Atmospheric chemistry and physics,
Journal Year:
2022,
Volume and Issue:
22(3), P. 2095 - 2119
Published: Feb. 15, 2022
Abstract.
Mineral
dust
impacts
key
processes
in
the
Earth
system,
including
radiation
budget,
clouds,
and
nutrient
cycles.
We
evaluate
aerosols
16
models
participating
sixth
phase
of
Coupled
Model
Intercomparison
Project
(CMIP6)
against
multiple
reanalyses
observations.
note
that
both
observations
used
here
have
their
limitations
particularly
emission
deposition
are
poorly
constrained.
Most
models,
multi-model
ensemble
mean
(MEM),
capture
spatial
patterns
seasonal
cycles
global
well.
However,
large
uncertainties
inter-model
diversity
found.
For
example,
emissions,
primarily
driven
by
model-simulated
surface
winds,
vary
a
factor
5
across
while
MEM
estimate
is
double
amount
reanalyses.
The
ranges
CMIP6
emission,
deposition,
burden,
optical
depth
(DOD)
larger
than
previous
generations
models.
Models
present
considerable
disagreement
over
North
China
America.
Here,
DOD
values
overestimated
most
with
1.2–1.7
times
compared
to
satellite
reanalysis
datasets.
Such
overestimates
can
reach
up
individual
also
fail
reproduce
some
features
regional
distribution,
such
as
accumulation
along
southern
edge
Himalayas.
Overall,
there
still
models'
simulated
processes,
which
feature
inconsistent
biases
throughout
life
cycle
between
relationship
connecting
mass
DOD.
Our
results
imply
modelled
becoming
more
uncertain
become
sophisticated.
More
detailed
output
size-resolved
variables
particular,
relating
future
intercomparison
projects,
needed
enable
better
constraints
potential
identification
observationally
constrained
links
properties.
Geophysical Research Letters,
Journal Year:
2021,
Volume and Issue:
48(4)
Published: Jan. 21, 2021
Abstract
The
Southern
Hemisphere
(SH)
surface
westerlies
fundamentally
control
regional
patterns
of
air
temperature,
storm
tracks,
and
precipitation
while
also
regulating
ocean
circulation,
heat
transport
carbon
uptake.
Wind‐forced
perturbation
experiments
commonly
apply
idealized
poleward
wind
shifts
ranging
between
0.5
10
degrees
latitude
intensification
factors
10%
300%.
In
addition,
changes
in
winds
are
often
prescribed
ad
hoc
as
a
zonally
uniform
anomaly
that
neglects
important
seasonal
differences.
Here
we
quantify
historical
projected
SH
westerly
based
on
examination
CMIP5,
CMIP6,
reanalysis
data.
We
find
significant
reduction
the
location
bias
CMIP6
ensemble
an
associated
shift
compared
to
CMIP5.
Under
high
emission
scenario,
end
21st
Century
mean
increase
∼10%
∼0.8°
latitude,
although
there
variations.
Atmospheric chemistry and physics,
Journal Year:
2021,
Volume and Issue:
21(6), P. 5015 - 5061
Published: March 31, 2021
Abstract.
Stratospheric
ozone
and
water
vapour
are
key
components
of
the
Earth
system,
past
future
changes
to
both
have
important
impacts
on
global
regional
climate.
Here,
we
evaluate
long-term
in
these
species
from
pre-industrial
period
(1850)
end
21st
century
Coupled
Model
Intercomparison
Project
phase
6
(CMIP6)
models
under
a
range
emissions
scenarios.
There
is
good
agreement
between
CMIP
multi-model
mean
observations
for
total
column
(TCO),
although
there
substantial
variation
individual
CMIP6
models.
For
mean,
TCO
has
increased
∼
300
DU
1850
305
1960,
before
rapidly
declining
1970s
1980s
following
use
emission
halogenated
ozone-depleting
substances
(ODSs).
projected
return
1960s
values
by
middle
SSP2-4.5,
SSP3-7.0,
SSP4-3.4,
SSP4-6.0,
SSP5-8.5
scenarios,
SSP3-7.0
scenarios
be
10
higher
than
2100.
However,
SSP1-1.9
SSP1-1.6
not
despite
reductions
ODSs
due
decreases
tropospheric
mixing
ratios.
This
pattern
similar
patterns,
except
tropics
where
most
values,
either
through
SSP1-2.6,
or
lower
stratospheric
resulting
an
acceleration
Brewer–Dobson
circulation
other
Shared
Socioeconomic
Pathways
(SSPs).
In
contrast
TCO,
poorer
observed
ratios,
with
underestimating
ratios
0.5
ppmv
at
70
hPa.
tropical
stratosphere
present-day
increase
further
century.
The
largest
increases
(∼
2
ppmv)
simulated
highest
assumed
forcing
pathway
(e.g.
SSP5-8.5).
Tropical
vapour,
lesser
extent
shows
large
variations
explosive
volcanic
eruptions.
Atmospheric chemistry and physics,
Journal Year:
2021,
Volume and Issue:
21(2), P. 853 - 874
Published: Jan. 21, 2021
Abstract.
This
paper
quantifies
the
pre-industrial
(1850)
to
present-day
(2014)
effective
radiative
forcing
(ERF)
of
anthropogenic
emissions
NOX,
volatile
organic
compounds
(VOCs;
including
CO),
SO2,
NH3,
black
carbon,
and
concentrations
methane,
N2O
ozone-depleting
halocarbons,
using
CMIP6
models.
Concentration
emission
changes
reactive
species
can
cause
multiple
in
composition
radiatively
active
species:
tropospheric
ozone,
stratospheric
water
vapour,
secondary
inorganic
aerosol,
methane.
Where
possible
we
break
down
ERFs
from
each
emitted
into
contributions
changes.
The
are
calculated
for
models
that
participated
AerChemMIP
experiments
as
part
project,
where
relevant
model
output
was
available.
1850
2014
multi-model
mean
(±
standard
deviations)
−1.03
±
0.37
W
m−2
SO2
emissions,
−0.25
0.09
carbon
(OC),
0.15
0.17
(BC)
−0.07
0.01
NH3.
For
combined
aerosols
(in
piClim-aer
experiment)
it
is
−1.01
0.25
m−2.
means
well-mixed
greenhouse
gases
(including
any
effects
on
ozone
aerosol
chemistry)
0.67
methane
(CH4),
0.26
0.07
nitrous
oxide
(N2O)
0.12
0.2
halocarbons
(HC).
Emissions
precursors
nitrogen
oxides
(NOx),
both
together
(O3)
lead
0.14
0.13,
0.20
respectively.
differences
different
reflect
complexity
their
chemistry
schemes,
especially
case
captures
increased
production.
Earth system science data,
Journal Year:
2022,
Volume and Issue:
14(12), P. 5573 - 5603
Published: Dec. 16, 2022
Abstract.
A
multitude
of
physical
and
biological
processes
on
which
ecosystems
human
societies
depend
are
governed
by
the
climate,
understanding
how
these
altered
climate
change
is
central
to
mitigation
efforts.
We
developed
a
set
climate-related
variables
at
as
yet
unprecedented
spatiotemporal
detail
basis
for
environmental
ecological
analyses.
downscaled
time
series
near-surface
relative
humidity
(hurs)
cloud
area
fraction
(clt)
under
consideration
orography
wind
well
speed
(sfcWind)
using
delta-change
method.
Combining
grids
with
mechanistically
information
temperature,
precipitation,
solar
radiation,
we
then
calculated
vapor
pressure
deficit
(vpd),
surface
downwelling
shortwave
radiation
(rsds),
potential
evapotranspiration
(pet),
moisture
index
(cmi),
site
water
balance
(swb)
monthly
temporal
30
arcsec
spatial
resolution
globally
from
1980
until
2018
(time-series
variables).
At
same
resolution,
further
estimated
climatological
normals
frost
frequency
(fcf),
snow
cover
days
(scd),
net
primary
productivity
(npp),
growing
degree
(gdd),
season
characteristics
periods
1981–2010,
2011–2040,
2041–2070,
2071–2100,
considering
three
shared
socioeconomic
pathways
(SSP126,
SSP370,
SSP585)
five
Earth
system
models
(projected
Time-series
showed
high
accuracy
when
validated
against
observations
meteorological
stations
compared
alternative
products.
Projected
were
also
highly
correlated
observations,
although
some
notable
biases,
e.g.,
days.
Together,
CHELSA-BIOCLIM+
dataset
presented
here
(https://doi.org/10.16904/envidat.332,
Brun
et
al.,
2022)
allows
improvement
our
patterns
that
including
impact
recent
future
changes
world's
associated
services
societies.
Atmospheric chemistry and physics,
Journal Year:
2022,
Volume and Issue:
22(3), P. 2095 - 2119
Published: Feb. 15, 2022
Abstract.
Mineral
dust
impacts
key
processes
in
the
Earth
system,
including
radiation
budget,
clouds,
and
nutrient
cycles.
We
evaluate
aerosols
16
models
participating
sixth
phase
of
Coupled
Model
Intercomparison
Project
(CMIP6)
against
multiple
reanalyses
observations.
note
that
both
observations
used
here
have
their
limitations
particularly
emission
deposition
are
poorly
constrained.
Most
models,
multi-model
ensemble
mean
(MEM),
capture
spatial
patterns
seasonal
cycles
global
well.
However,
large
uncertainties
inter-model
diversity
found.
For
example,
emissions,
primarily
driven
by
model-simulated
surface
winds,
vary
a
factor
5
across
while
MEM
estimate
is
double
amount
reanalyses.
The
ranges
CMIP6
emission,
deposition,
burden,
optical
depth
(DOD)
larger
than
previous
generations
models.
Models
present
considerable
disagreement
over
North
China
America.
Here,
DOD
values
overestimated
most
with
1.2–1.7
times
compared
to
satellite
reanalysis
datasets.
Such
overestimates
can
reach
up
individual
also
fail
reproduce
some
features
regional
distribution,
such
as
accumulation
along
southern
edge
Himalayas.
Overall,
there
still
models'
simulated
processes,
which
feature
inconsistent
biases
throughout
life
cycle
between
relationship
connecting
mass
DOD.
Our
results
imply
modelled
becoming
more
uncertain
become
sophisticated.
More
detailed
output
size-resolved
variables
particular,
relating
future
intercomparison
projects,
needed
enable
better
constraints
potential
identification
observationally
constrained
links
properties.