Abstract.
The
effective
radiative
forcing
due
to
aerosol-cloud
interactions
(ERFaci)
is
difficult
quantify,
leading
large
uncertainties
in
model
projections
of
historical
and
climate
sensitivity.
In
this
study,
satellite
observations
reanalysis
data
are
used
examine
the
low-level
cloud
responses
aerosols.
While
some
studies
it
assumed
that
activation
rate
droplet
number
concentration
(Nd)
response
variations
sulfate
aerosols
(SO4)
or
aerosol
index
(AI)
has
a
one-to-one
relationship
estimation
ERFaci,
we
find
assumption
be
incorrect,
demonstrate
explicitly
accounting
for
crucial
accurate
ERFaci
estimation.
This
corroborated
through
“perfect-model”
cross
validation
using
state-of-the-art
models,
which
compares
our
estimates
with
“true”
ERFaci.
Our
results
suggest
smaller
less
uncertain
value
global
than
previous
(-0.39
±
0.29
W
m-2
SO4
-0.24
0.18
AI,
90
%
confidence),
indicating
may
impactful
previously
thought.
also
consistent
observationally
constrained
total
feedback
“top-down”
models
weaker
better
match
observed
hemispheric
warming
asymmetry
over
period.
Oxford Open Climate Change,
Journal Year:
2023,
Volume and Issue:
3(1)
Published: Jan. 1, 2023
Abstract
Improved
knowledge
of
glacial-to-interglacial
global
temperature
change
yields
Charney
(fast-feedback)
equilibrium
climate
sensitivity
1.2
±
0.3°C
(2σ)
per
W/m2,
which
is
4.8°C
1.2°C
for
doubled
CO2.
Consistent
analysis
over
the
full
Cenozoic
era—including
‘slow’
feedbacks
by
ice
sheets
and
trace
gases—supports
this
implies
that
CO2
was
300–350
ppm
in
Pliocene
about
450
at
transition
to
a
nearly
ice-free
planet,
exposing
unrealistic
lethargy
sheet
models.
Equilibrium
warming
today’s
GHG
amount
10°C,
reduced
8°C
human-made
aerosols.
not
‘committed’
warming;
rapid
phaseout
emissions
would
prevent
most
from
occurring.
However,
decline
aerosol
since
2010
should
increase
1970–2010
rate
0.18°C
decade
post-2010
least
0.27°C
decade.
Thus,
under
present
geopolitical
approach
emissions,
will
exceed
1.5°C
2020s
2°C
before
2050.
Impacts
on
people
nature
accelerate
as
increases
hydrologic
(weather)
extremes.
The
enormity
consequences
demands
return
Holocene-level
temperature.
Required
actions
include:
(1)
increasing
price
accompanied
development
abundant,
affordable,
dispatchable
clean
energy,
(2)
East-West
cooperation
way
accommodates
developing
world
needs,
(3)
intervention
with
Earth’s
radiation
imbalance
phase
down
massive
‘geo-transformation’
climate.
Current
political
crises
an
opportunity
reset,
especially
if
young
can
grasp
their
situation.
Proceedings of the National Academy of Sciences,
Journal Year:
2022,
Volume and Issue:
119(46)
Published: Nov. 7, 2022
How
clouds
respond
to
anthropogenic
sulfate
aerosols
is
one
of
the
largest
sources
uncertainty
in
radiative
forcing
climate
over
industrial
era.
This
limits
our
ability
predict
equilibrium
sensitivity
(ECS)-the
global
warming
following
a
doubling
atmospheric
CO2.
Here,
we
use
satellite
observations
quantify
relationships
between
and
low-level
while
carefully
controlling
for
meteorology.
We
then
combine
with
estimates
change
concentration
since
about
1850
constrain
associated
forcing.
estimate
that
cloud-mediated
from
[Formula:
see
text]
W
m-2
ocean
(95%
confidence).
constraint
implies
ECS
likely
2.9
4.5
K
(66%
Our
results
indicate
aerosol
less
uncertain
probably
larger
than
ranges
proposed
by
recent
assessments.
Surveys in Geophysics,
Journal Year:
2024,
Volume and Issue:
45(6), P. 1757 - 1783
Published: May 7, 2024
Abstract
Satellite
observations
from
the
Clouds
and
Earth’s
Radiant
Energy
System
show
that
energy
imbalance
has
doubled
0.5
±
0.2
Wm
−2
during
first
10
years
of
this
century
to
1.0
−
2
past
decade.
The
increase
is
result
a
0.9
0.3
absorbed
solar
radiation
(ASR)
partially
offset
by
0.4
0.25
in
outgoing
longwave
(OLR).
Despite
marked
differences
ASR
OLR
trends
hiatus
(2000–2010),
transition-to-El
Niño
(2010–2016)
post-El
(2016–2022)
periods,
net
top-of-atmosphere
flux
(NET)
remain
within
0.1
per
decade
one
another,
implying
steady
acceleration
climate
warming.
Northern
southern
hemisphere
NET
are
consistent
0.06
0.31
due
compensation
between
weak
hemispheric
trend
opposite
sign.
We
find
large
decreases
stratocumulus
middle
clouds
over
sub-tropics
low
at
mid-latitudes
primary
reasons
for
increasing
northern
(NH).
These
changes
especially
eastern
Pacific
Ocean,
coincide
with
increases
sea-surface
temperature
(SST).
decrease
cloud
fraction
higher
SSTs
NH
lead
significant
cloud-free
regions,
which
compensate
increase.
Decreases
reflection
weaker
reduction
low-cloud
account
hemisphere,
while
weak.
Changes
cover
response
SST
imply
feedback
change
yet
contribution
radiative
forcing
or
internal
variability
cannot
be
ruled
out.
Geophysical Research Letters,
Journal Year:
2023,
Volume and Issue:
50(2)
Published: Jan. 18, 2023
Abstract
A
supervised
neural
network
algorithm
is
used
to
categorize
near‐global
satellite
retrievals
into
three
mesoscale
cellular
convective
(MCC)
cloud
morphology
patterns.
At
constant
amount,
patterns
differ
in
brightness
associated
with
the
amount
of
optically
thin
features.
Environmentally
driven
transitions
from
closed
MCC
other
patterns,
typically
accompanied
by
more
features,
are
as
a
framework
quantify
contribution
optical
depth
component
shortwave
feedback.
marine
heat
wave
an
out‐of‐sample
test
occurrence
predictions.
Morphology
shifts
between
65°S
and
65°N
under
projected
environmental
changes
(i.e.,
abrupt
quadrupling
CO
2
)
assuming
cover
contributes
0.04
0.07
W
m
−2
K
−1
(aggregate
0.06)
global
mean
Atmospheric chemistry and physics,
Journal Year:
2023,
Volume and Issue:
23(2), P. 1073 - 1090
Published: Jan. 20, 2023
Abstract.
Marine
stratocumuli
cool
the
Earth
effectively
due
to
their
high
reflectance
of
incoming
solar
radiation
and
persistent
occurrence.
The
susceptibility
cloud
albedo
droplet
number
concentration
perturbations
depends
strongly
on
large-scale
meteorological
conditions.
Studies
focused
dependence
adjustments
often
overlook
covariability
among
factors
geographical
temporal
variability.
We
use
8
years
satellite
observations
sorted
by
day
location
show
global
distribution
marine
low-cloud
susceptibility.
find
an
overall
brightening
potential
for
most
warm
clouds,
which
is
more
pronounced
over
subtropical
coastal
regions.
A
weak
darkening
in
annual
mean
evident
remote
SE
Pacific
Atlantic.
that
fields
from
ERA5
reanalysis
data,
including
lower-tropospheric
stability,
free-tropospheric
relative
humidity,
sea
surface
temperature,
boundary
layer
depth,
have
distinct
covariabilities
each
eastern
ocean
basins
where
prevail.
This
leads
a
markedly
different
cycle
basin.
Moreover,
we
basin-specific
regional
relationships
between
key
susceptibilities
are
absent
analysis.
Our
results
stress
importance
considering
distinctiveness
when
scaling
up
local-to-global
response
aerosol
perturbations.
Nature Geoscience,
Journal Year:
2023,
Volume and Issue:
16(12), P. 1092 - 1098
Published: Nov. 20, 2023
Abstract
The
impact
of
anthropogenic
aerosols
on
clouds
is
a
leading
source
uncertainty
in
estimating
the
effect
human
activity
climate
system.
challenge
lies
scale
difference
between
(~1–10
km)
and
general
circulation
(>1,000
km).
To
address
this,
we
use
convection-permitting
simulations
conducted
long
narrow
domain,
to
resolve
convection
while
also
including
representation
large-scale
processes.
We
examine
set
that
include
sea
surface
temperature
gradient—which
drives
circulation—and
compare
these
with
no
gradient.
show
effective
radiative
forcing
due
aerosol–cloud
interactions
strongly
enhanced
by
adjustments
aerosol.
find
an
increase
aerosol
concentration
suppresses
precipitation
shallow-convective
regions,
which
enhances
water
vapour
transport
portion
domain
dominated
deep
convection.
subsequent
latent
heat
release
deep-convective
regions
strengthens
overturning
evaporation.
These
changes
can
explain
cloudiness
under
higher
concentrations
and,
consequently,
large
effect.
This
work
highlights
fundamental
importance
understanding
from
interactions.
Atmospheric chemistry and physics,
Journal Year:
2023,
Volume and Issue:
23(20), P. 13125 - 13141
Published: Oct. 18, 2023
Abstract.
Interactions
between
aerosols
and
liquid
clouds
are
one
of
the
largest
sources
uncertainty
in
historical
radiative
forcing
climate.
One
widely
shared
goal
to
reduce
this
is
decompose
anomalies
arising
from
aerosol–cloud
interactions
into
components
associated
with
changes
cloud-droplet
number
concentration
(Twomey
effect),
liquid-water-path
adjustments,
cloud-fraction
adjustments.
However,
there
has
not
been
a
quantitative
foundation
for
simultaneously
estimating
these
global
satellite
observations.
Here
we
present
method
assessing
shortwave
flux
Twomey
effect
cloud
adjustments
over
ocean
55∘
S
N.
We
find
that
larger
aerosol
concentrations
widespread
brightening
effect,
positive
adjustment
decreasing
water
path
subtropical
stratocumulus
regions,
negative
increasing
fraction
subtropics
midlatitudes.
The
total
have
contributed
−0.77
±
0.25
−1.02
0.43
W
m−2,
respectively,
effective
since
1850
domain
(95
%
confidence).
Our
findings
suggest
make
contribution
than
commonly
believed.
npj Climate and Atmospheric Science,
Journal Year:
2024,
Volume and Issue:
7(1)
Published: March 22, 2024
Abstract
Southern
Ocean
(SO)
air
is
amongst
the
most
pristine
on
Earth,
particularly
during
winter.
Historically,
there
has
been
a
focus
biogenic
sources
as
an
explanation
for
seasonal
cycle
in
cloud
condensation
nuclei
concentrations
(
N
CCN
).
also
sensitive
to
strength
of
sink
terms,
although
magnitude
this
term
varies
considerably.
Wet
deposition,
process
encompassing
coalescence
scavenging
(drizzle
formation),
one
such
that
may
be
especially
relevant
over
SO.
Using
boundary
layer
climatology,
and
precipitation
observations
from
Kennaook/Cape
Grim
Observatory
(CGO),
we
find
statistically
significant
difference
between
when
upwind
meteorology
dominated
by
open
mesoscale
cellular
convection
(MCC)
closed
MCC.
When
MCC
dominant,
lower
median
(69
cm
−3
)
found
compared
(89
dominant.
Open
precipitate
more
heavily
(1.72
mm
day
−1
frequently
(16.7%
time)
than
(0.29
,
4.5%).
These
relationships
are
observed
hold
across
with
maximum
minimum
Austral
summer
(DJF).
Furthermore,
morphology
strongly
depends
meteorological
conditions.
The
relationship
can
further
examined
diurnal
season.
Although
was
again
negative
out
phase
cycle,
leading
it
~3
hours,
suggesting
other
factors,
specifically
play
primary
role
influencing
precipitation.
Atmospheric chemistry and physics,
Journal Year:
2025,
Volume and Issue:
25(4), P. 2123 - 2146
Published: Feb. 19, 2025
Abstract.
Aerosol–cloud
interactions
(ACIs)
are
a
leading
source
of
uncertainty
in
estimates
the
historical
effective
radiative
forcing
(ERF).
One
reason
for
this
is
difficulty
estimating
ERF
from
aerosol–cloud
(ERFaci)
climate
models,
which
typically
requires
multiple
calls
to
radiation
code.
Most
commonly
used
methods
also
cannot
disentangle
contributions
different
processes
ERFaci.
Here,
we
develop
new,
computationally
efficient
method
shortwave
(SW)
ERFaci
liquid
clouds
using
histograms
monthly
averaged
cloud
fraction
partitioned
by
droplet
radius
(re)
and
water
path
(LWP).
Multiplying
with
SW
kernels
gives
total
clouds,
can
be
decomposed
into
Twomey
effect,
LWP
adjustments,
(CF)
adjustments.
We
test
data
five
CMIP6-era
Moderate
Resolution
Imaging
Spectroradiometer
(MODIS)
satellite
instrument
simulator
generate
histograms.
Our
similar
other
established
regions
prevalent
indicates
that
CF
adjustments
have
contributed
−0.34
±
0.23,
−0.22
0.13,
−0.09
0.11
W
m−2,
respectively,
since
1850
ensemble
mean
(95
%
confidence).
These
results
demonstrate
widespread
adoption
MODIS
re–LWP
joint
histogram
diagnostic
would
allow
its
components
quickly
accurately
diagnosed
model
outputs,
crucial
step
reducing
ERF.
Atmospheric chemistry and physics,
Journal Year:
2025,
Volume and Issue:
25(8), P. 4443 - 4454
Published: April 23, 2025
Abstract.
In
2020,
the
International
Maritime
Organization
(IMO)
implemented
strict
new
regulations
on
emissions
of
sulfate
aerosol
from
world's
shipping
fleet.
This
can
be
expected
to
lead
a
reduction
in
aerosol-driven
cooling,
unmasking
portion
greenhouse
gas
warming.
The
magnitude
effect
is
uncertain,
however,
due
large
remaining
uncertainties
climate
response
aerosols.
Here,
we
investigate
this
question
using
an
18-member
ensemble
fully
coupled
simulations
evenly
sampling
key
modes
variability
with
NCAR
model,
Community
Earth
System
Model
version
2
(CESM2).
We
show
that,
while
there
clear
physical
system
IMO
regulations,
including
surface
temperature
increase,
do
not
find
global
mean
influence
that
significantly
different
zero.
20-year
average
warming
for
2020–2040
+0.03
°C,
5
%–95
%
confidence
range
[-0.09,0.19],
reflecting
weakness
perturbation
relative
internal
variability.
do,
robust,
non-zero
regional
part
North
Atlantic.
also
maximum
annual
and
occurs
around
1
decade
after
2029,
which
means
have
likely
had
very
limited
observed
date.
further
discuss
our
results
light
other,
recent
publications
reached
conclusions.
Overall,
may
contribute
up
0.16
°C
[-0.17,0.52]
individual
years
during
decade,
consistent
some
early
studies,
such
unlikely
been
discernible
above
by
end
2023
fact
zero
throughout
period.