Atmospheric chemistry and physics,
Journal Year:
2021,
Volume and Issue:
21(5), P. 3427 - 3446
Published: March 5, 2021
Abstract.
Long-range
transport
of
biogenic
emissions
from
the
coast
Antarctica,
precipitation
scavenging,
and
cloud
processing
are
main
processes
that
influence
observed
variability
in
Southern
Ocean
(SO)
marine
boundary
layer
(MBL)
condensation
nuclei
(CN)
(CCN)
concentrations
during
austral
summer.
Airborne
particle
measurements
on
HIAPER
GV
north–south
transects
between
Hobart,
Tasmania,
62∘
S
Clouds,
Radiation
Aerosol
Transport
Experimental
Study
(SOCRATES)
were
separated
into
four
regimes
comprising
combinations
high
low
CCN
CN.
In
5
d
HYSPLIT
back
trajectories,
air
parcels
with
elevated
almost
always
shown
to
have
crossed
Antarctic
coast,
a
location
phytoplankton
relative
rest
SO
region
south
Australia.
The
presence
was
also
consistent
fractions
over
their
trajectory,
suggesting
there
substantial
growth
biogenically
formed
particles
through
processing.
Cases
fraction,
due
cumulus
clouds,
had
CN
concentrations,
previously
reported
new
formation
outflow
regions.
Measurements
associated
previous
1.5
trajectory
indicating
effectively
scavenged
by
precipitation.
A
coarse-mode
fitting
algorithm
used
determine
primary
aerosol
(PMA)
contribution,
which
accounted
for
<20
%
(at
0.3
supersaturation)
droplet
number
concentrations.
Vertical
profiles
large
(Dp>0.07
µm)
indicated
occurs
more
frequently
above
MBL;
however,
recently
typically
MBL,
volatile
compound
oxidation
products.
R/V
Investigator
as
part
second
Aerosols,
Precipitation,
atmospheric
Composition
Over
southeRn
(CAPRICORN-2)
campaign
conducted
same
period
SOCRATES
study.
near
Australia,
likely
continental
coastal
emissions.
source
south,
sources
midlatitudes,
enhanced
sink
cyclonic
circulation
Ferrel
polar
cells
(around
60∘
S)
create
opposing
latitudinal
gradients
concentration
an
minimum
55
S.
airborne
not
influenced
Australian
but
still
show
evidence
S,
addition,
gradient
composition,
Tasmanian
coasts,
is
apparent
hygroscopicity
derived
spectra
size
distribution.
hygroscopic
north,
greater
fraction
sea
salt
PMA,
less
sulfate
organic
originating
Antarctica.
Nature Reviews Microbiology,
Journal Year:
2019,
Volume and Issue:
17(9), P. 569 - 586
Published: June 18, 2019
In
the
Anthropocene,
in
which
we
now
live,
climate
change
is
impacting
most
life
on
Earth.
Microorganisms
support
existence
of
all
higher
trophic
forms.
To
understand
how
humans
and
other
forms
Earth
(including
those
are
yet
to
discover)
can
withstand
anthropogenic
change,
it
vital
incorporate
knowledge
microbial
'unseen
majority'.
We
must
learn
not
just
microorganisms
affect
production
consumption
greenhouse
gases)
but
also
they
will
be
affected
by
human
activities.
This
Consensus
Statement
documents
central
role
global
importance
biology.
It
puts
humanity
notice
that
impact
depend
heavily
responses
microorganisms,
essential
for
achieving
an
environmentally
sustainable
future.
The
majority
with
share
often
goes
unnoticed
despite
underlying
major
biogeochemical
cycles
food
webs,
thereby
taking
a
key
change.
highlights
microbiology
issues
call
action
microbiologists.
Geophysical Research Letters,
Journal Year:
2019,
Volume and Issue:
46(14), P. 8329 - 8337
Published: July 16, 2019
Abstract
The
Community
Earth
System
Model
Version
2
(CESM2)
has
an
equilibrium
climate
sensitivity
(ECS)
of
5.3
K.
ECS
is
emergent
property
both
feedbacks
and
aerosol
forcing.
increase
in
over
the
previous
version
(CESM1)
result
cloud
feedbacks.
Interim
versions
CESM2
had
a
land
model
that
damped
ECS.
Part
change
results
from
evolving
configuration
to
reproduce
long‐term
trend
global
regional
surface
temperature
twentieth
century
response
forcings.
Changes
made
reduce
aerosols
also
impacted
feedbacks,
which
significantly
influence
simulations
compare
very
well
observations
present
climate.
It
critical
understand
whether
high
ECS,
outside
best
estimate
range
1.5–4.5
K,
plausible.
Journal of Geophysical Research Atmospheres,
Journal Year:
2019,
Volume and Issue:
124(23), P. 13026 - 13054
Published: Oct. 23, 2019
Abstract
Aerosols
have
significant
and
complex
impacts
on
regional
climate
in
East
Asia.
Cloud‐aerosol‐precipitation
interactions
(CAPI)
remain
most
challenging
studies.
The
quantitative
understanding
of
CAPI
requires
good
knowledge
aerosols,
ranging
from
their
formation,
composition,
transport,
radiative,
hygroscopic,
microphysical
properties.
A
comprehensive
review
is
presented
here
centered
the
based
chiefly,
but
not
limited
to,
publications
special
section
named
EAST‐AIRcpc
concerning
(1)
observations
aerosol
loading
properties,
(2)
relationships
between
aerosols
meteorological
variables
affecting
CAPI,
(3)
mechanisms
behind
(4)
quantification
impact
climate.
Heavy
Asia
has
radiative
effects
by
reducing
surface
radiation,
increasing
air
temperature,
lowering
boundary
layer
height.
key
factor
absorption,
which
particularly
strong
central
China.
This
absorption
can
a
wide
range
such
as
creating
an
imbalance
forcing
at
top
bottom
atmosphere,
leading
to
inconsistent
retrievals
cloud
space‐borne
ground‐based
instruments.
Aerosol
delay
or
suppress
initiation
development
convective
clouds
whose
microphysics
be
further
altered
effect
aerosols.
For
same
thickness,
likelihood
precipitation
influenced
aerosols:
suppressing
light
rain
enhancing
heavy
rain,
delaying
intensifying
thunderstorms,
onset
isolated
showers
parts
Rainfall
become
more
inhomogeneous
extreme
heavily
polluted
urban
regions.
Proceedings of the National Academy of Sciences,
Journal Year:
2020,
Volume and Issue:
117(30), P. 17591 - 17598
Published: July 13, 2020
Significance
All
cloud
droplets
on
Earth
form
from
tiny
airborne
particles
known
as
aerosols.
Additional
aerosols
anthropogenic
activity
have
produced
more
but
at
smaller
sizes.
The
smaller,
numerous
in
clouds
do
not
collide
effectively,
therefore
resulting
less
precipitation.
Using
a
combination
of
time-lapse
satellite
imagery
and
air
mass
trajectory
modeling,
we
show
that
can
enhance
fraction
extend
the
lifetime
overcast
fields
primarily
under
stable
atmospheric
conditions
typically
found
off
west
coasts
subtropical
stratocumulus-dominated
regions.
Longer-lived
stronger
cooling
influence
climate
therefore,
need
to
be
correctly
parameterized
models
so
accurate
projections
change
achieved.
Atmospheric chemistry and physics,
Journal Year:
2019,
Volume and Issue:
19(16), P. 10497 - 10523
Published: Aug. 21, 2019
Abstract.
Aerosol
optical
depth
(AOD)
has
become
a
crucial
metric
for
assessing
global
climate
change.
Although
and
regional
AOD
trends
have
been
studied
extensively,
it
remains
unclear
what
factors
are
driving
the
inter-decadal
variations
in
how
to
quantify
relative
contribution
of
each
dominant
factor.
This
study
used
long-term
(1980–2016)
aerosol
dataset
from
Modern-Era
Retrospective
Analysis
Research
Applications,
version
2
(MERRA-2)
reanalysis,
along
with
two
satellite-based
datasets
(MODIS/Terra
MISR)
2001
2016,
investigate
loading.
Statistical
models
based
on
emission
meteorological
parameters
were
developed
identify
main
changes
their
contribution.
Evaluation
MERRA-2
ground-based
measurements
AERONET
indicated
significant
spatial
agreement
scale
(r=
0.85,
root-mean-square
error
=
0.12,
mean
fractional
38.7
%,
gross
9.86
%
index
0.94).
However,
when
observations
China
Remote
Sensing
Network
(CARSNET)
employed
independent
verification,
results
showed
that
AODs
generally
underestimated
CARSNET
(relative
bias
0.72
=-34.3
%).
In
general,
was
able
quantitatively
reproduce
annual
seasonal
both
scales,
as
observed
by
MODIS/Terra,
although
some
differences
found
compared
MISR.
Over
37-year
period
this
study,
decreasing
over
Europe
eastern
United
States.
contrast,
southern
Asia
increases,
but
increasing
trend
former
reversed
sharply
most
recent
decade.
The
statistical
analyses
suggested
explained
larger
proportion
variability
(20.4
%–72.8
%)
almost
all
regions
interest
(ROIs)
during
1980–2014
(0
%–56
Further
analysis
also
SO2
factor,
explaining
12.7
%–32.6
variation
anthropogenic-aerosol-dominant
regions,
while
black
carbon
or
organic
leading
factor
biomass-burning-dominant
(BBD)
contributing
24.0
%–27.7
variation.
Additionally,
wind
speed
be
parameter,
11.8
%–30.3
variance
mineral-dust-dominant
ambient
humidity
(including
soil
moisture
humidity)
top
parameter
BBD
accounting
11.7
%–35.5
indicate
is
key
determining
change
AOD.
Nature Communications,
Journal Year:
2019,
Volume and Issue:
10(1)
Published: Sept. 30, 2019
Abstract
Particles
formed
in
the
atmosphere
via
nucleation
provide
about
half
number
of
atmospheric
cloud
condensation
nuclei,
but
many
locations,
this
process
is
limited
by
growth
newly
particles.
That
often
organic
vapors.
Identification
these
vapors
and
their
sources
thus
fundamental
for
simulating
changes
to
aerosol-cloud
interactions,
which
are
one
most
uncertain
aspects
anthropogenic
climate
forcing.
Here
we
present
direct
molecular-level
observations
a
distribution
forested
environment
that
can
explain
simultaneously
observed
nanoparticle
from
3
50
nm.
Furthermore,
volatility
sufficient
without
invoking
particle-phase
processes.
The
agreement
between
mass
growth,
predicted
condensing
represents
an
important
step
forward
characterization
particle
growth.
Journal of Advances in Modeling Earth Systems,
Journal Year:
2019,
Volume and Issue:
11(6), P. 1735 - 1758
Published: May 17, 2019
Abstract
We
analyze
the
atmospheric
processes
that
explain
large
changes
in
radiative
feedbacks
between
two
latest
climate
configurations
of
Hadley
Centre
Global
Environmental
model.
use
a
set
atmosphere‐only
change
simulations
(
amip
and
amip‐p4K
)
to
separate
contributions
differences
feedback
parameter
from
all
model
developments
configurations.
show
are
mostly
driven
by
shortwave
cloud
midlatitudes,
mainly
over
Southern
Ocean.
Two
new
schemes
most
differences:
introduction
aerosol
scheme
development
mixed‐phase
scheme.
Both
reduce
strength
preexisting
negative
midlatitudes.
The
dampens
strong
aerosol‐cloud
interaction,
it
also
suppresses
clear‐sky
feedback.
increases
amount
liquid
water
path
(LWP)
present
day
reduces
increase
LWP
with
warming.
contribute
reducing
warmer
climate.
enhances
strong,
preexisting,
positive
fraction
assess
realism
comparing
present‐day
against
observations
discuss
avenues
could
help
constrain
relevant
processes.