Atmospheric chemistry and physics,
Journal Year:
2024,
Volume and Issue:
24(6), P. 3883 - 3904
Published: April 2, 2024
Abstract.
Arctic
air
masses
undergo
intense
transformations
when
moving
southward
from
closed
sea
ice
to
warmer
open
waters
in
marine
cold-air
outbreaks
(CAOs).
Due
the
lack
of
measurements
diabatic
heating
and
moisture
uptake
rates
along
CAO
flows,
studies
often
depend
on
atmospheric
reanalysis
output.
However,
uncertainties
connected
those
datasets
remain
unclear.
Here,
we
present
height-resolved
airborne
observations
heating,
uptake,
cloud
evolution
measured
a
quasi-Lagrangian
manner.
The
investigated
was
observed
1
April
2022
during
HALO-(AC)3
campaign.
Shortly
after
passing
sea-ice
edge,
maximum
over
6
K
h−1
0.3
gkg-1h-1
were
near
surface.
Clouds
started
forming
vertical
mixing
within
deepening
boundary
layer
intensified.
are
compared
with
fifth-generation
global
(ERA5)
Copernicus
Regional
Reanalysis
(CARRA).
Compared
these
observations,
mean
absolute
errors
ERA5
versus
CARRA
data
14
%
higher
for
temperature
(1.14
1.00
K)
62
specific
humidity
ice-free
ocean
(0.112
g
kg−1
0.069
kg−1).
We
relate
differences
issues
representation
marginal
zone
corresponding
surface
fluxes
ERA5,
as
well
scheme
producing
excess
liquid-bearing,
precipitating
clouds,
which
causes
too-dry
layer.
CARRA's
high
spatial
resolution
demonstrated
fidelity
towards
make
it
promising
candidate
further
mass
transformations.
Journal of Advances in Modeling Earth Systems,
Journal Year:
2023,
Volume and Issue:
15(3)
Published: March 1, 2023
Abstract
Pollen,
one
type
of
primary
biological
aerosol
particle
(PBAP),
is
emitted
from
the
terrestrial
biosphere
and
can
undergo
physical
changes
in
atmosphere
via
rupture.
To
examine
fate
pollen
its
atmospheric
processing,
a
emission
transport
scheme
coupled
to
Weather
Research
Forecasting
Model
with
Chemistry
(WRF‐Chem).
We
simulate
impacts
on
cloud
properties
precipitation
Southern
Great
Plains
12
19
April
2013,
period
both
high
emissions
convective
activity.
conduct
suite
ensemble
runs
that
three
different
rupture
mechanisms
generate
subpollen
particles,
including
(a)
humidity‐induced
surface
rupture,
(b)
in‐atmosphere
plus
(c)
lightning‐induced
where
in‐cloud
cloud‐to‐ground
lightning
strikes
trigger
events.
When
relative
humidity
(>80%),
coarse
(∼1
μg
m
−3
)
converted
into
fine
particles
(∼1.2e
−4
),
which
produces
80%
more
than
The
humidity‐driven
predominantly
further
enhanced
during
frontal
thunderstorm.
During
strong
convection,
vertical
updrafts
lift
(∼0.5e
upper
troposphere
(∼12
km)
laterally
transports
ruptured
anvil
top
outflow.
In
regions
influence
warm
formation
by
decreasing
low
(<4
water
mixing
ratios
increasing
ice
phase
hydrometeors
aloft
(>10
km).
Geophysical Research Letters,
Journal Year:
2023,
Volume and Issue:
50(18)
Published: Sept. 14, 2023
Abstract
The
estimation
of
cloud
radiative
forcing
due
to
aerosol‐cloud
interactions,
RF
aci
(also
known
as
the
first
indirect
effect),
relies
on
approximating
albedo
susceptibility
changes
in
droplet
concentration,
β
.
depends
and
both
which
can
be
observed
by
satellites.
Satellite
observations
are
often
spatially
aggregated
coarser
resolutions,
typically
1
×
1°
scenes.
However,
such
spatial
scales,
tends
heterogeneous,
whereas
approximation
assumes
homogeneity.
Here,
we
demonstrate
that
common
practice
aggregating
satellite
data
neglecting
heterogeneity
results
an
average
overestimation
10%
previous
estimates
Additionally,
establish
a
relationship
between
magnitude
bias
Stratocumulus
morphologies,
providing
physical
context
for
associated
bias.
Lastly,
propose
correction
method
applied
gridded
data.
Atmospheric chemistry and physics,
Journal Year:
2023,
Volume and Issue:
23(16), P. 9365 - 9383
Published: Aug. 24, 2023
Abstract.
Marine
cold-air
outbreaks
are
important
parts
of
the
high-latitude
climate
system
and
characterised
by
strong
surface
fluxes
generated
air–sea
temperature
gradient.
These
promote
cloud
formation,
which
can
be
identified
in
satellite
imagery
distinct
transformation
stratiform
“streets”
into
a
broken
field
cumuliform
clouds
downwind
outbreak.
This
evolution
morphology
changes
radiative
properties
therefore
is
importance
to
energy
budget.
While
drivers
stratocumulus-to-cumulus
transitions,
such
as
aerosols
or
sea
gradient,
have
been
extensively
studied
for
subtropical
clouds,
factors
influencing
transitions
at
higher
latitudes
relatively
poorly
understood.
work
uses
reanalysis
data
create
set
composite
trajectories
moving
off
Arctic
ice
edge
co-locates
these
with
generate
unique
view
liquid-dominated
development
within
outbreaks.
The
results
this
analysis
show
that
embedded
distinctive
relative
following
other
region.
initial
strength
outbreak
shows
lasting
effect
on
properties,
differences
between
weak
events
visible
over
30
h
after
air
has
left
edge.
However,
while
(measured
magnitude
marine
index)
affects
it
does
not
affect
timing
transition
top-of-atmosphere
albedo.
In
contrast,
aerosol
conditions
do
strongly
but
correlated
break-up,
leading
an
enhanced
cooling
through
high-aerosol
due
delayed
break-up.
Both
environment
frequency
expected
change
future
Arctic,
provide
insight
how
will
clouds.
also
highlight
need
information
about
present-day
sources
correctly
model
development.
Atmospheric chemistry and physics,
Journal Year:
2024,
Volume and Issue:
24(5), P. 2913 - 2935
Published: March 6, 2024
Abstract.
Warm
boundary
layer
clouds
in
the
eastern
North
Atlantic
region
exhibit
significant
diurnal
variations
cloud
properties.
However,
cycle
of
aerosol
indirect
effect
(AIE)
for
these
remains
poorly
understood.
This
study
takes
advantage
recent
advancements
spatial
resolution
geostationary
satellites
to
explore
daytime
variation
AIE
by
estimating
susceptibilities
changes
droplet
number
concentration
(Nd).
Cloud
retrievals
month
July
over
4
years
(2018–2021)
from
Spinning
Enhanced
Visible
and
Infrared
Imager
(SEVIRI)
on
Meteosat-11
this
are
analyzed.
Our
results
reveal
a
“U-shaped”
liquid
water
path
(LWP),
albedo,
fraction.
Clouds
found
be
more
susceptible
Nd
perturbations
at
noon
less
morning
evening.
The
magnitude
sign
depend
heavily
state
defined
LWP
precipitation
conditions.
Non-precipitating
thin
account
44
%
all
warm
July,
they
contribute
most
observed
variation.
thick
least
frequent
(10
%),
negative
albedo
compared
clouds.
Precipitating
dominant
(46
but
their
show
minimal
throughout
day.
We
find
evidence
that
non-precipitating
is
influenced
combination
transition
between
“lagged”
responses
perturbations.
fraction
susceptibility
can
attributed
morphology
(e.g.,
overcast
or
broken).
dissipation
development
do
not
adequately
explain
susceptibilities.
Additionally,
primarily
driven
intensity
response
rather
than
frequency
occurrence
states.
imply
polar-orbiting
with
an
overpass
time
13:30
LT
underestimate
mean
values
susceptibility,
as
observe
daily
minima
region.
Atmospheric chemistry and physics,
Journal Year:
2024,
Volume and Issue:
24(6), P. 3883 - 3904
Published: April 2, 2024
Abstract.
Arctic
air
masses
undergo
intense
transformations
when
moving
southward
from
closed
sea
ice
to
warmer
open
waters
in
marine
cold-air
outbreaks
(CAOs).
Due
the
lack
of
measurements
diabatic
heating
and
moisture
uptake
rates
along
CAO
flows,
studies
often
depend
on
atmospheric
reanalysis
output.
However,
uncertainties
connected
those
datasets
remain
unclear.
Here,
we
present
height-resolved
airborne
observations
heating,
uptake,
cloud
evolution
measured
a
quasi-Lagrangian
manner.
The
investigated
was
observed
1
April
2022
during
HALO-(AC)3
campaign.
Shortly
after
passing
sea-ice
edge,
maximum
over
6
K
h−1
0.3
gkg-1h-1
were
near
surface.
Clouds
started
forming
vertical
mixing
within
deepening
boundary
layer
intensified.
are
compared
with
fifth-generation
global
(ERA5)
Copernicus
Regional
Reanalysis
(CARRA).
Compared
these
observations,
mean
absolute
errors
ERA5
versus
CARRA
data
14
%
higher
for
temperature
(1.14
1.00
K)
62
specific
humidity
ice-free
ocean
(0.112
g
kg−1
0.069
kg−1).
We
relate
differences
issues
representation
marginal
zone
corresponding
surface
fluxes
ERA5,
as
well
scheme
producing
excess
liquid-bearing,
precipitating
clouds,
which
causes
too-dry
layer.
CARRA's
high
spatial
resolution
demonstrated
fidelity
towards
make
it
promising
candidate
further
mass
transformations.