel sterilize enhance cell proliferation migration promote neoangiogenesis, which could improve infected healing female mice.

Language: Английский

Citations

101

Biochar as Sustainable Alternative and Green Adsorbent for the Remediation of Noxious Pollutants: A Comprehensive Review DOI Creative Commons

Stuti Jha,

Rama Gaur, Syed Shahabuddin

et al.

Toxics, Journal Year: 2023, Volume and Issue: 11(2), P. 117 - 117

Published: Jan. 25, 2023

The current water crisis necessitates the development of new materials for wastewater treatment. A variety nanomaterials are continuously being investigated their potential as adsorbents environmental remediation. Researchers intend to develop a low-cost, simple, and sustainable material that can cater removal pollutants. Biochar derived from biowaste is candidate existing problem pollution. review focuses on various aspects biochar, such its sources, preparation methods, mechanism, applications treatment, regeneration. Compared with other adsorbents, biochar considered an environmentally friendly, sustainable, cost-effective substitute waste management, climate protection, soil improvement, etc. special properties porosity, surface area, charge, functional groups be easily modified by chemical resulting in improved adsorption properties. Therefore, view increasing pollution problems encountered researchers treating pollutants, great importance. This also highlights challenges prospective areas explored studied more detail future.

Language: Английский

Citations

98

A bioinspired antibacterial and photothermal membrane for stable and durable clean water remediation DOI

Yiyan Yang,

Lei Yang,

Fengying Yang

et al.

Materials Horizons, Journal Year: 2022, Volume and Issue: 10(1), P. 268 - 276

Published: Nov. 8, 2022

The tobramycin-doped polydopamine nanoparticles were developed to construct solar evaporator, which exhibited synergistic antibacterial behaviors and high water evaporation rate, thus achieving stable reuse even under microbe-rich environment.

Language: Английский

Citations

81

Cellulose‐based Interfacial Solar Evaporators: Structural Regulation and Performance Manipulation DOI
Weijie Wu, Yuanting Xu,

Xiaofan Ma

et al.

Advanced Functional Materials, Journal Year: 2023, Volume and Issue: 33(36)

Published: May 15, 2023

Abstract The shortage of freshwater resources has become a major obstacle threatening human development, and directly utilizing solar energy by evaporators is emerging as promising method to produce from the seawater. Compared many synthetic polymer‐based evaporators, cellulose‐based are expected offer more interesting features benefiting renewable feature abundant reserves cellulose‐contained naturally occurring materials. First, according different fabrication methods, can be divided into two types, i.e., top‐down utilization (wood‐based) bottom‐up assembled (cellulose composite‐based), respectively. schemes also bring their own unique advantages, such bimodal porous structure wood‐based artificial interconnection microporous network cellulose composite‐based evaporators. Subsequently, this review further summarizes most recent advances highlights those focusing on structural regulation strategies (e.g., drilled channel array, asymmetric wettability structure, delignification, 2D waterway, etc.) evaporation performance improvements salt resistance, high rate, etc.). Finally, challenges in field potential solutions discussed, which anticipated provide new opportunities toward future development other kinds biomass‐based

Language: Английский

Citations

75

A melanin-inspired robust aerogel for multifunctional water remediation DOI
Peng Yang,

Wanjie Bai,

Yuan Zou

et al.

Materials Horizons, Journal Year: 2023, Volume and Issue: 10(3), P. 1020 - 1029

Published: Jan. 1, 2023

Solar-driven vapor generation has emerged as a promising wastewater remediation technology for clean water production. However, the complicated and diversified contaminants in still restrict its practical applications. Herein, inspired by melanin nature, robust aerogel was facilely fabricated multifunctional via one-pot condensation copolymerization of 5,6-dihydroxyindole formaldehyde. Benefiting from superhydrophilicity, underwater superoleophobicity, synergistic coordination effects, resulting not only showed excellent performances oil resistance oil-water separation ability, but also removed organic dyes heavy metal ions simultaneously. Moreover, owing to admirable light harvesting capacity porous microstructure fast transportation, aerogel-based evaporator exhibited an evaporation rate 1.42 kg m-2 h-1 with 91% efficiency under 1 sun illumination, which can be reused long-term evaporation. Note that such stable could maintained even containing complex multicomponent contaminants. Outdoor experiments lotus pond natural sunlight proved great potential All those features this all-in-one melanin-inspired may provide new strategies development photothermal devices solar-driven remediation.

Language: Английский

Citations

73

Photocatalytic Degradation of Methylene Blue Dye from Wastewater by Using Doped Zinc Oxide Nanoparticles DOI Open Access

Shreya Modi,

Virendra Kumar Yadav, Abdelfattah Amari

et al.

Water, Journal Year: 2023, Volume and Issue: 15(12), P. 2275 - 2275

Published: June 17, 2023

ZnO is a semiconductor material that has important physical and chemical properties, which are frequently significantly enhanced by the addition of impurities, such as doping. A study structural properties pristine functionalized (i.e., doped with Antimony Tungsten) nanoparticles been conducted for photocatalyst-based degradation methylene blue (MB) dye under both Ultraviolet (UV) solar light. Authors have used 1% concentration dopant doping purposes. The synthesized materials were characterized analysis, functional group identification, spectroscopic measurements, morphological examination using X-ray diffraction (XRD), Fourier transform-infrared (FTIR), UV-Vis spectroscopy (UV-Vis), Field emission scanning electron microscope (FESEM) techniques. XRD analysis confirmed synthesized-doped retained wurtzite hexagonal structure purity 99%. Transmission (TEM) data reveals average size pure ZnO-NPs was found to be 7 nm; after increased 18 nm 9.55 nm, respectively, ZnO-W ZnO-Sb. As per FESEM results, minor changes observed Differential reflectance UV-DRS revealed confirmation antimony tungsten, exhibited shift. decrease in band-gap on makes more efficient photocatalytic applications. efficiency catalysts (PCD) analyzed UV irradiation. This effect pH, nano-photocatalyst dose, initial (ICD) PCD MB. obtained analytical results showed ideal conditions MB follows: pH = 9, quantity 300 mg/L, an dose 10 ppm. These lead about 91% ZnO-Sb exposure radiation. reusability also stability nano-photocatalysts. current research may pave way removal hazardous dyes from wastewater discharged many industries.

Language: Английский

Citations

66

Advanced Polymeric Nanocomposite Membranes for Water and Wastewater Treatment: A Comprehensive Review DOI Open Access
Abhispa Sahu, Raghav Dosi, Carly O. Kwiatkowski

et al.

Polymers, Journal Year: 2023, Volume and Issue: 15(3), P. 540 - 540

Published: Jan. 20, 2023

Nanomaterials have been extensively used in polymer nanocomposite membranes due to the inclusion of unique features that enhance water and wastewater treatment performance. Compared pristine membranes, incorporation nanomodifiers not only improves membrane performance (water permeability, salt rejection, contaminant removal, selectivity), but also intrinsic properties (hydrophilicity, porosity, antifouling properties, antimicrobial mechanical, thermal, chemical stability) these membranes. This review focuses on applications different types nanomaterials: zero-dimensional (metal/metal oxide nanoparticles), one-dimensional (carbon nanotubes), two-dimensional (graphene associated structures), three-dimensional (zeolites frameworks) nanomaterials combined with polymers towards novel polymeric nanocomposites for applications. will show combinations impart enhanced into membrane; however, underlying issues modification processes environmental impact are less obvious. highlights utility computational methods toward understanding structural functional Here, we highlight fabrication methods, advantages, challenges, impact, future scope advanced based systems

Language: Английский

Citations

58

MXene-PVA-TiO2-based photothermal-catalytic membrane with high structural stability for efficient desalination and photodegradation DOI
Jiawei Sun, Muhammad Usman Farid, Min Wei Boey

et al.

Chemical Engineering Journal, Journal Year: 2023, Volume and Issue: 468, P. 143744 - 143744

Published: May 26, 2023

Language: Английский

Citations

45