Nano Letters,
Journal Year:
2024,
Volume and Issue:
24(28), P. 8453 - 8464
Published: May 21, 2024
Material
advances
in
soft
bioelectronics,
particularly
those
based
on
stretchable
nanocomposites─functional
nanomaterials
embedded
viscoelastic
polymers
with
irreversible
or
reversible
bonds─have
driven
significant
progress
translational
medical
device
research.
The
unique
mechanical
properties
inherent
the
nanocomposites
enable
stiffness
matching
between
tissue
and
device,
as
well
its
spontaneous
adaptation
to
Chemical Reviews,
Journal Year:
2024,
Volume and Issue:
124(18), P. 10435 - 10508
Published: Sept. 16, 2024
The
mechanical
properties
of
polymer
gels
devote
to
emerging
devices
and
machines
in
fields
such
as
biomedical
engineering,
flexible
bioelectronics,
biomimetic
actuators,
energy
harvesters.
Coupling
network
architectures
interactions
has
been
explored
regulate
supportive
characteristics
gels;
however,
systematic
reviews
correlating
mechanics
interaction
forces
at
the
molecular
structural
levels
remain
absent
field.
This
review
highlights
engineering
gel
a
comprehensive
mechanistic
understanding
regulation.
Molecular
alters
architecture
manipulates
functional
groups/moieties
level,
introducing
various
permanent
or
reversible
dynamic
bonds
dissipative
energy.
usually
uses
monomers,
cross-linkers,
chains,
other
additives.
Structural
utilizes
casting
methods,
solvent
phase
regulation,
mechanochemistry,
macromolecule
chemical
reactions,
biomanufacturing
technology
construct
tailor
topological
structures,
heterogeneous
modulus
compositions.
We
envision
that
perfect
combination
may
provide
fresh
view
extend
exciting
new
perspectives
this
burgeoning
also
summarizes
recent
representative
applications
with
excellent
properties.
Conclusions
are
provided
from
five
aspects
concise
summary,
mechanism,
biofabrication
upgraded
applications,
synergistic
methodology.
Nano Letters,
Journal Year:
2024,
Volume and Issue:
24(28), P. 8453 - 8464
Published: May 21, 2024
Material
advances
in
soft
bioelectronics,
particularly
those
based
on
stretchable
nanocomposites─functional
nanomaterials
embedded
viscoelastic
polymers
with
irreversible
or
reversible
bonds─have
driven
significant
progress
translational
medical
device
research.
The
unique
mechanical
properties
inherent
the
nanocomposites
enable
stiffness
matching
between
tissue
and
device,
as
well
its
spontaneous
adaptation
to
