Short-Term Stability of Electrochemical Properties of Layer-by-Layer Coated Heterogeneous Ion Exchange Membranes DOI Creative Commons
В. В. Сарапулова,

E. Nevakshenova,

Kseniia Tsygurina

et al.

Membranes, Journal Year: 2022, Volume and Issue: 13(1), P. 45 - 45

Published: Dec. 29, 2022

Layer-by-layer adsorption allows the creation of versatile functional coatings for ion exchange membranes, but stability coating and resulting properties modified membranes in their operation is a frequently asked question. This paper examines changes voltammetric curves layer-by-layer coated cation pH-metry desalination chamber with studied membrane an auxiliary anion after short-term tests, including over-limiting current modes. The practical did not affect curves, enhanced generation H+ OH− ions system polyethylenimine Ca2+ containing solution. It shown that distinction between different polyamines persists during that, case polyethylenimine, there additional zone growth potential drop stronger as indicated by pH-metry.

Language: Английский

Efficient and feasible biocatalysts: Strategies for enzyme improvement. A review DOI
Samah Hashim Albayati,

Nima Ghahremani Nezhad,

Abdulrahman M Taki

et al.

International Journal of Biological Macromolecules, Journal Year: 2024, Volume and Issue: 276, P. 133978 - 133978

Published: July 20, 2024

Language: Английский

Citations

12

A comprehensive review of lipase-catalyzed acidolysis as a method for producing structured glycerides DOI
Veymar G. Tacias-Pascacio, Pedro Abellanas-Pérez, Diandra de Andrades

et al.

International Journal of Biological Macromolecules, Journal Year: 2025, Volume and Issue: unknown, P. 142878 - 142878

Published: April 1, 2025

Language: Английский

Citations

2

The effects of the chemical modification on immobilized lipase features are affected by the enzyme crowding in the support DOI Creative Commons
Pedro Abellanas-Pérez, Diego Carballares, Javier Rocha‐Martín

et al.

Biotechnology Progress, Journal Year: 2023, Volume and Issue: 40(1)

Published: Oct. 12, 2023

In this article, we have analyzed the interactions between enzyme crowding on a given support and its chemical modification (ethylenediamine via carbodiimide route picryl sulfonic (TNBS) of primary amino groups) activity stability. Lipase from Thermomyces lanuginosus (TLL) lipase B Candida antarctica (CALB) were immobilized octyl-agarose beads at two very different loadings, one them exceeding capacity support, well under capacity. Chemical modifications highly loaded lowly biocatalysts gave results in terms stability, which could increase or decrease depending loading. For example, both increased their after while effect was opposite for biocatalysts. Additionally, with TNBS CALB biocatalyst stability activity.

Language: Английский

Citations

11

The nature of the buffer alters the effects of the chemical modification on the stability of immobilized lipases DOI Creative Commons
Pedro Abellanas-Pérez, Diego Carballares, Javier Rocha‐Martín

et al.

Process Biochemistry, Journal Year: 2023, Volume and Issue: 133, P. 20 - 27

Published: Aug. 9, 2023

The objective of this paper was to analyze whether an interaction between the effects buffer nature and chemical modification on enzyme stability exists. For this, lipase B from Candida antarctica (CALB) Thermomyces lanuginosus (TLL) were immobilized octyl agarose beads modified with picryl sulfonic acid (TNBS) ethylenediamine via carbodiimide route. obtained biocatalysts them inactivated in different buffers (2-amino-2-(hydroxymethyl)propane-1,3-diol (Tris)-HCl, N-(2-hydroxyethyl)piperazine-N′-(2-ethanesulfonic acid) (HEPES) or phosphate). A significant found surfaces their stabilities these buffers. While phosphate where lowest for both unmodified enzymes, differences become much smaller after some modifications. In many instances, improves when using a negative other one (e.g., TNBS TLL positive Tris-HCl buffers, amination CALB decreased its HEPES while it almost had no effect phosphate).Thus, clear co-interactions established.

Language: Английский

Citations

9

Mineralization of Lipase from Thermomyces lanuginosus Immobilized on Methacrylate Beads Bearing Octadecyl Groups to Improve Enzyme Features DOI Open Access
José Renato Guimarães, Diego Carballares, Javier Rocha‐Martín

et al.

Catalysts, Journal Year: 2022, Volume and Issue: 12(12), P. 1552 - 1552

Published: Dec. 1, 2022

Lipase from Thermomyces lanuginosus (TLL) has been immobilized on Purolite Lifetech® ECR8806F (viz. methacrylate macroporous resin containing octadecyl groups, designated as C18-TLL), and the enzyme performance compared to that of octyl-agarose, agarose C8-TLL. The hydrolytic activity versus p-nitrophenol butyrate decreased significantly, a lower extent S-methyl mandelate (more than twofold), while triacetin R-methyl mandelate, was higher for biocatalyst prepared using C18 (up almost five-fold). Regarding stability, C18-TLL significantly more stable Next, biocatalysts were mineralized zinc, copper or cobalt phosphates. Mineralization increased this very S-isomer, effects C8-TLL diverse (hydrolytic increase decrease dependent metal substrate). zinc salt treatment stability both biocatalysts, but with impact agarose-C8-TLL. On contrary, treatments intensively C18-TLL. results show even enzymes following same strategy, differences in conformation cause mineralization have activity, specificity.

Language: Английский

Citations

7

Fe3O4@silica-thermolysin: A robust, advantageous, and reusable microbial nanobiocatalyst for proteolysis and milk-clotting DOI
Vitor A. Ungaro,

João Pedro Alves Fairbanks,

Liane M. Rossi

et al.

International Journal of Biological Macromolecules, Journal Year: 2024, Volume and Issue: 278, P. 134503 - 134503

Published: Aug. 5, 2024

Language: Английский

Citations

0

Short-Term Stability of Electrochemical Properties of Layer-by-Layer Coated Heterogeneous Ion Exchange Membranes DOI Creative Commons
В. В. Сарапулова,

E. Nevakshenova,

Kseniia Tsygurina

et al.

Membranes, Journal Year: 2022, Volume and Issue: 13(1), P. 45 - 45

Published: Dec. 29, 2022

Layer-by-layer adsorption allows the creation of versatile functional coatings for ion exchange membranes, but stability coating and resulting properties modified membranes in their operation is a frequently asked question. This paper examines changes voltammetric curves layer-by-layer coated cation pH-metry desalination chamber with studied membrane an auxiliary anion after short-term tests, including over-limiting current modes. The practical did not affect curves, enhanced generation H+ OH− ions system polyethylenimine Ca2+ containing solution. It shown that distinction between different polyamines persists during that, case polyethylenimine, there additional zone growth potential drop stronger as indicated by pH-metry.

Language: Английский

Citations

1